Abstract
Low driving voltage, high luminance, and high efficiency are the important parameters of organic light-emitting diodes (OLEDs) for their application of display and lighting. Usually, synthesis of new materials, doping technique and designing suitable device structures were the main methods to use for realizing the aim of the wide application of OLEDs. In this paper, we try to obtain a high efficiency and low driving voltage tandem OLED with ultrathin films through optimizing the thickness of hole transporting layer (HTL), electron transport layer (ETL), emission layer (EML), and charge generation layer (CGL). As a result, we got the ultrathin tandem OLED with a very low driving voltage of 7.44 V, the luminance of 16,080 cd/m2, the current efficiency of 16.08 cd/A, and power efficiency of 6.28 lm/W, respectively. This research not only saves the cost and improves the power efficiency, which may supply a theoretical basis for the development of OLEDs in the lighting field.
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References
Pfeiffer, M., Forrest, S.R., Leo, K., Thompson, M. E.: Electrophosphorescent p-i-n organic light emitting devices for Very-High-Efficiency Flat-Panel displays. Adv. Mater. (Weinheim, Ger.) 14, 1633 (2002)
Zhou, X., Blochwitz, J., Pfeiffer, M., Nollau, A., Fritz, T., Leo, K.: Enhanced hole injection into amorphous hole-transport layers of organic light emitting diodes using controlled p-type doping. Adv. Funct. Mater. 11, 310 (2001)
Qasim, K., Wang, B.P., Zhang, Y.P., Li, P.F., Wang, Y.S., Li, S.J., Lee, S. T., Liao, L.S., Lei, W., Bao, Q.L.: Solution-processed extremely efficient multicolor perovskite light emitting diodes utilizing doped electron transport layer. Adv. Funct. Mater. 27(21), 1606874(2017)
Huang, J., Pfeiffer, M., Werner, A., Blochwitz, J., Leo, K., Liu, S.: Low-voltage organic electroluminescent devices using pin structures. Appl. Phys. Lett. 80, 139 (2002)
Soman, A., Manuraj, M., Unni, K.N.N.: Addressing the efficiency roll-off in a fluorescent OLED by facile electron transport layer doping and carrier confinement. Opt. Mater. 79, 413–419 (2018)
Walzer, K., Maenning, B., Pfeiffer, M., Leo, K.: Highly efficient organic devices based on electrically doped transport layers. Chem. Rev. 107, 1233 (2007)
Chang, C.C., Hsieh, M.T., Chen, J.F., Hwang, S.W., Chen, C.H.: Highly power efficient organic light emitting diodes with a doping layer. Appl. Phys. Lett. 89, 253504 (2006)
Ikeda, H., Sakata, J., Hayakawa, M., Aoyama, T., Kawakami, T., Kamata, K., Iwaki, Y., Seo, S., Noda, Y., Nomura, R., Yamazaki, S.: Low-Drive-Voltage OLEDs with a buffer layer having molybdenum oxide. SID Int. Symp. Digest Tech. Papers 37, 923 (2006)
Chen, D.C., Liu, K.K., Gan, L., Liu, M., Gao, K., Xie, G.Z., Ma, Y.G., Shi, Y.C., Su, J.: Modulation of exciton generation in organic active planar p-n heterojunction: toward low driving voltage and high-efficiency OLEDs employing conventional and thermally activated delayed fluorescent emitters. Adv. Mater. 28(31), 6758–6765 (2016)
Deng, Y.H., Li, Y.Q., Ou, Q.D., Wang, Q.K., Sun, F.Z., Chen, X.Y., Tang, J.X.: The doping effect of cesium-based compounds on carrier transport and operational stability in organic light-emitting diodes. Org. Electron. 15, 1215–1221 (2014)
Chiba, T., Pu, Y.J., Ide, T., Ohisa, S., Fukuda, H., Hikichi, T., Takashima, D., Takahashi, T., Kawata, S., Kido, J.: Addition of Lithium 8-Quinolate into polyethylenimine electron-injection layer in OLEDs: not only reducing driving voltage but also improving device lifetime. ACS Appl. Mater. Interfaces. 9(21), 18113–18119 (2017)
Gao, W., Kahn, A.: Controlled p-doping of zinc phthalocyanine by coevaporation with tetrafluorotetracyanoquinodimethane: a direct and inverse photoemission study. Appl. Phys. Lett. 79, 4040 (2001)
Walzer, K., Maennig, B., Pfeiffer, M., Leo, K.: Highly efficient organic devices based on electrically doped transport layers. Chem. Rev. 107(4), 1233 (2007)
Zhou, Y., Fuentes-Hernandez, C., Shim, J., Meyer, J., Giordano, A.J., Li, H., Winget, P., Papadopoulos, T., Cheun, H., Kim, J., Fenoll, M., Dindar, A., Haske, W., Najafabadi, E., Khan, T.M., Sojoudi, H., Barlow, S., Graham, S., Brédas, J. L., Marder, S.R., Kahn, A., Kippelen, B.: A universal method to produce low-work function electrodes for organic electronics. Science 336, 327 (2012)
Deng, Z.B., Ding, X.M., Lee, S.T., Gambling, W.A.: Enhanced brightness and efficiency in organic electroluminescent devices using SiO2 buffer layers. Appl. Phys. Lett. 74, 2227 (1999)
Tong, S.W., Lee, C.S., Lifshitz, Y., Gao, D.Q., Lee, S.T.: Conducting fluorocarbon coatings for organic light-emitting diodes. Appl. Phys. Lett. 84, 4032 (2004)
Zhao, J.M., Zhang, S.T., Wang, X.J., Zhang, Y.Q., Wang, X.Z., Zhong, G.Y., Wang, Z.J., Ding, W., Huang, X.M., Hou, X.Y.: Dual role of LiF as a hole-injection buffer in organic light-emitting diodes. Appl. Phys. Lett. 84, 2913 (2003)
Wang, C.T., Ting, C.C., Kao, P.C., Li, S.R., Chu, S.Y.: Improvement of OLED performance by tuning of silver oxide buffer layer composition on silver grid surface using UV-ozone treatment. Appl. Phys. Lett. 113, 051602 (2018)
Zhang, J., Xin, L.W., Gao, J., Liu, Y., Rui, H.S., Lin, X., Hua, Y.L., Wu, X.M., Yin, S.G.: Improving the performance of organic light-emitting devices by incorporating non-doped TCNQ as electron buffer layer. J. Mater. Sci.: Mater. Electron. 28(17), 12761–12767 (2017)
Han, C., Xie, G., Xu, H., Zhang, Z., Yu, D., Zhao, Y., Yan, P., Deng, Z., Li, Q., Liu, S.: Towards highly efficient blue-phosphorescent organic light-emitting diodes with low operating voltage and excellent efficiency stability. Chem. Eur. J. 17, 445 (2011)
Gong, S., Chang, Y.L., Wu, K., White, R., Lu, Z.H., Song, D., Yang, C.: High-power-efficiency blue electrophosphorescence enabled by the synergistic combination of phosphine-oxide-based host and electron-transporting materials. Chem. Mater. 26, 1463 (2014)
Sasabe, H., Gonmori, E., Chiba, T., Li, Y.J., Tanaka, D., Su, S.J., Takeda, T., Pu, Y.J., Nakayama, K.I., Kido, J.: Wide-energy-gap electron-transport materials containing 3, 5-dipyridylphenyl moieties for an ultra high efficiency blue organic light-emitting device. Chem. Mater. 20, 5951 (2008)
Xiao, L., Su, S.J., Agata, Y., Lan, H., Kido, J.: Nearly 100% internal quantum efficiency in an organic Blue-Light electrophosphorescent device using a weak electron transporting material with a wide energy gap. Adv. Mater. 21, 1271 (2009)
Ye, H., Chen, D., Liu, M., Su, S.J., Wang, Y.F., Lo, C.C., Lien, A., Kido, J.: Pyridine-Containing Electron-Transport materials for highly efficient blue phosphorescent OLEDs with ultralow operating voltage and reduced efficiency roll-off. Adv. Funct. Mater. 24, 3268 (2014)
Jeon, S.O., Jang, S.E., Son, H.S., Lee, J.Y.: External quantum efficiency above 20% in deep blue phosphorescent organic light-emitting diodes. Adv. Mater. 23, 1436 (2011)
Kim, C.Y., Ha, D.G., Kang, H.H., Yun, H.J., Kwon, S.K., Kim, J.J., Kim, Y.H.: Synthesis and characterization of new blue light emitting iridium complexes containing a trimethylsilyl group. J. Mater. Chem. 22, 22721 (2012)
Deng, Y.H., Ou, Q.D., Wang, Q.K., Wei, H.X., Li, Y.Q., Lee, S.T., Tang, J.X.: The role of charge generation layers in the operational stability of tandem organic light-emitting diodes. J. Mater. Chem. C 2, 1982–1989 (2014)
Deng, Y.H., Wang, J.J., Ou, Q.D., Zhang, D.Y., Chen, L.Z., Li, Y.Q., Tang, J.X.: The electro-optic performance and photovoltaic effect of organic devices based on cesium carbonate/Al/molybdenum trioxide intermediate connector. Org. Electron. 51, 452–457 (2017)
Fung, M.K., Li, Y.Q., Liao, L.S.: Lead-free inverted planar Formamidinium Tin Triiodide Perovskite solar cells achieving power conversion efficiencies up to 6.22%. Adv. Mater. 28(42), 1–28 (2016)
Acknowledgements
The authors gratefully acknowledge the Hunan Provincial Natural Science Foundation of China (No. 2018JJ3010, 2017JJ2009), Scientific Research Fund of Hunan Provincial Education Department (No. 15B033), the Hunan Provincial Applied Basic Research Base of Optoelectronic Information Technology (GD18K05), Science and Technology Plan Project of Hunan Province (No. 2016TP1020), Open fund project of Hunan Provincial Key Laboratory of Intelligent Information Processing and Application for Hengyang normal university (No. 2017IIPAYB02), the Science and Technology Development Plan Project in Hengyang City (No. 2017KJ159), the Excellent Talents Program of HYNU, and the college students inquiry learning and innovative experimental project of Hengyang Normal University (No. CX1754).
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Deng, Y. et al. (2020). An Ultrathin Tandem Organic Light-Emitting Diodes with Very Low Driving Voltage and High Efficiency. In: Peng, Y., Dong, X. (eds) Proceedings of 2018 International Conference on Optoelectronics and Measurement. Lecture Notes in Electrical Engineering, vol 567. Springer, Singapore. https://doi.org/10.1007/978-981-13-8595-7_15
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DOI: https://doi.org/10.1007/978-981-13-8595-7_15
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