Abstract
The energy sector is one of the main sources of greenhouse gas emissions, in both the transport and electricity subsectors. Taking into account the current context of the energy sector, relevant case studies concerning biofuels and CO2 capture in power plants are defined and inventoried to evaluate their carbon footprints; the suitability of these carbon footprints as single indicators is then discussed. The methodological framework proposed in the Life Cycle Assessment standards is followed. The fuel systems evaluated involve second-generation biofuels from short-rotation poplar biomass: (i) synthetic fuels (gasoline and diesel) produced via biomass pyrolysis and bio-oil upgrading and (ii) hydrogen produced via biomass gasification and biosyngas processing. Four case studies of coal power plants with CO2 capture technology are also evaluated, including post-combustion CO2 recovery through chemical absorption, membrane separation, cryogenic fractionation, and pressure swing adsorption. Inventory data for the analysis are based on process simulation, robust databases, and scientific literature. The carbon footprints calculated show a promising life-cycle global warming performance of the energy products evaluated. However, conflicting results are found when evaluating other impact categories. Therefore, decisions and recommendations based solely on carbon footprints only capture a partial picture of the environmental performance, although different levels of risk are associated with the use of carbon footprints as single indicators, depending on the type of systems and products under evaluation. The use of multi-indicator approaches is recommended because the inclusion of additional impact categories leads to a more comprehensive evaluation of the environmental performance of energy product systems, thus facilitating a more sensible decision-making process oriented towards environmental sustainability.
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Abbreviations
- ADP:
-
Abiotic depletion potential
- AP:
-
Acidification potential
- CCS:
-
CO2 capture and storage
- CCU:
-
CO2 capture and utilization
- CED:
-
Cumulative non-renewable energy demand
- CF:
-
Carbon footprinting
- CFB:
-
Circulating fluidized bed
- CO2 eq:
-
Carbon dioxide equivalent
- DEA:
-
Data envelopment analysis
- EEA:
-
European Environment Agency
- EP:
-
Eutrophication potential
- FU:
-
Functional unit
- GCC:
-
Gas and char combustor
- GHG:
-
Greenhouse gas
- GWP:
-
Global warming impact potential
- IPCC:
-
Intergovernmental Panel on Climate Change
- ISO:
-
International Organization for Standardization
- LCA:
-
Life cycle assessment
- LCI:
-
Life cycle inventory analysis
- LCIA:
-
Life cycle impact assessment
- MEA:
-
Monoethanolamine
- ODP:
-
Ozone layer depletion potential
- PAS:
-
Publicly available specification
- POFP:
-
Photochemical oxidant formation potential
- PSA:
-
Pressure swing adsorption
- RED:
-
Renewable energy directive
- SMR:
-
Steam methane reforming
- TS:
-
Technical specification
- WGS:
-
Water-gas shift
References
Aspen Technology (2013) Aspen Plus®. http://www.aspentech.com/products/aspen-plus.aspx. Accessed 10 Oct 2013
British Standards Institution (2011) PAS 2050:2011 Specification for the assessment of the life cycle greenhouse gas emissions of goods and services. BSI, London
Cooper WW, Seiford LM, Tone K (2007) Data envelopment analysis: a comprehensive text with models, applications, references and DEA-solver software. Springer, New York
Curran MA (2007) Studying the effect on system preference by varying coproduct allocation in creating life-cycle inventory. Environ Sci Technol 41:7145–7151
Dones R, Bauer C, Bolliger R et al (2007) Life cycle inventories of energy systems: Results for current systems in Switzerland and other UCTE countries, ecoinvent report No. 5. Swiss Centre for Life Cycle Inventories, Dübendorf
European Commission (2006) Biofuels in the European Union—a vision for 2030 and beyond. European Communities, Luxembourg
European Environment Agency (2009) EMEP/EEA air pollutant emission inventory guidebook 2009. EEA, Copenhagen
European Union (2009) Directive 2009/28/EC of the European Parliament and of the Council of 23 April 2009 on the promotion of the use of energy from renewable sources and amending and subsequently repealing Directives 2001/77/EC and 2003/30/EC. Official Journal of the European Union, 5 June 2009
Fan J, Kalnes TN, Alward M et al (2011) Life cycle assessment of electricity generation using fast pyrolysis bio-oil. Renew Energ 36:632–641
Finkbeiner M (2009) Carbon footprinting—opportunities and threats. Int J Life Cycle Ass 14:91–94
Forster P, Ramaswamy V, Artaxo P et al (2007) Changes in atmospheric constituents and in radiative forcing. In: Solomon S, Qin D, Manning M et al (eds) Climate change 2007: the physical science basis—contribution of working group I to the fourth assessment report of the intergovernmental panel on climate change. Cambridge University Press, Cambridge, pp 129–234
Frischknecht R, Jungbluth N, Althaus HJ et al (2007) Overview and methodology, ecoinvent report No. 1. Swiss Centre for Life Cycle Inventories, Dübendorf
Gasol CM, Gabarrell X, Antón A et al (2009) LCA of poplar bioenergy system compared with Brassica carinata energy crop and natural gas in regional scenario. Biomass Bioenerg 33:119–129
Goedkoop M, Schryver A de, Oele M et al (2010) Introduction to LCA with SimaPro 7. PRé Consultants, Amersfoort
Guinée JB, Gorrée M, Heijungs R et al (2001) Life cycle assessment: an operational guide to the ISO standards. Centre of Environmental Science, Leiden
Hoefnagels R, Smeets E, Faaij A (2010) Greenhouse gas footprints of different biofuel production systems. Renew Sust Energ Rev 14:1661–1694
Huber GW, Iborra S, Corma A (2006) Synthesis of transportation fuels from biomass: chemistry, catalysts, and engineering. Chem Rev 106:4044–4098
International Energy Agency (2012) World Energy Outlook 2012. OECD/IEA, Paris
International Organization for Standardization (2006a) ISO 14040:2006 Environmental management—life cycle assessment—principles and framework. ISO, Geneva
International Organization for Standardization (2006b) ISO 14044:2006 Environmental management—life cycle assessment—requirements and guidelines. ISO, Geneva
International Organization for Standardization (2013) ISO/TS 14067:2013 Greenhouse gases—carbon footprint of products—requirements and guidelines for quantification and communication. ISO, Geneva
Iribarren D (2010) Life cycle assessment of mussel and turbot aquaculture: application and insights. University of Santiago de Compostela, Santiago de Compostela
Iribarren D, Hospido A, Moreira MT, Feijoo G (2010a) Carbon footprint of canned mussels from a business-to-consumer approach—a starting point for mussel processors and policy makers. Environ Sci Policy 13:509–521
Iribarren D, Vázquez-Rowe I, Moreira MT, Feijoo G (2010b) Further potentials in the joint implementation of life cycle assessment and data envelopment analysis. Sci Total Environ 408:5265–5272
Iribarren D, Dufour J (2012) Life cycle assessment of biodiesel production from free fatty acid-rich wastes. Renew Energ 38:155–162
Iribarren D, Peters JF, Dufour J (2012a) Life cycle assessment of transportation fuels from biomass pyrolysis. Fuel 97:812–821
Iribarren D, Peters JF, Petrakopoulou F, Dufour J (2012b) Well-to-wheels comparison of the environmental profile of pyrolysis-based biofuels. In: Krautkremer B, Ossenbrink H, Baxter D et al (eds) Proceedings of the 20th European biomass conference and exhibition. ETA-Florence Renewable Energies, Florence, pp 2195–2198
Iribarren D, Susmozas A, Sanz A (2013a) Contrasting the life-cycle performance of conventional and alternative diesel fuels. In: Silva C, Rivera A (eds) Diesel fuels: characteristics, performances and environmental impacts. Nova Science Publishers, New York, pp 153–167
Iribarren D, Susmozas A, Dufour J (2013b) Life-cycle assessment of Fischer–Tropsch products from biosyngas. Renew Energ 59:229–236
Iribarren D, Petrakopoulou F, Dufour J (2013c) Environmental and thermodynamic evaluation of CO2 capture, transport and storage with and without enhanced resource recovery. Energy 50:477–485
Kendall A, Yuan J (2013) Comparing life cycle assessments of different biofuel options. Curr Opin Chem Biol 17:439–443
Khoo HH, Tan RBH (2006) Life cycle investigation of CO2 recovery and sequestration. Environ Sci Technol 40:4016–4024
Kohl M, Iribarren D, Petrakopoulou F, Dufour J (2013) Life cycle assessment of bioethanol from microalgae. In: Krautkremer B, Ossenbrink H, Baxter D et al (eds) Proceedings of the 21st European biomass conference and exhibition. ETA-Florence Renewable Energies, Florence, pp 1818–1822
Laurent A, Olsen SI, Hauschild MZ (2012) Limitations of carbon footprint as indicator of environmental sustainability. Environ Sci Technol 46:4100–4108
Mata TM, Martins AA, Caetano NS (2010) Microalgae for biodiesel production and other applications: a review. Renew Sust Energ Rev 14:217–232
Merrild H (2009) Indicators for waste management: how representative is global warming as an indicator for environmental performance of waste management?. Technical University of Denmark, Kongens Lyngby
Mondal MK, Balsora HK, Varshney P (2012) Progress and trends in CO2 capture/separation technologies: a review. Energy 46:431–441
Pehnt M, Henkel J (2009) Life cycle assessment of carbon dioxide capture and storage from lignite power plants. Int J Greenh Gas Con 3:49–66
Reap J, Roman F, Duncan S, Bras B (2008a) A survey of unresolved problems in life cycle assessment—part 1: goal and scope and inventory analysis. Int J Life Cycle Ass 13:290–300
Reap J, Roman F, Duncan S, Bras B (2008b) A survey of unresolved problems in life cycle assessment—part 2: impact assessment and interpretation. Int J Life Cycle Ass 13:374–388
Schmidheiny S (1992) Changing course: a global business perspective on development and the environment. MIT Press, Cambridge
Schreiber A, Zapp P, Kuckshinrichs W (2009) Environmental assessment of German electricity generation from coal-fired power plants with amine-based carbon capture. Int J Life Cycle Ass 14:547–559
Sinden G (2009) The contribution of PAS 2050 to the evolution of international greenhouse gas emission standards. Int J Life Cycle Ass 14:195–203
Singh B, Strømman AH, Hertwich EG (2011) Comparative life cycle environmental assessment of CCS technologies. Int J Greenh Gas Con 5:911–921
Spath P, Aden A, Eggeman T et al (2005) Biomass to hydrogen production detailed design and economics utilizing the Battelle Columbus Laboratory indirectly-heated gasifier. NREL, Golden
Susmozas A, Iribarren D, Dufour J (2013) Life-cycle performance of indirect biomass gasification as a green alternative to steam methane reforming for hydrogen production. Int J Hydrogen Energ 38:9961–9972
Swain PK, Das LM, Naik SN (2011) Biomass to liquid: a prospective challenge to research and development in 21st century. Renew Sust Energ Rev 15:4917–4933
Vázquez-Rowe I, Iribarren D (2014) Life-cycle benchmarking approaches oriented towards energy policy making: Launching the CFP+DEA method. J Clean Prod (in press)
Vázquez-Rowe I, Iribarren D, Moreira MT, Feijoo G (2010) Combined application of life cycle assessment and data envelopment analysis as a methodological approach for the assessment of fisheries. Int J Life Cycle Ass 15:272–283
Verein Deutscher Ingenieure (2012) VDI guideline 4600: cumulative energy demand (KEA) —terms, definitions, methods of calculation. VDI, Düsseldorf
Weidema BP, Thrane M, Christensen P et al (2008) Carbon footprint: a catalyst for LCA? J Ind Ecol 12:3–6
Acknowledgements
This research has been supported by the Regional Government of Madrid (S2009/ENE-1743) and the Spanish Ministry of Economy and Competitiveness (CTQ2011-28216-C02-02 and ENE2011-29643-C02-01). The authors would like to thank Jens F. Peters and Ana Susmozas for valuable scientific exchange.
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Iribarren, D., Dufour, J. (2014). Carbon Footprint as a Single Indicator in Energy Systems: The Case of Biofuels and CO2 Capture Technologies. In: Muthu, S. (eds) Assessment of Carbon Footprint in Different Industrial Sectors, Volume 2. EcoProduction. Springer, Singapore. https://doi.org/10.1007/978-981-4585-75-0_4
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