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Removal of Carbon Disulfide from Gas Streams Using Dielectric Barrier Discharge Plasma Coupled with MnO2 Catalysis System

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Abstract

The removal of gaseous carbon disulfide (CS2) via dielectric barrier discharge (DBD) combined with MnO2 catalysis has been investigated. CS2 removal and energy yield (EY) had been examined as a function of catalyzer position in DBD reactor, initial CS2 concentration, input power, and gas residence time. The results showed that DBD combined with MnO2 catalyst can improve the CS2 energy and removal efficiency, and MnO2 catalyst placed in afterglow area can enhance the CS2 removal efficiency by about 10 % as compared with DBD treatment only. When increasing initial CS2 concentration and flow rate, a higher EY is obtained. The possible CS2 removal pathways by DBD combined with MnO2 were proposed based on the product identification by FT-IR.

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Acknowledgments

The authors wish to thank the Scientific Research Foundation for the Returned overseas Chinese Scholars, Ministry of Education of China (2012JYLH0426); Natural Science Foundation of China (NSFC) (21177034) and Key Laboratory of Environmental Science and Engineering of Jiangsu province, China (ZD071202) for support this study.

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Authors and Affiliations

  1. School of Resources and Environmental Engineering, Hefei University of Technology, Hefei, 230009, People’s Republic of China

    Chengzhu Zhu, Xiaohui Wang, Qin Huang & Jiaquan Wang

  2. Center of Analysis and Measurement, Hefei University of Technology, Hefei, 230009, People’s Republic of China

    Jun Lu

  3. New York State Department of Health, Wadsworth Center, Albany, NY, 12201-0509, USA

    Li Huang

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  1. Chengzhu Zhu
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  2. Jun Lu
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  3. Xiaohui Wang
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  4. Qin Huang
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  5. Li Huang
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  6. Jiaquan Wang
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Correspondence to Li Huang or Jiaquan Wang.

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Zhu, C., Lu, J., Wang, X. et al. Removal of Carbon Disulfide from Gas Streams Using Dielectric Barrier Discharge Plasma Coupled with MnO2 Catalysis System. Plasma Chem Plasma Process 33, 569–579 (2013). https://doi.org/10.1007/s11090-013-9446-8

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  • DOI: https://doi.org/10.1007/s11090-013-9446-8

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