Abstract
Atmospheric chemistry models simulate the physical and chemical transformation of airborne nitrogen (N) compounds and their sinks through wet and dry deposition. This chapter reviews modelling approaches for simulating atmospheric N deposition and their recent applications for estimating N deposition to China. Parameterizations of wet deposition include scavenging via both convective updrafts and large-scale precipitation. Dry deposition is often simulated as the product of number density and dry deposition velocity based on the resistance-in-series model using local land properties and meteorological conditions. Recent modelling studies have reported the annual total N deposition to China in the range of 7.9–20.1 Tg N year−1. Reduced N (NHx) accounts for 60–80% of the total, reflecting high NH3 emissions from agricultural activities in China. Dry deposition contributes 39–62% of total deposition depending on the specific model. More direct dry deposition measurements are needed to better evaluate model results. There are also considerable uncertainties in modelling N deposition resulting from the complexity of deposition mechanisms, the uncertainty of input parameters and the properties of N components. Future work to improve the deposition mechanisms and N emission estimates is needed to obtain better modelling of atmospheric N deposition to China.
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Acknowledgments
The authors gratefully acknowledge the financial support by the National Key Research and Development Program of China (2017YFC0210100).
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Zhang, L., Wang, X., Zhao, Y., Zhang, Q., Chang, M., Wang, Q. (2020). Modelling Atmospheric Nitrogen Deposition in China. In: Liu, X., Du, E. (eds) Atmospheric Reactive Nitrogen in China. Springer, Singapore. https://doi.org/10.1007/978-981-13-8514-8_4
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