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The Development and Applications of Phase Cycling in Multidimensional Optical Spectroscopy

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Book cover Coherent Multidimensional Spectroscopy

Part of the book series: Springer Series in Optical Sciences ((SSOS,volume 226))

Abstract

Although most experiments are performed using a non-collinear beam geometry, multidimensional optical spectroscopy experiments can also be performed using collinear and partially collinear beam geometries. Phase cycling is an important procedure to enable multidimensional optical spectroscopy experiments to be performed in collinear and partially collinear beam geometries. In this chapter, we present the general theory of phase cycling and summarizes the development and applications of the phase cycling procedures in various multidimensional optical spectroscopies. These applications include fully collinear two dimensional optical spectroscopy, pump-probe geometry third order and fifth order two dimensional optical spectroscopies, and fifth order three dimensional optical spectroscopy.

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Acknowledgements

This work is supported by grants from the Singapore Ministry of Education Academic Research Fund (Tier 2 MOE2015-T2-1-039 and Tier 1 RG16/15).

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Authors and Affiliations

  1. Division of Chemistry and Biological Chemistry, School of Physical and Mathematical Sciences, Nanyang Technological University, 21 Nanyang Link, Singapore, 637371, Singapore

    Howe-Siang Tan

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  1. Howe-Siang Tan
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Correspondence to Howe-Siang Tan .

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  1. Department of Chemistry, Korea University, Seoul, Korea (Republic of)

    Minhaeng Cho

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Tan, HS. (2019). The Development and Applications of Phase Cycling in Multidimensional Optical Spectroscopy. In: Cho, M. (eds) Coherent Multidimensional Spectroscopy. Springer Series in Optical Sciences, vol 226. Springer, Singapore. https://doi.org/10.1007/978-981-13-9753-0_4

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