Skip to main content
Log in

A model for the shear viscosity of non-colloidal suspensions with Newtonian matrix fluids

  • Original Contribution
  • Published:
Rheologica Acta Aims and scope Submit manuscript

Abstract

We present a model for the shear viscosity of non-colloidal suspensions with Newtonian matrix fluids. The model is based on the original idea first presented by Brinkman (Applied Sci Research A1:27-34. 1947) for the viscous force exerted by a flowing fluid on a dense swarm of spherical particles. In particular, we consider an inertialess suspension in which the mean flow is driven by a pressure difference, and simultaneously, the suspension is subject to simple shear. Assuming steady state, incompressibility and taking into account a resistance force which is generated due to the presence of the particles in the flow, the three-dimensional governing equations for the mean flow around a single spherical particle are solved analytically. Self-consistency of the model provides a relationship between the resistance parameter and the volume fraction of the solid phase. A volume, or an ensemble, averaging of the total stress gives the bulk properties and an expression for the relative (bulk) viscosity of the suspension. The viscosity expression reduces to the Einstein limit for dilute suspensions and agrees well with empirical formulas from the literature in the semi-dilute and concentrated regimes. Since the model is based on a single particle and its average interaction with the other particles is isotropic, no normal stress differences can be predicted. A possible method of addressing this problem is provided in the paper.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5

Similar content being viewed by others

References

  • Batchelor GK (1970) The stress system in a suspension of force-free particles. J Fluid Mech 41:545–570

    Article  Google Scholar 

  • Batchelor GK, Green JT (1972) The determination of the bulk stress in a suspension of spherical particles to order c2. J Fluid Mech 56(3):401–427

    Article  Google Scholar 

  • Barnes HA (2003) A review of the rheology of filled viscoelastic systems. Rheology Reviews:1–36.

  • Brady JF, Morris JF (1997) Microstructure of strongly sheared suspensions and its impact on rheology and diffusion. J Fluid Mech 348:103–139

    Article  Google Scholar 

  • Bergenholtz J, Brady JF, Vicic M (2002) The non-Newtonian rheology of dilute colloidal suspensions. J Fluid Mech 456:239–275

    Article  Google Scholar 

  • Brinkman HC (1947) A calculation of the viscous force exerted by a flowing fluid on a dense swarm of particles. Appl Sci Res A1:27–34

    Google Scholar 

  • Cox RG, Zia IYZ, Mason SG (1968) Particle motion in sheared suspensions XXV. Streamlines around cylinders and spheres. J Colloid Interface Sci 27(1):7–18

    Article  Google Scholar 

  • Dai SC, Bertevas E, Qi F, Tanner RI (2013) Viscometric functions for non-colloidal sphere suspensions with Newtonian matrices. J Rheology 57:493–510

    Article  Google Scholar 

  • Denn MM, Morris JF (2014) Rheology of non-Brownian suspensions. Ann Rev Chem Biomol Eng 5:203–228

    Article  Google Scholar 

  • Durlofsky L, Brady JF (1987) Analysis of the Brinkman equations as a model for flow in porous media. Phys Fluids 30:3329–3341

    Article  Google Scholar 

  • Einstein A (1906) Eine Neue Bestimmung der Molekul Dimensionen. Ann Phys 19:289–305

    Article  Google Scholar 

  • Einstein A (1911) Berichtigung: Eine Neue Bestimmung der Molekul Dimensionen. Ann Phys 34:591–592

    Article  Google Scholar 

  • Hill RJ, Koch DL, Ladd AJC (2001) The first effects of fluid inertia on flows in ordered and random arrays of spheres. J Fluid Mech 448:213–241

    Google Scholar 

  • Howells ID (1974) Drag due to the motion of a Newtonian fluid through a sparse random array of small fixed rigid objects. J Fluid Mech 64:449–475

    Article  Google Scholar 

  • Housiadas KD, Tanner RI (2012) The drag on a sedimenting sphere in a sheared weakly viscoelastic fluid. J. Non-Newtonian Fluid Mech 183:52–56

    Article  Google Scholar 

  • Kao SV, Cox RG, Mason SG (1977) Streamlines around single spheres and trajectories of pair of spheres in two-dimensional creeping flows. Chem Eng Sci 32:1505–1515

    Article  Google Scholar 

  • Krieger IM, Dougherty TJ (1959) A mechanism for non-Newtonian flow in suspensions at rigid spheres. Trans Soc Rheol 3:137–152

    Article  Google Scholar 

  • Landau LD, Lifshitz EM (1959) Fluid mechanics. Pergamon Press, London

    Google Scholar 

  • Leal LG (2007) Advanced transport phenomena. Cambridge University Press, New York

    Book  Google Scholar 

  • Maron SH, Pierce PE (1956) Application of Ree-Eyring generalized flow theory to suspensions of spherical particles. J Colloid Sci 11:80–95

    Article  Google Scholar 

  • Morris JF (2009) A review of microstructure in concentrated suspensions and its applications for rheology and bulk flow. Rheol Acta 48:909–923

    Article  Google Scholar 

  • Pasquino R, Grizzuti N, Maffettone PL (2008) Rheology of dilute and semidilute noncolloidal hard sphere suspensions. J Rheology 52(6):1369–1384

    Article  Google Scholar 

  • Pivkin IV, Caswell B, Karaniadakis GM (2011) Reviews in computational chemistry, vol 27, chapter 2, edited by Kenny B. Wiley, Lipkowitz

    Google Scholar 

  • Rallison JM (2012) The stress in a dilute suspension of liquid spheres in a second-order fluid. J Fluid Mech 693:500–507

    Article  Google Scholar 

  • Santamaria-Holek I, Mendoza CI (2010) The rheology of concentrated suspensions of arbitrarily-shaped particles. J Colloidal Interface Sci 346:118–126

    Article  Google Scholar 

  • Sierou A, Brady JF (2002) Rheology and microstructure in concentrated noncolloidal suspensions. J Rheology 46:1031–1056

    Article  Google Scholar 

  • Singh A, Nott PR (2000) Normal stresses and microstructure in bounded sheared suspensions via Stokesian dynamics simulations. J Fluid Mech 412:279–301

    Article  Google Scholar 

  • Singh P, Hesla TI, Josheph DD (2003) Distributed Lagrange multiplier method for particulate flows with collisions. Int J Multiph Flow 29(3):495–509

    Article  Google Scholar 

  • Stickel JJ, Powell RP (2005) Fluid mechanics and rheology of dense suspensions. Annu Rev Fluid Mech 37:129–149

    Article  Google Scholar 

  • Tanner RI, Dai SC, Qi F, Housiadas KD (2013a) Viscometric functions of semi-dilute non colloidal suspensions of spheres in a viscoelastic matrix. J Non-Newtonian Fluid Mech 201:130–133

    Article  Google Scholar 

  • Tanner RI, Qi F, Dai S-C (2013b) Scaling the normal stresses in concentrated non-colloidal suspensions of spheres. Rheol Acta 52:201–295

    Article  Google Scholar 

  • Yantsios SG (2012) On the distributed Lagrange multiplier/fictitious domain method for rigid-particle-laden flows: a proposition for an alternative formulation of the Lagrange multipliers. Int J Numer Meth Fluids 70:1027–1047

    Article  Google Scholar 

  • Zarraga IE, Hill DA, Leighton DT (2000) The characterization of the total stress of concentrated suspensions of noncolloidal spheres in Newtonian fluids. J Rheol 44(2):185–220

    Article  Google Scholar 

Download references

Acknowledgment

We thank the Australian Research Council for supporting part of this work via Grant DP110103414.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Kostas D. Housiadas.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Housiadas, K.D., Tanner, R.I. A model for the shear viscosity of non-colloidal suspensions with Newtonian matrix fluids. Rheol Acta 53, 831–841 (2014). https://doi.org/10.1007/s00397-014-0800-4

Download citation

  • Received:

  • Revised:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s00397-014-0800-4

Keywords

Navigation