Skip to main content

High-Energy Time-Resolved Electron Diffraction

  • Chapter
  • First Online:

Part of the book series: Springer Handbooks ((SHB))

Abstract

This chapter reviews the application of relativistic energy ultrashort electron beams to the direct investigation of structural changes in matter at atomic length scale with sub-picosecond (sub-ps) resolution by time-resolved electron diffraction ( ) . There are many benefits of using higher-energy electron beams for time-resolved electron scattering instrumentation, due mainly to the space charge force suppression at relativistic energies, which enables more intense and shorter electron bunches. Speed-of-light probes, higher penetration, and shorter de Broglie wavelength are other advantages associated with MeV electron energy.

The use of MeV beams for electron scattering demands excellent beam quality in both the transverse and longitudinal phase spaces, i. e., an exquisitely high six-dimensional ( ) brightness. Expertise from the low-energy microscopy and diffraction community has converged with advances made in relativistic electron sources for high-energy particle accelerators and fourth-generation synchrotron light sources in the effort to create and deliver electron beams with these characteristics.

This is a preview of subscription content, log in via an institution.

Buying options

Chapter
USD   29.95
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
eBook
USD   279.00
Price excludes VAT (USA)
  • Available as EPUB and PDF
  • Read on any device
  • Instant download
  • Own it forever
Hardcover Book
USD   359.00
Price excludes VAT (USA)
  • Durable hardcover edition
  • Dispatched in 3 to 5 business days
  • Free shipping worldwide - see info

Tax calculation will be finalised at checkout

Purchases are for personal use only

Learn about institutional subscriptions

References

  • J. Hemminger, G. Fleming, M. Ratner: Directing Matter and Energy: Five Challenges for Science and the Imagination, Report from the Basic Energy Sciences Advisory Committee (Dept. of Energy, Washington 2007)

    Google Scholar 

  • J. Hemminger, J. Sarrao, G. Crabtree, G. Fleming, M. Ratner: Challenges at the Frontiers of Matter and Energy: Transformative Opportunities for Discovery Science, Report from the Basic Energy Sciences Advisory Committee (Dept. of Energy, Washington 2015)

    Google Scholar 

  • E. Hall, S. Stemmer, H. Zheng, Y. Zhu, G. Maracas: Future of Electron Scattering and Diffraction (Dept. of Energy, Washington 2014)

    Google Scholar 

  • W.E. King, G.H. Campbell, A. Frank, B. Reed, J.F. Schmerge, B.J. Siwick, B.C. Stuart, P.M. Weber: Ultrafast electron microscopy in materials science, biology, and chemistry, J. Appl. Phys. 97(11), 111101 (2005)

    Google Scholar 

  • F. Carbone, P. Musumeci, O.J. Luiten, C. Hebert: A perspective on novel sources of ultrashort electron and x-ray pulses, Chem. Phys. 392(1), 1 (2012)

    CAS  Google Scholar 

  • F. Schotte, M. Lim, T.A. Jackson, A.V. Smirnov, J. Soman, J.S. Olson, G.N. Phillips, M. Wulff, P.A. Anfinrud: Watching a protein as it functions with 150-ps time-resolved x-ray crystallography, Science 300(5627), 1944 (2003)

    CAS  Google Scholar 

  • A.H. Zewail: Femtochemistry: Atomic-scale dynamics of the chemical bond, J. Phys. Chem. A 104(24), 5660 (2000)

    CAS  Google Scholar 

  • T. Brabec, F. Krausz: Intense few-cycle laser fields: Frontiers of nonlinear optics, Rev. Mod. Phys. 72(2), 545 (2000)

    CAS  Google Scholar 

  • T. Pfeifer, C. Spielmann, G. Gerber: Femtosecond x-ray science, Rep. Prog. Phys. 69(2), 443 (2006)

    Google Scholar 

  • D.H. Bilderback, P. Elleaume: Review of third and next generation synchrotron light sources, J. Phys. B 38(9), S773 (2005)

    CAS  Google Scholar 

  • C. Bostedt, J.D. Bozek, P.H. Bucksbaum, R.N. Coffee, J.B. Hastings, Z. Huang, R.W. Lee, S. Schorb, J.N. Corlett, P. Denes, P. Emma, R.W. Falcone, R.W. Schoenlein, G. Doumy, E.P. Kanter, B. Kraessig, S. Southworth, L. Young, L. Fang, M. Hoener, N. Berrah, C. Roedig, L.F. DiMauro: Ultra-fast and ultra-intense x-ray sciences: First results from the Linac Coherent Light Source free-electron laser, J. Phys. B 46(16), 164003 (2013)

    Google Scholar 

  • C. Bostedt, S. Boutet, D.M. Fritz, Z. Huang, H.J. Lee, H.T. Lemke, A. Robert, W.F. Schlotter, J.J. Turner, G.J. Williams: Linac Coherent Light Source: The first five years, Rev. Mod. Phys. 88(1), 015007 (2016)

    Google Scholar 

  • J. Spence: X-ray imaging: Ultrafast diffract-and-destroy movies, Nat. Photonics 2(7), 390 (2008)

    CAS  Google Scholar 

  • R. Henderson: Realizing the potential of electron cryo-microscopy, Q. Rev. Biophys. 37(1), 3 (2004)

    CAS  Google Scholar 

  • F. Vigliotti, S. Chen, C.-Y. Ruan, V.A. Lobastov, A.H. Zewail: Ultrafast electron crystallography of surface structural dynamics with atomic-scale resolution, Angew. Chem. 43, 2705–2709 (2004)

    CAS  Google Scholar 

  • G. Mourou, S. Williamson: Picosecond electron diffraction, Appl. Phys. Lett. 41(1), 44 (1982)

    CAS  Google Scholar 

  • A.A. Ischenko, S.A. Aseyev (Eds.): Time-Resolved Electron Diffraction, Advances in Imaging and Electron Physic, Vol. 184 (Elsevier, Amsterdam 2014)

    Google Scholar 

  • A.H. Zewail: 4-D ultrafast electron diffraction, crystallography, and microscopy, Annu. Rev. Phys. Chem. 57(1), 65 (2006)

    CAS  Google Scholar 

  • G. Sciaini, R.J.D. Miller: Femtosecond electron diffraction: Heralding the era of atomically resolved dynamics, Rep. Prog. Phys. 74(9), 096101 (2011)

    Google Scholar 

  • P. Gallant, P. Forget, F. Dorchies, Z. Jiang, J.C. Kieffer, P.A. Jaanimagi, J.C. Rebuffie, C. Goulmy, J.F. Pelletier, M. Sutton: Characterization of a subpicosecond x-ray streak camera for ultrashort laser-produced plasmas experiments, Rev. Sci. Instrum. 71(10), 3627 (2000)

    CAS  Google Scholar 

  • B.J. Siwick, J.R. Dwyer, R.E. Jordan, R.J.D. Miller: Ultrafast electron optics: Propagation dynamics of femtosecond electron packets, J. Appl. Phys. 92(3), 1643 (2002)

    CAS  Google Scholar 

  • B.W. Reed: Femtosecond electron pulse propagation for ultrafast electron diffraction, J. Appl. Phys. 100(3), 034916 (2006)

    Google Scholar 

  • J. Cao, Z. Hao, H. Park, C. Tao, D. Kau, L. Blaszczyk: Femtosecond electron diffraction for direct measurement of ultrafast atomic motions, Appl. Phys. Lett. 83(5), 1044 (2003)

    CAS  Google Scholar 

  • B.J. Siwick, J.R. Dwyer, R.E. Jordan, R.J.D. Miller: An atomic-level view of melting using femtosecond electron diffraction, Science 302(5649), 1382 (2003)

    CAS  Google Scholar 

  • L. Waldecker, R. Bertoni, R. Ernstorfer: Compact femtosecond electron diffractometer with 100 keV electron bunches approaching the single-electron pulse duration limit, J. Appl. Phys. 117(4), 044903 (2015)

    Google Scholar 

  • P. Baum: On the physics of ultrashort single-electron pulses for time-resolved microscopy and diffraction, Chem. Phys. 423, 55 (2013)

    CAS  Google Scholar 

  • R. Ernstorfer, M. Harb, C.T. Hebeisen, G. Sciaini, T. Dartigalongue, R.J.D. Miller: The formation of warm dense matter: Experimental evidence for electronic bond hardening in gold, Science 323(5917), 1033 (2009)

    CAS  Google Scholar 

  • R.C. Dudek, P.M. Weber: Ultrafast diffraction imaging of the electrocyclic ring-opening reaction of 1,3-cyclohexadiene, J. Phys. Chem. A 105(17), 4167 (2001)

    CAS  Google Scholar 

  • H. Ihee, V.A. Lobastov, U.M. Gomez, B.M. Goodson, R. Srinivasan, C.-Y. Ruan, A.H. Zewail: Direct imaging of transient molecular structures with ultrafast diffraction, Science 291(5503), 458 (2001)

    CAS  Google Scholar 

  • F. Carbone, P. Baum, P. Rudolf, A.H. Zewail: Structural preablation dynamics of graphite observed by ultrafast electron crystallography, Phys. Rev. Lett. 100(3), 139901 (2008)

    Google Scholar 

  • N. Gedik, D.S. Yang, G. Logvenov, I. Bozovic, A.H. Zewail: Nonequilibrium phase transitions in cuprates observed by ultrafast electron crystallography, Science 316(5823), 425 (2007)

    CAS  Google Scholar 

  • T. Ishikawa, S.A. Hayes, S. Keskin, G. Corthey, M. Hada, K. Pichugin, A. Marx, J. Hirscht, K. Shionuma, K. Onda, Y. Okimoto, S.Y. Koshihara, T. Yamamoto, H. Cui, M. Nomura, Y. Oshima, M. Abdel-Jawad, R. Kato, R.J.D. Miller: Direct observation of collective modes coupled to molecular orbital-driven charge transfer, Science 350(6267), 1501 (2015)

    CAS  Google Scholar 

  • M. Eichberger, H. Schäfer, M. Krumova, M. Beyer: Snapshots of cooperative atomic motions in the optical suppression of charge density waves, Nature 468(7325), 799 (2010)

    CAS  Google Scholar 

  • T. van Oudheusden, E.F. De Jong, S.B. van der Geer, W.P.E.M. Op 't Root, O.J. Luiten, B.J. Siwick: Electron source concept for single-shot sub-100 fs electron diffraction in the 100 keV range, J. Appl. Phys. 102(9), 093501 (2007)

    Google Scholar 

  • X.J. Wang, X. Qiu, I. Ben-Zvi: Experimental observation of high-brightness microbunching in a photocathode RF electron gun, Phys. Rev. E 54, R3121 (1996)

    CAS  Google Scholar 

  • T. van Oudheusden, P.L.E.M. Pasmans, S.B. van der Geer, M.J. de Loos, M.J. van der Wiel, O.J. Luiten: Compression of subrelativistic space-charge-dominated electron bunches for single-shot femtosecond electron diffraction, Phys. Rev. Lett. 105(26), 264801 (2010)

    Google Scholar 

  • R.P. Chatelain, V.R. Morrison, C. Godbout, B.J. Siwick: Ultrafast electron diffraction with radio-frequency compressed electron pulses, Appl. Phys. Lett. 101(8), 081901 (2012)

    Google Scholar 

  • D. Alesini, A. Battisti, M. Ferrario, L. Foggetta, V. Lollo, L. Ficcadenti, V. Pettinacci, S. Custodio, E. Pirez, P. Musumeci: New technology based on clamping for high gradient radio frequency photogun, Phys. Rev. ST Accel. Beams 18(9), 092001 (2015)

    Google Scholar 

  • X.J. Wang, Z. Wu, H. Ihee: Potential of femtosecond relativistic electron diffraction. In: Proc. 2003 Part. Accel. Conf. (2003) p. 420

    Google Scholar 

  • X.J. Wang, D. Xiang, T.K. Kim, H.H. Ihee: Potential of femtosecond electron diffraction using near-relativistic electrons from a photocathode RF electron gun, J. Korean Phys. Soc. 48(3), 390–396 (2006)

    Google Scholar 

  • R. Akre, D. Dowell, P. Emma, J. Frisch, S. Gilevich: Commissioning the Linac Coherent Light Source injector, Phys. Rev. ST Accel. Beams 11(3), 030703 (2008)

    Google Scholar 

  • J.B. Hastings, F.M. Rudakov, D.H. Dowell, J.F. Schmerge, J.D. Cardoza, J.M. Castro, S.M. Gierman, H. Loos, P.M. Weber: Ultrafast time-resolved electron diffraction with megavolt electron beams, Appl. Phys. Lett. 89(18), 184109 (2006)

    Google Scholar 

  • P. Musumeci, J.T. Moody, C.M. Scoby: Relativistic electron diffraction at the UCLA Pegasus photoinjector laboratory, Ultramicroscopy 108(11), 1450 (2008)

    CAS  Google Scholar 

  • R. Li, C. Tang, Y. Du, W. Huang, Q. Du, J. Shi, L. Yan, X. Wang: Experimental demonstration of high quality MeV ultrafast electron diffraction, Rev. Sci. Instrum. 80(8), 083303 (2009)

    Google Scholar 

  • P. Musumeci, J.T. Moody, C.M. Scoby, M.S. Gutierrez, M. Westfall: Laser-induced melting of a single crystal gold sample by time-resolved ultrafast relativistic electron diffraction, Appl. Phys. Lett. 97(6), 063502 (2010)

    Google Scholar 

  • C.T. Hebeisen, G. Sciaini, M. Harb, R. Ernstorfer, T. Dartigalongue, S.G. Kruglik, R.J.D. Miller: Grating enhanced ponderomotive scattering for visualization and full characterization of femtosecond electron pulses, Opt. Express 16(5), 3334 (2008)

    Google Scholar 

  • Y. Murooka, N. Naruse, S. Sakakihara, M. Ishimaru, J. Yang, K. Tanimura: Transmission-electron diffraction by MeV electron pulses, Appl. Phys. Lett. 98(25), 251903 (2011)

    Google Scholar 

  • P. Zhu, Y. Zhu, Y. Hidaka, L. Wu, J. Cao: Femtosecond time-resolved MeV electron diffraction, New J. Phys. 17(6), 063004 (2015)

    Google Scholar 

  • S. Manz, A. Casandruc, D. Zhang, Y. Zhong: Mapping atomic motions with ultrabright electrons: Towards fundamental limits in space-time resolution, Faraday Discuss. 177, 467 (2015)

    CAS  Google Scholar 

  • S.P. Weathersby, G. Brown, M. Centurion, T.F. Chase, R. Coffee, J. Corbett, J.P. Eichner, J.C. Frisch, A.R. Fry, M. Gühr, N. Hartmann, C. Hast, R. Hettel, R.K. Jobe, E.N. Jongewaard, J.R. Lewandowski, R.K. Li, A.M. Lindenberg, I. Makasyuk, J.E. May, D. McCormick, M.N. Nguyen, A.H. Reid, X. Shen, K. Sokolowski-Tinten, T. Vecchione, S.L. Vetter, J. Wu, J. Yang, H.A. Dürr, X.J. Wang: Mega-electron-volt ultrafast electron diffraction at SLAC National Accelerator Laboratory, Rev. Sci. Instrum. 86(7), 073702 (2015)

    CAS  Google Scholar 

  • L.W. Feng, L. Lin, S.L. Huang, S.W. Quan, T. Jiang, P.F. Zhu, J.K. Hao, F. Zhu, F. Wang, F. Fu, R. Wang, L. Zhao, D. Xiang, K.X. Liu: Ultrafast electron diffraction with megahertz MeV electron pulses from a superconducting radio-frequency photoinjector, Appl. Phys. Lett. 107(22), 224101 (2015)

    Google Scholar 

  • D. Filippetto, H. Qian: Design of a high-flux instrument for ultrafast electron diffraction and microscopy, J. Phys. B 49(10), 104003 (2016)

    Google Scholar 

  • D. Xiang, F. Fu, J. Zhang, X. Huang, L. Wang, X. Wang, W. Wan: Accelerator-based single-shot ultrafast transmission electron microscope with picosecond temporal resolution and nanometer spatial resolution, Nucl. Instrum. Methods Phys. Res. A 759, 74 (2014)

    CAS  Google Scholar 

  • B. Hou, V. Malka, K. Krushelnick, J. Faure: Electron diffraction using ultrafast electron bunches from a laser-wakefield accelerator at kHz repetition rate, Appl. Phys. Lett. 102(6), 064104 (2013)

    Google Scholar 

  • F. Salvat, J.D. Martnez, R. Mayol, J. Parellada: Analytical Dirac-Hartree-Fock-Slater screening function for atoms (\(Z=1-92\)), Phys. Rev. A 36(2), 467 (1987)

    CAS  Google Scholar 

  • F. Salvat, R. Mayol: Elastic scattering of electrons and positrons by atoms. Schrödinger and Dirac partial wave analysis, Comput. Phys. Commun. 74(3), 358 (1993)

    CAS  Google Scholar 

  • H. Shinotsuka, S. Tanuma, C.J. Powell, D.R. Penn: Calculations of electron inelastic mean free paths. X. Data for 41 elemental solids over the 50 eV to 200 keV range with the relativistic full Penn algorithm, Surf. Interface Anal. 47(9), 871 (2015)

    CAS  Google Scholar 

  • L. Reimer: Transmission Electron Microscopy: Physics of Image Formation and Microanalysis, Springer Series in Optical Sciences, Vol. 36 (Springer, New York 2013)

    Google Scholar 

  • J.C.H. Spence: Outrunning damage: Electrons vs. x-rays-timescales and mechanisms, Struct. Dyn. 4(4), 044027 (2017)

    Google Scholar 

  • P. Grivet, P.W. Hawkes, A. Septier: Electron Optics, 2nd edn. (Pergamon, New York 1972)

    Google Scholar 

  • C.A. Brau: What brightness means. In: The Physics and Applications of High Brightness Electron Beams, ed. by J. Rosenzweig, G. Travish, L. Serafini (World Scientific, Singapore 2003) p. 20

    Google Scholar 

  • G.H. Jansen: Coulomb interactions in particle beams, J. Vac. Sci. Technol. B 6(6), 1977 (1988)

    CAS  Google Scholar 

  • J.T. Moody, P. Musumeci, M.S. Gutierrez, J.B. Rosenzweig, C.M. Scoby: Longitudinal phase space characterization of the blow-out regime of RF photoinjector operation, Phys. Rev. ST Accel. Beams 12(7), 070704 (2009)

    Google Scholar 

  • I.V. Bazarov, B.M. Dunham, C.K. Sinclair: Maximum achievable beam brightness from photoinjectors, Phys. Rev. Lett. 102(10), 104801 (2009)

    Google Scholar 

  • D. Filippetto, P. Musumeci, M. Zolotorev, G. Stupakov: Maximum current density and beam brightness achievable by laser-driven electron sources, Phys. Rev. ST Accel. Beams 17(2), 024201 (2014)

    Google Scholar 

  • I.V. Bazarov, C.K. Sinclair: Multivariate optimization of a high brightness DC gun photoinjector, Phys. Rev. ST Accel. Beams 8(3), 034202 (2005)

    Google Scholar 

  • P. Musumeci, J.T. Moody, R.J. England, J.B. Rosenzweig, T. Tran: Experimental generation and characterization of uniformly filled ellipsoidal electron-beam distributions, Phys. Rev. Lett. 100(24), 244801 (2008)

    CAS  Google Scholar 

  • J.B. Rosenzweig, A. Cahill, V. Dolgashev, C. Emma, A. Fukusawa, R. Li, C. Limborg, J. Maxson, P. Musumeci, A. Nause, R. Pakter, R. Pompili, R. Roussel, B. Spataro, S. Tantawi: Next generation high brightness electron beams from ultra-high field cryogenic radiofrequency photocathode sources, arXiv:1603.01657 [physics.acc-ph] (2016)

    Google Scholar 

  • Y. Ding, A. Brachmann, F.J. Decker, D. Dowell, P. Emma, J. Frisch, S. Gilevich, G. Hays, P. Hering, Z. Huang, R. Iverson, H. Loos, A. Miahnahri, H.D. Nuhn, D. Ratner, J. Turner, J. Welch, W. White, J. Wu: Measurements and simulations of ultralow emittance and ultrashort electron beams in the Linac Coherent Light Source, Phys. Rev. Lett. 102(25), 254801 (2009)

    CAS  Google Scholar 

  • A. Arnold, M. Freitag, P. Murcek, J. Teichert, H. Vennekate, R. Xiang, P. Kniesel, P. Lu, M. Stirbet, G. Ciovati, L. Turhington: RF performance results of the 2nd ELBE SRF gun. In: Proc. SRF2015 (2015) p. THPB055

    Google Scholar 

  • D.T. Palmer: The Next Generation Photoinjector, Ph.D. Thesis (Stanford University, Stanford 1998)

    Google Scholar 

  • T. Schietinger, M. Pedrozzi, M. Aiba, V. Arsov, S. Bettoni, B. Beutner, M. Calvi, P. Craievich, M. Dehler, F. Frei: Commissioning experience and beam physics measurements at the SwissFEL injector test facility, Phys. Rev. Accel. Beams 19(10), 100702 (2016)

    Google Scholar 

  • P. Musumeci, L. Faillace, A. Fukasawa: Novel radio-frequency gun structures for ultrafast relativistic electron diffraction, Microsc. Microanal. 15(4), 290 (2009)

    CAS  Google Scholar 

  • A. Fukasawa, H. To, S.K. Mahapatra, B. Baumgartner, A. Cahill, K. Fitzmorris, R. Li, P. Musumeci, J.B. Rosenzweig, B. Spataro, D. Alesini, L. Ficcadenti, A. Valloni, L. Palumbo: Progress on the hybrid gun project at UCLA, Phys. Procedia 52, 2 (2014)

    Google Scholar 

  • E. Pirez, P. Musumeci, J. Maxson, D. Alesini: S-band 1.4 cell photoinjector design for high brightness beam generation, Nucl. Instrum. Methods Phys. Res. A 865, 109 (2016)

    Google Scholar 

  • F. Sannibale, D. Filippetto, C.F. Papadopoulos, J. Staples, R. Wells, B. Bailey, K. Baptiste, J. Corlett, C. Cork, S. De Santis: Advanced photoinjector experiment photogun commissioning results, Phys. Rev. ST Accel. Beams 15(10), 103501 (2012)

    Google Scholar 

  • A. Arnold, J. Teichert: Overview on superconducting photoinjectors, Phys. Rev. ST Accel. Beams 14(2), 024801 (2011)

    Google Scholar 

  • E. Esarey, C.B. Schroeder, W.P. Leemans: Physics of laser-driven plasma-based electron accelerators, Rev. Mod. Phys. 81(3), 1229 (2009)

    CAS  Google Scholar 

  • O. Lundh, J. Lim, C. Rechatin, L. Ammoura, A. Ben-Ismail, X. Davoine, G. Gallot, J.-P. Goddet, E. Lefebvre, V. Malka: Few femtosecond, few kiloampere electron bunch produced by a laser-plasma accelerator, Nat. Phys. 7(3), 219 (2011)

    CAS  Google Scholar 

  • J. Faure, B. van der Geer, B. Beaurepaire, G. Gallé, A. Vernier, A. Lifschitz: Concept of a laser-plasma-based electron source for sub-10-fs electron diffraction, Phys. Rev. Accel. Beams 19(2), 021302 (2016)

    Google Scholar 

  • Z.-H. He, A.G.R. Thomas, B. Beaurepaire, J.A. Nees, B. Hou, V. Malka, K. Krushelnick, J. Faure: Electron diffraction using ultrafast electron bunches from a laser-wakefield accelerator at kHz repetition rate, Appl. Phys. Lett. 102(6), 064104 (2013)

    Google Scholar 

  • D.H. Dowell, I. Bazarov, B. Dunham, K. Harkay, C. Hernandez-Garcia, R. Legg, H. Padmore, T. Rao, J. Smedley, W. Wan: Cathode R&D for future light sources, Nucl. Instrum. Methods Phys. Res. A 622(3), 685 (2010)

    CAS  Google Scholar 

  • J. Maxson, H. Lee, A.C. Bartnik, J. Kiefer, I. Bazarov: Adaptive electron beam shaping using a photoemission gun and spatial light modulator, Phys. Rev. ST Accel. Beams 18(2), 023401 (2015)

    Google Scholar 

  • D.H. Dowell, J.F. Schmerge: Quantum efficiency and thermal emittance of metal photocathodes, Phys. Rev. ST Accel. Beams 12(7), 074201 (2009)

    Google Scholar 

  • M.C. Divall, E. Prat, S. Bettoni, C. Vicario, A. Trisorio, T. Schietinger, C.P. Hauri: Intrinsic emittance reduction of copper cathodes by laser wavelength tuning in an RF photoinjector, Phys. Rev. ST Accel. Beams 18(3), 033401 (2015)

    Google Scholar 

  • J.M. Maxson, I.V. Bazarov, W. Wan, H.A. Padmore, C.E. Coleman-Smith: Fundamental photoemission brightness limit from disorder induced heating, New J. Phys. 15(10), 103024 (2013)

    Google Scholar 

  • S. Karkare, I. Bazarov: Effects of surface nonuniformities on the mean transverse energy from photocathodes, Phys. Rev. Appl. 4(2), 024015 (2015)

    Google Scholar 

  • L. Cultrera, S. Karkare, H. Lee, X. Liu, I. Bazarov, B. Dunham: Cold electron beams from cryocooled, alkali antimonide photocathodes, Phys. Rev. ST Accel. Beams 18(11), 113401 (2015)

    Google Scholar 

  • D.T. Pierce, F. Meier, P. Zürcher: Negative electron affinity GaAs: A new source of spin-polarized electrons, Appl. Phys. Lett. 26(12), 670 (1975)

    CAS  Google Scholar 

  • J. Maxson, D. Cesar, G. Calmasini, A. Ody, P. Musumeci, D. Alesini: Direct measurement of sub-10 fs relativistic electron beams with ultralow emittance, Phys. Rev. Lett. 118(15), 154802 (2016)

    Google Scholar 

  • M.J. de Loos, S.B. van der Geer, Y.M. Saveliev, V.M. Pavlov, A.J.W. Reitsma, S.M. Wiggins, J. Rodier, T. Garvey, D.A. Jaroszynski: Radial bunch compression: Path-length compensation in an RF photoinjector with a curved cathode, Phys. Rev. ST Accel. Beams 9(8), 084201 (2006)

    Google Scholar 

  • K. Floettmann, V.V. Paramonov: Beam dynamics in transverse deflecting RF structures, Phys. Rev. ST Accel. Beams 17(2), 024001 (2014)

    Google Scholar 

  • P. Musumeci, H.A. Bender, N.S. Wilcox: Imaging single electrons to enable the generation of ultrashort beams for single-shot femtosecond relativistic electron diffraction, J. Appl. Phys. 110(7), 074512 (2011)

    Google Scholar 

  • Y. Glinec, J. Faure, A. Guemnie-Tafo, V. Malka, H. Monard, J.P. Larbre, V. De Waele, J.L. Marignier, M. Mostafavi: Absolute calibration for a broad range single shot electron spectrometer, Rev. Sci. Instrum. 77(10), 103301 (2006)

    Google Scholar 

  • A. Buck, K. Zeil, A. Popp, K. Schmid, A. Jochmann, S.D. Kraft, B. Hidding, T. Kudyakov, C.M.S. Sears, L. Veisz, S. Karsch, J. Pawelke, R. Sauerbrey, T. Cowan, F. Krausz, U. Schramm: Absolute charge calibration of scintillating screens for relativistic electron detection, Rev. Sci. Instrum. 81(3), 033301 (2010)

    CAS  Google Scholar 

  • R.K. Li, P. Musumeci, H.A. Bender, N.S. Wilcox, M. Wu: Imaging single electrons to enable the generation of ultrashort beams for single-shot femtosecond relativistic electron diffraction, J. Appl. Phys. 110(7), 074512 (2011)

    Google Scholar 

  • R. Ischebeck, E. Prat, V. Thominet, C.O. Loch: Transverse profile imager for ultrabright electron beams, Phys. Rev. ST Accel. Beams 18(8), 082802 (2015)

    Google Scholar 

  • M.W. Tate, P. Purohit, D. Chamberlain, K.X. Nguyen, R.M. Hovden, C.S. Chang, P. Deb, E. Turgut, J.T. Heron, D.G. Schlom, D.C. Ralph, G.D. Fuchs, K.S. Shanks, H.T. Philipp, D.A. Muller, S.M. Gruner: High dynamic range pixel array detector for scanning transmission electron microscopy, Microsc. Microanal. 22, 237 (2016)

    CAS  Google Scholar 

  • E. Nogales: The development of cryo-EM into a mainstream structural biology technique, Nat. Methods 13(1), 24 (2015)

    Google Scholar 

  • M. Battaglia, D. Contarato, P. Denes, P. Giubilato: Cluster imaging with a direct detection CMOS pixel sensor in transmission electron microscopy, Nucl. Instrum. Methods Phys. Res. A 608(2), 363 (2009)

    CAS  Google Scholar 

  • A. Gliserin, M. Walbran, F. Krausz, P. Baum: Sub-phonon-period compression of electron pulses for atomic diffraction, Nat. Commun. 6, 8723 (2015)

    CAS  Google Scholar 

  • R.P. Chatelain, V.R. Morrison, B.L.M. Klarenaar, B.J. Siwick: Coherent and incoherent electron–phonon coupling in graphite observed with radio-frequency compressed ultrafast electron diffraction, Phys. Rev. Lett. 113(23), 235502 (2014)

    Google Scholar 

  • K. Ishioka, M. Hase, M. Kitajima, L. Wirtz, A. Rubio, H. Petek: Ultrafast electron–phonon decoupling in graphite, Phys. Rev. B 77(12), 121402 (2008)

    Google Scholar 

  • S.G. Anderson, P. Musumeci, J.B. Rosenzweig, W.J. Brown, R.J. England, M. Ferrario, J.S. Jacob, M.C. Thompson, G. Travish, A.M. Tremaine: Velocity bunching of high-brightness electron beams, Phys. Rev. ST Accel. Beams 8(1), 014401 (2005)

    Google Scholar 

  • M. Ferrario, D. Alesini, A. Bacci, M. Bellaveglia, R. Boni, M. Boscolo, M. Castellano, E. Chiadroni, A. Cianchi, L. Cultrera: Experimental demonstration of emittance compensation with velocity bunching, Phys. Rev. Lett. 104(5), 054801 (2010)

    CAS  Google Scholar 

  • X.H. Lu, C.X. Tang, R.K. Li, H. To, G. Andonian, P. Musumeci: Generation and measurement of velocity bunched ultrashort bunch of pC charge, Phys. Rev. ST Accel. Beams 18(3), 032802 (2015)

    Google Scholar 

  • I. Dornmair, C.B. Schroeder, K. Floettmann: Plasma-driven ultrashort bunch diagnostics, Phys. Rev. ST Accel. Beams 19(6), 062801 (2016)

    Google Scholar 

  • R.K. Li, P. Musumeci: Single-shot MeV transmission electron microscopy with picosecond temporal resolution, Phys. Rev. Appl. 2(2), 024003 (2014)

    Google Scholar 

  • B. Zeitler, K. Floettmann, F. Grüner: Linearization of the longitudinal phase space without higher harmonic field, Phys. Rev. ST Accel. Beams 18(12), 120102 (2015)

    Google Scholar 

  • M.J. de Loos, S.B. van der Geer: General particle tracer, http://www.pulsar.nl/gpt (1996)

  • M. Eichberger, N. Erasmus, K. Haupt, G. Kassier, A. von Flotow, J. Demsar, H. Schwoerer: Femtosecond streaking of electron diffraction patterns to study structural dynamics in crystalline matter, Appl. Phys. Lett. 102(12), 121106 (2013)

    Google Scholar 

  • E. Curry, S. Fabbri, P. Musumeci, A. Gover: THz-driven zero-slippage IFEL scheme for phase space manipulation, New J. Phys. 18(11), 113045 (2016)

    Google Scholar 

  • P. Baum, A. Zewail: Femtosecond diffraction with chirped electron pulses, Chem. Phys. Lett. 462(1–3), 14 (2008)

    CAS  Google Scholar 

  • P. Musumeci, J.T. Moody, C.M. Scoby, M.S. Gutierrez, T. Tran: RF streak camera based ultrafast relativistic electron diffraction, Rev. Sci. Instrum. 80(1), 013302 (2009)

    CAS  Google Scholar 

  • Z.H. He, B. Beaurepaire, J.A. Nees, G. Gall, S.A. Scott, J.R.S. Perez, M.G. Lagally, K. Krushelnick, A.G.R. Thomas, J. Faure: Capturing structural dynamics in crystalline silicon using chirped electrons from a laser wakefield accelerator, Sci. Rep. 6, 36224 (2016)

    CAS  Google Scholar 

  • R. Li, W. Huang, Y. Du, L. Yan, Q. Du, J. Shi, J. Hua, H. Chen, T. Du, H. Xu, C. Tang: Note: Single-shot continuously time-resolved MeV ultrafast electron diffraction, Rev. Sci. Instrum. 81(3), 036110 (2010)

    Google Scholar 

  • N. Hartmann, W. Helml, A. Galler, M.R. Bionta, J. Grünert, S.L. Molodtsov, K.R. Ferguson, S. Schorb, M.L. Swiggers, S. Carron: Sub-femtosecond precision measurement of relative x-ray arrival time for free-electron lasers, Nat. Photonics 8, 706709 (2014)

    Google Scholar 

  • F. Tavella, N. Stojanovic, G. Geloni, M. Gensch: Few-femtosecond timing at fourth-generation x-ray light sources, Nat. Photonics 5(3), 162 (2011)

    CAS  Google Scholar 

  • E. Allaria, G. De Ninno, S. Di Mitri, W.M. Fawley, E. Ferrari, L. Fröhlich, G. Penco, P. Sigalotti, S. Spampinati, C. Spezzani: Energy slicing analysis for time-resolved measurement of electron-beam properties, Phys. Rev. ST Accel. Beams 17(1), 010704 (2014)

    Google Scholar 

  • J.T. Moody, P. Musumeci, G. Anderson, S. Anderson, S. Betts, S. Fisher, D. Gibson, A. Tremaine, S. Wu: The LLNL/UCLA high gradient inverse free electron laser accelerator, Energy 70, 140 (2012)

    Google Scholar 

  • C.M. Scoby, P. Musumeci, J.T. Moody, M.S. Gutierrez: Electro-optic sampling at 90 degree interaction geometry for time-of-arrival stamping of ultrafast relativistic electron diffraction, Phys. Rev. ST Accel. Beams 13(2), 022801 (2010)

    Google Scholar 

  • A. Angelovski, M. Kuntzsch, M.K. Czwalinna, A. Penirschke, M. Hansli, C. Sydlo, V. Arsov, S. Hunziker, H. Schlarb, M. Gensch: Evaluation of the cone-shaped pickup performance for low charge sub-10 fs arrival-time measurements at free electron laser facilities, Phys. Rev. ST Accel. Beams 18(1), 012801 (2015)

    Google Scholar 

  • M. Harmand, R. Coffee, M.R. Bionta, M. Chollet, D. French, D. Zhu, D.M. Fritz, H.T. Lemke, N. Medvedev, B. Ziaja, S. Toleikis, M. Cammarata: Achieving few-femtosecond time-sorting at hard x-ray free-electron lasers, Nat. Photonics 7(3), 215 (2013)

    CAS  Google Scholar 

  • A.L. Cavalieri, D.M. Fritz, S.H. Lee, P.H. Bucksbaum, D.A. Reis, J. Rudati, D.M. Mills, P.H. Fuoss, G.B. Stephenson, C.C. Kao, D.P. Siddons, D.P. Lowney, A.G. MacPhee, D. Weinstein, R.W. Falcone, R. Pahl, J. Als-Nielsen, C. Blome, S. Düsterer, R. Ischebeck, H. Schlarb, H. Schulte-Schrepping, T. Tschentscher, J. Schneider, O. Hignette, F. Sette, K. Sokolowski-Tinten, H.N. Chapman, R.W. Lee, T.N. Hansen, O. Synnergren, J. Larsson, S. Techert, J. Sheppard, J.S. Wark, M. Bergh, C. Caleman, G. Huldt, D. van der Spoel, N. Timneanu, J. Hajdu, R.A. Akre, E. Bong, P. Emma, P. Krejcik, J. Arthur, S. Brennan, K.J. Gaffney, A.M. Lindenberg, K. Luening, J.B. Hastings: Clocking femtosecond x-rays, Phys. Rev. Lett. 94(11), 114801 (2005)

    CAS  Google Scholar 

  • M. Gao, H. Jean-Ruel, R.R. Cooney, J. Stampe, M. de Jong, M. Harb, G. Sciaini, G. Moriena, R.J.D. Miller: Full characterization of RF compressed femtosecond electron pulses using ponderomotive scattering, Opt. Express 20(11), 12048 (2012)

    CAS  Google Scholar 

  • G.H. Kassier, K. Haupt, N. Erasmus, E.G. Rohwer, H.M. von Bergmann, H. Schwoerer, S.M.M. Coelho, F.D. Auret: A compact streak camera for 150 fs time resolved measurement of bright pulses in ultrafast electron diffraction, Rev. Sci. Instrum. 81(10), 105103 (2010)

    CAS  Google Scholar 

  • D.B. Cesar, P. Musumeci, D. Alesini: Ultrafast gating of a mid-infrared laser pulse by a sub-pC relativistic electron beam, J. Appl. Phys. 118(23), 234506 (2015)

    Google Scholar 

  • R. Ulbricht, E. Hendry, J. Shan, T.F. Heinz, M. Bonn: Carrier dynamics in semiconductors studied with time-resolved terahertz spectroscopy, Rev. Mod. Phys. 83(2), 543 (2011)

    CAS  Google Scholar 

  • A. Cavalleri, S. Wall, C. Simpson, E. Statz, D.W. Ward, K.A. Nelson, M. Rini, R.W. Schoenlein: Tracking the motion of charges in a terahertz light field by femtosecond x-ray diffraction, Nature 442(7103), 664 (2006)

    CAS  Google Scholar 

  • M. Reiser: Theory and Design of Charged Particle Beams (Wiley-VCH, Weinheim 2008)

    Google Scholar 

  • C. Gulliford, A. Bartnik, I. Bazarov: Multiobjective optimizations of a novel cryocooled DC gun based ultrafast electron diffraction beam line, Phys. Rev. Accel. Beams 19(9), 093402 (2016)

    Google Scholar 

  • S. Karkare, D. Dimitrov, W. Schaff, L. Cultrera, A. Bartnik, X. Liu, E. Sawyer, T. Esposito, I. Bazarov: Monte Carlo charge transport and photoemission from negative electron affinity GaAs photocathodes, J. Appl. Phys. 113(10), 104904 (2013)

    Google Scholar 

  • H. Dürr, X. Wang: Ultrafast Science Opportunities with Electron Microscopy, Report SLAC-R-1039 (SLAC National Accelerator Laboratory, Stanford 2016)

    Google Scholar 

  • S.D. Brorson, J.G. Fujimoto, E.P. Ippen: Femtosecond electronic heat-transport dynamics in thin gold films, Phys. Rev. Lett. 59(17), 1962 (1987)

    CAS  Google Scholar 

  • S.I. Anisimov, B.L. Kapeliovich, T.L. Perelman: Electron emission from metal surfaces exposed to ultrashort laser pulses, Zh. Eksp. Teor. Fiz. 66(776), 375 (1974)

    Google Scholar 

  • P.B. Allen: Theory of thermal relaxation of electrons in metals, Phys. Rev. Lett. 59(13), 1460 (1987)

    CAS  Google Scholar 

  • Y. Giret, N. Naruse, S.L. Daraszewicz, Y. Murooka, J. Yang, D.M. Duffy, A.L. Shluger, K. Tanimura: Determination of transient atomic structure of laser-excited materials from time-resolved diffraction data, Appl. Phys. Lett. 103(25), 253107 (2013)

    Google Scholar 

  • S.L. Daraszewicz, Y. Giret, N. Naruse, Y. Murooka, J. Yang, D.M. Duffy, A.L. Shluger, K. Tanimura: Structural dynamics of laser-irradiated gold nanofilms, Phys. Rev. B 88(18), 184101 (2013)

    Google Scholar 

  • M.Z. Mo, X. Shen, Z. Chen, R.K. Li, M. Dunning, K. Sokolowski-Tinten, Q. Zheng, S.P. Weathersby, A.H. Reid, R. Coffee, I. Makasyuk, S. Edstrom, D. McCormick, K. Jobe, C. Hast, S.H. Glenzer, X. Wang: Single-shot mega-electronvolt ultrafast electron diffraction for structure dynamic studies of warm dense matter, Rev. Sci. Instrum. 87(11), 11D810 (2016)

    CAS  Google Scholar 

  • T. Chase, M. Trigo, A.H. Reid, R. Li, T. Vecchione, X. Shen, S. Weathersby, R. Coffee, N. Hartmann, D.A. Reis, X.J. Wang, H.A. Dürr: Ultrafast electron diffraction from non-equilibrium phonons in femtosecond laser heated Au films, Appl. Phys. Lett. 108(4), 041909 (2016)

    Google Scholar 

  • E.M. Mannebach, R. Li, K.-A. Duerloo, C. Nyby, P. Zalden, T. Vecchione, F. Ernst, A.H. Reid, T. Chase, X. Shen, S. Weathersby, C. Hast, R. Hettel, R. Coffee, N. Hartmann, A.R. Fry, Y. Yu, L. Cao, T.F. Heinz, E.J. Reed, H.A. Dürr, X. Wang, A.M. Lindenberg: Dynamic structural response and deformations of monolayer MoS2 visualized by femtosecond electron diffraction, Nano Lett. 15(10), 6889 (2015)

    Google Scholar 

  • P.-F. Zhu, F.-C. Fu, L. Sheng-Guang, D. Xiang, J. Zhang, J.-M. Cao: Time-resolved visualization of laser-induced heating of gold with MeV ultrafast electron diffraction, Chin. Phys. Lett. 31(11), 116101 (2014)

    Google Scholar 

  • S. Manz, A. Casandruc, D. Zhang, Y. Zhong, R.A. Loch, A. Marx, T. Hasegawa, L.C. Liu, S. Bayesteh, H. Delsim-Hashemi, M. Hoffmann, M. Felber, M. Hachmann, F. Mayet, J. Hirscht, S. Keskin, M. Hada, S.W. Epp, K. Flottmann, R.J.D. Miller: Mapping atomic motions with ultrabright electrons: Towards fundamental limits in space-time resolution, Faraday Discuss. 177, 467 (2015)

    CAS  Google Scholar 

  • P. Zhu, Y. Zhu, Y. Hidaka, L. Wu, J. Cao, H. Berger, J. Geck, R. Kraus, S. Pjerov, Y. Shen, R.I. Tobey, J.P. Hill, X.J. Wang: Femtosecond time-resolved MeV electron diffraction, New J. Phys. 17(6), 063004 (2015)

    Google Scholar 

  • I. Hargittai: Gas-phase electron diffraction for molecular structure determination. In: Electron Crystallography: Novel Approaches for Structure Determination of Nanosized Materials, ed. by T.E. Weirich, J.L. Lábár, X. Zou (Springer, Dordrecht 2006) p. 197

    Google Scholar 

  • J.C. Williamson, A.H. Zewail: Structural femtochemistry: Experimental methodology, Proc. Natl. Acad. Sci. U.S.A. 88(11), 5021 (1991)

    CAS  Google Scholar 

  • J.C. Williamson, A.H. Zewail: Ultrafast electron diffraction. Velocity mismatch and temporal resolution in crossed-beam experiments, Chem. Phys. Lett. 209(1), 10 (1993)

    CAS  Google Scholar 

  • J.C. Williamson, J. Cao, H. Ihee, H. Frey, A.H. Zewail: Clocking transient chemical changes by ultrafast electron diffraction, Nature 386(6621), 159 (1997)

    CAS  Google Scholar 

  • J. Cao, H. Ihee, A.H. Zewail: Ultrafast electron diffraction and direct observation of transient structures in a chemical reaction, Proc. Natl. Acad. Sci. U.S.A. 96(2), 338 (1999)

    CAS  Google Scholar 

  • J. Yang, M. Guehr, T. Vecchione, M.S. Robinson, R. Li, N. Hartmann, X. Shen, R. Coffee, J. Corbett, A. Fry, K. Gaffney, T. Gorkhover, C. Hast, K. Jobe, I. Makasyuk, A. Reid, J. Robinson, S. Vetter, F. Wang, S. Weathersby, C. Yoneda, M. Centurion, X. Wang: Diffractive imaging of a rotational wavepacket in nitrogen molecules with femtosecond megaelectronvolt electron pulses, Nat. Commun. 7, 11232 (2016)

    CAS  Google Scholar 

  • J. Yang, M. Guehr, X. Shen, R. Li, T. Vecchione, R. Coffee, J. Corbett, A. Fry, N. Hartmann, C. Hast, K. Hegazy, K. Jobe, I. Makasyuk, J. Robinson, M.S. Robinson, S. Vetter, S. Weathersby, C. Yoneda, X. Wang, M. Centurion: Diffractive imaging of coherent nuclear motion in isolated molecules, Phys. Rev. Lett. 117(15), 153002 (2016)

    Google Scholar 

  • S.P. Weathersby, G. Brown, M. Centurion, T.F. Chase, R. Coffee, J. Corbett, J.P. Eichner, J.C. Frisch, A.R. Fry, M. Gühr, N. Hartmann, C. Hast, R. Hettel, R.K. Jobe, E.N. Jongewaard, J.R. Lewandowski, R.K. Li, A.M. Lindenberg, I. Makasyuk, J.E. May, D. McCormick, M.N. Nguyen, A.H. Reid, X. Shen, K. Sokolowski-Tinten, T. Vecchione, S.L. Vetter, J. Wu, J. Yang, H.A. Dürr, X.J. Wang: Mega-electron-volt ultrafast electron diffraction at SLAC National Accelerator Laboratory, Rev. Sci. Instrum. 86(7), 073702 (2015)

    CAS  Google Scholar 

  • J. Yang, M. Guehr, T. Vecchione, M.S. Robinson, R. Li, N. Hartmann, X. Shen, R. Coffee, J. Corbett, A. Fry, K. Gaffney, T. Gorkhover, C. Hast, K. Jobe, I. Makasyuk, A. Reid, J. Robinson, S. Vetter, F. Wang, S. Weathersby, C. Yoneda, X. Wang, M. Centurion: Femtosecond gas phase electron diffraction with MeV electrons, Faraday Discuss. 194, 563 (2016)

    CAS  Google Scholar 

  • X.J. Wang, X. Qiu, I. Ben-Zvi: Experimental observation of high-brightness microbunching in a photocathode RF electron gun, Phys. Rev. E 54(4), R3121 (1996)

    CAS  Google Scholar 

  • O. Bostanjoglo: High-speed electron microscopy. In: Electron Microscopy and Holography, Advances in Imaging and Electron Physics, Vol. 121, ed. by P.W. Hawkes (Elsevier, Amsterdam 2002) pp. 1–51

    Google Scholar 

  • H. Dömer, O. Bostanjoglo: High-speed transmission electron microscope, Rev. Sci. Instrum. 74(10), 4369 (2003)

    Google Scholar 

  • T. LaGrange, M.R. Armstrong, K. Boyden, C.G. Brown, G.H. Campbell, J.D. Colvin, W.J. DeHope, A.M. Frank, D.J. Gibson, F.V. Hartemann, J.S. Kim, W.E. King, B.J. Pyke, B.W. Reed, M.D. Shirk, R.M. Shuttlesworth, B.C. Stuart, B.R. Torralva, N.D. Browning: Single-shot dynamic transmission electron microscopy, Appl. Phys. Lett. 89(4), 044105 (2006)

    Google Scholar 

  • J.S. Kim, T. LaGrange, B.W. Reed, M.L. Taheri, M.R. Armstrong, W.E. King, N.D. Browning, G.H. Campbell: Imaging of transient structures using nanosecond in situ TEM, Science 321(5895), 1472 (2008)

    CAS  Google Scholar 

  • A.H. Zewail: Four-dimensional electron microscopy, Science 328(5975), 187 (2010)

    CAS  Google Scholar 

  • A. Rose: Television pickup tubes and the problem of vision, Adv. Electron. Electron Phys. 1, 131 (1948)

    Google Scholar 

  • B.W. Reed, M.R. Armstrong, N.D. Browning, G.H. Campbell, J.E. Evans, T. LaGrange, D.J. Masiel: The evolution of ultrafast electron microscope instrumentation, Microsc. Microanal. 15(4), 272 (2009)

    CAS  Google Scholar 

  • J.C.H. Spence, G. Subramanian, P. Musumeci: Hollow cone illumination for fast TEM, and outrunning damage with electrons, J. Phys. B 48(21), 214003 (2015)

    Google Scholar 

  • R.F. Egerton, P. Li, M. Malac: Radiation damage in the TEM and SEM, Micron 35(6), 399 (2004)

    CAS  Google Scholar 

  • D.H. Dowell, M. Ferrario, T. Kimura, J. Lewellen, C. Limborg, P. Raimondi, J.F. Schmerge, L. Serafini, T. Smith, L. Young: A two-frequency RF photocathode gun, Nucl. Instrum. Methods Phys. Res. A 528(1), 316 (2004)

    CAS  Google Scholar 

  • J.C.H. Spence: High-Resolution Electron Microscopy (Oxford Univ. Press, Oxford 2013)

    Google Scholar 

  • J.K. Lim, P. Frigola, G. Travish, J.B. Rosenzweig, S.G. Anderson, W.J. Brown, J.S. Jacob, C.L. Robbins, A.M. Tremaine: Adjustable, short focal length permanent-magnet quadrupole based electron beam final focus system, Phys. Rev. ST Accel. Beams 8(7), 072401 (2005)

    Google Scholar 

  • D. Cesar, J. Maxson, P. Musumeci, Y. Sun, J. Harrison, P. Frigola, F.H. O'Shea, H. To, D. Alesini, R.K. Li: Demonstration of single-shot picosecond time-resolved MeV electron imaging using a compact permanent magnet quadrupole based lens, Phys. Rev. Lett. 117(2), 024801 (2016)

    CAS  Google Scholar 

  • L. Cultrera, S. Karkare, H. Lee, X. Liu, I. Bazarov, B. Dunham: Cold electron beams from cryocooled, alkali antimonide photocathodes, Phys. Rev. ST Accel. Beams 18, 113401 (2015)

    Google Scholar 

  • T. Shibuya, N. Hayashizaki, M. Yoshida: Fabrication of two dimensional nano-scale photocathode arrays in transparent conductor for high coherence beam generation. In: Proc. Int. Part. Accel. Conf. IPAC'16 (2016) p. WEPMY040

    Google Scholar 

  • H. Lee, L. Cultrera, I. Bazarov: Intrinsic emittance reduction in transmission mode photocathodes, Appl. Phys. Lett. 108(12), 124105 (2016)

    Google Scholar 

  • F. Carbone, B. Barwick, O.H. Kwon, H.S. Park, J.S. Baskin, A.H. Zewail: EELS femtosecond resolved in 4-D ultrafast electron microscopy, Chem. Phys. Lett. 468, 107 (2009)

    CAS  Google Scholar 

  • F. Carbone, O.H. Kwon, A.H. Zewail: Dynamics of chemical bonding mapped by energy-resolved 4-D electron microscopy, Science 325, 181 (2009)

    CAS  Google Scholar 

  • L. Piazza, C. Ma, H.X. Yang, A. Mann, Y. Zhu, J.Q. Li, F. Carbone: Ultrafast structural and electronic dynamics of the metallic phase in a layered manganite, Struct. Dyn. 1, 014501 (2014)

    CAS  Google Scholar 

  • D.A. Plemmons, S.T. Park, A.H. Zewail, D.J. Flannigan: Characterization of fast photoelectron packets in weak and strong laser fields in ultrafast electron microscopy, Ultramicroscopy 146, 97 (2014)

    CAS  Google Scholar 

  • R.M. van der Veen, T.J. Penfold, A.H. Zewail: Ultrafast core-loss spectroscopy in 4-D electron microscopy, Struct. Dyn. 2, 024302 (2015)

    Google Scholar 

  • A. Feist, K.E. Echternkamp, J. Schauss, S.V. Yalunin, S. Schäfer, C. Ropers: Quantum coherent optical phase modulation in an ultrafast transmission electron microscope, Nature 521, 200 (2015)

    CAS  Google Scholar 

  • R.F. Egerton: Electron Energy-Loss Spectroscopy in the Electron Microscope, 3rd edn. (Springer, New York 2011)

    Google Scholar 

  • R.K. Li, X.J. Wang: Femtosecond mega-electron-volt electron energy-loss spectroscopy, Phys. Rev. Appl. 8, 054017 (2017)

    Google Scholar 

  • F. Fu, S. Liu, P. Zhu, D. Xiang, J. Zhang, J. Cao: High quality single shot ultrafast MeV electron diffraction from a photocathode radio-frequency gun, Rev. Sci. Instrum. 85(8), 083701 (2014)

    Google Scholar 

  • L.K. Rudge, S. Mathisen, P. Aden, R.J. Cash, J.A. Clarke, D.M.P. Holland, J.W. McKenzie, M.D. Roper, T.C.Q. Noakes, J. Jones, A. Kalinin, B.L. Militsyn, B.D. Muratori, D. Scott, F. Jackson, P. Williams, Y. Saveliev, D. Angal-Kalinin, M. Surman, D.A. Wann, P.D. Lane, J.G. Underwood: Single shot multi MeV ultrafast electron diffraction at VELA. In: Proc. IPAC2014 (2014) p. TUPW1017

    Google Scholar 

  • S. Setiniyaz, H.W. Kim, I.-H. Baek, J. Nam, M. Chae, B.-H. Han, B. Gudkov, K.H. Jang, S. Park, Y.U. Jeong, S. Miginsky, N. Vinokurov: Beam characterization at the KAERI UED beamline, J. Korean Phys. Soc. 69(6), 1019 (2016)

    Google Scholar 

Download references

Acknowledgements

Pietro Musumeci would like to acknowledge graduate student E. Cropp (partially supported by the National Science Foundation under Grant No. DMR 1548924) who patiently helped with final editing and sorting of the references.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Pietro Musumeci .

Editor information

Editors and Affiliations

Rights and permissions

Reprints and permissions

Copyright information

© 2019 Springer Nature Switzerland AG

About this chapter

Check for updates. Verify currency and authenticity via CrossMark

Cite this chapter

Musumeci, P., Li, R. (2019). High-Energy Time-Resolved Electron Diffraction. In: Hawkes, P.W., Spence, J.C.H. (eds) Springer Handbook of Microscopy. Springer Handbooks. Springer, Cham. https://doi.org/10.1007/978-3-030-00069-1_19

Download citation

Publish with us

Policies and ethics