Abstract
Difference frequency generation is a flexible method for the generation of mid-infrared light. It allows downshifting a near-infrared optical signal to the mid-infrared region by means of a nonlinear process, enabling to take full advantage of the availability of optical communications components for the generation of the multi-tone signals that are characteristic of molecular dispersion spectroscopic methods. In this way, it is possible to avoid several issues associated with optical instruments in which directly modulated mid-infrared quantum cascade lasers are employed. In this paper, we take full advantage of this benefit to implement the first heterodyne phase sensitive dispersion spectroscopy gas sensor based on a difference frequency generation source. The performance of the instrument is validated by detecting with high sensitivity methane in the 3.4 µm mid-infrared band.
Similar content being viewed by others
References
I.D. Lindsay, P. Groß, C.J. Lee, B. Adhimoolam, K.-J. Boller, Opt. Express 14, 12341 (2006)
J. Manne, A. Lim, W. Jäger, J. Tulip, Appl. Opt. 50, E112 (2011)
H. Moser, W. Pölz, J.P. Waclawek, J. Ofner, B. Lendl, Anal. Bioanal. Chem. 409, 729 (2016)
G.B. Rieker, J.B. Jeffries, R.K. Hanson, Appl. Opt. 48, 5546 (2009)
K. Sun, X. Chao, R. Sur, C.S. Goldenstein, J.B. Jeffries, R.K. Hanson, Meas. Sci. Technol. 24, 125203 (2013)
M. Wei, R. Kan, B. Chen, Z. Xu, C. Yang, X. Chen, H. Xia, M. Hu, Y. He, J. Liu, X. Fan, W. Wang, Appl. Phys. B 123, 149 (2017)
V. Spagnolo, P. Patimisco, S. Borri, G. Scamarcio, B.E. Bernacki, J. Kriesel, Opt. Lett. 37, 4461 (2012)
J. Peltola, T. Hieta, M. Vainio, Opt. Lett. 40, 2933 (2015)
G. Wysocki, D. Weidmann, Opt. Express 18, 26123 (2010)
A. Hangauer, G. Spinner, M. Nikodem, G. Wysocki, Appl. Phys. Lett. 103, 191107 (2013)
P. Martín-Mateos, P. Acedo, Opt. Express 22, 15143 (2014)
P. Martín-Mateos, J. Hayden, P. Acedo, B. Lendl, Anal. Chem. 89, 5916 (2017)
W. Ding, L. Sun, L. Yi, X. Ming, Appl. Opt. 55, 8698 (2016)
L. Zhang, G. Tian, J. Li, B. Yu, Appl. Spectrosc. 68, 1095 (2014)
J. Faist, F. Capasso, D.L. Sivco, C. Sirtori, A.L. Hutchinson, A.Y. Cho, Science 264, 553 (1994)
R.F. Curl, F. Capasso, C. Gmachl, A.A. Kosterev, B. McManus, R. Lewicki, M. Pusharsky, G. Wysocki, F.K. Tittel, Chem. Phys. Lett. 487, 1 (2010)
M.R. Alcaráz, A. Schwaighofer, C. Kristament, G. Ramer, M. Brandstetter, H. Goicoechea, B. Lendl, Anal. Chem. 87, 6980 (2015)
K.P. Petrov, S. Waltman, U. Simon, R.F. Curl, F.K. Tittel, E.J. Dlugokencky, L.W. Hollberg, Appl. Phys. B 61, 553–558 (1995)
H.Y. Clark, L. Corner, W. Denzer, G. Hancock, A. Hutchinson, M. Islam, R. Peverall, G.A.D. Ritchie, Chem. Phys. Lett. 399, 102 (2004)
E. Baumann, F.R. Giorgetta, W.C. Swann, A.M. Zolot, I. Coddington, N.R. Newbury, Phys. Rev. A 84, 62513 (2011)
P. Maddaloni, P. Malara, G. Gagliardi, P. De Natale, Appl. Phys. B 85, 219 (2006)
J.J. Scherer, J.B. Paul, H.J. Jost, M.L. Fischer, Appl. Phys. B 110, 271 (2013)
D. Richter, B.P. Wert, A. Fried, P. Weibring, J.G. Walega, J.W.C. White, B.H. Vaughn, F.K. Tittel, Opt. Lett. 34, 172 (2009)
D. Richter, A. Fried, B.P. Wert, J.G. Walega, F.K. Tittel, Appl. Phys. B. 75, 281 (2002)
A. Hangauer, G. Spinner, M. Nikodem, G. Wysocki, Opt. Express 22, 23439 (2014)
M. Nikodem, K. Krzempek, R. Karwat, G. Dudzik, K. Abramski, G. Wysocki, Opt. Lett. 39, 4420 (2014)
K. Krzempek, K.M. Abramski, M. Nikodem, Laser Phys. Lett. 14, 95702 (2017)
S. Paul, P. Martín-Mateos, N. Heermeier, F. Küppers, P. Acedo, ACS Photon. 4, 2664 (2017)
R. Szedlak, J. Hayden, P. Martín-Mateos, M. Holzbauer, A. Harrer, B. Schwarz, B. Hinkov, D. MacFarland, T. Zederbauer, H. Detz, A.M. Andrews, W. Schrenk, P. Acedo, B. Lendl, G. Strasser, Opt. Eng. 57, 11005 (2017)
P. Martín-Mateos, J. Hayden, P. Acedo, B. Lendl, In Proceedings of SPIE 10110, Photonic Instrumentation Engineering IV, 1011018, (2017)
K. Krzempek, G. Sobon, K.M. Abramski, Opt. Express 21, 20023 (2013)
Acknowledgements
The authors would like to thank the Spanish Ministry of Economy and Competitiveness for supporting the project under the Grant TEC-2014-52147-R (MOSSI). The work by Borja Jerez has been performed in the frame of a FPU Program, #FPU014/06338, granted by the Spanish Ministry of Education, Culture and Sports.
Author information
Authors and Affiliations
Corresponding author
Additional information
This article is part of the topical collection “Mid-infrared and THz Laser Sources and Applications” guest edited by Wei Ren, Paolo De Natale and Gerard Wysocki.
Rights and permissions
About this article
Cite this article
Martín-Mateos, P., Jerez, B., de Dios, C. et al. Mid-infrared heterodyne phase-sensitive dispersion spectroscopy using difference frequency generation. Appl. Phys. B 124, 66 (2018). https://doi.org/10.1007/s00340-018-6935-8
Received:
Accepted:
Published:
DOI: https://doi.org/10.1007/s00340-018-6935-8