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Analogy between Surface and Molecular Organometallic Chemistry

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Book cover Surface and Interfacial Organometallic Chemistry and Catalysis

Part of the book series: Topics in Organometallic Chemistry ((TOPORGAN,volume 16))

Abstract

Homogeneous and heterogeneous catalysis traditionally pertains to different communities, and it is thought that they are directed by different rules. In contrast, surface organometallic chemistry has been developed on the basis that chemical bonds are formed and cleaved in both cases, and therefore that common features between these two fields exist, and that they are based on similar molecular phenomena. In this review, the reaction of organometallic reagents with oxides or metallic particles, the method of characterization of these solids and their reactivity are discussed. This approach, named surface organometallic chemistry, leads to better defined heterogeneous catalysts, which can be understood at a molecular level, and therefore allowing structure-activity relationships to be obtained. Analogies and differences between molecular and surface organometallic chemistry will also be addressed.

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Acknowledgments

We are grateful to the CNRS, CPE Lyon, the Minister of Research and Education, the Région Rhônes-Alpes district, BASF AG, BP Chemicals, Rhodia, Shell and IFP for financial support and helpful discussions. We also want to thank the numerous students and research associates who have participated over the years in this research effort.

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  1. Laboratoire de Chimie Organometallique de Surface, UMR 9986 CPE Lyon---CNRS, 43 Bd du 11 Novembre 1918, 69616, Villeurbanne Cedex, France

    Jean-Pierre Candy, Christophe Copéret & Jean-Marie Basset

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  1. Jean-Pierre Candy
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Correspondence to Christophe Copéret .

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Candy, JP., Copéret, C., Basset, JM. Analogy between Surface and Molecular Organometallic Chemistry. In: Copéret, C., Chaudret, B. (eds) Surface and Interfacial Organometallic Chemistry and Catalysis. Topics in Organometallic Chemistry, vol 16. Springer, Berlin, Heidelberg. https://doi.org/10.1007/b138076

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