Abstract
Magnetic hysteretic behavior of a system composed of oriented crystallites of Mn12-acetate complex were investigated as a function of temperature, and the directions of external magnetic field. Periodic magnetization steps were observed in the hysteresis loops. These steps suggest the existence of peaks in the relaxation rate at the fields corresponding to the jumps, which has been confirmed by the relaxation experiments performed with these fields at different temperatures. We attribute these observations to thermally assisted resonant tunneling of the magnetic moment the cluster in a double well potential, and propose a theoretical model to account for our results.
Access this chapter
Tax calculation will be finalised at checkout
Purchases are for personal use only
Preview
Unable to display preview. Download preview PDF.
References
L. Neel (1955) Adv. Phys. 4, 191.
J. Tejada, X.X Zhang, and EM. Chudnovsky (1993) Phys. Rev. B 47, 14977.
X.X. Zhang et al. (1994) J. Magn. Magn. Matter. 137, L235.
J.M Hernandez, X.X. Zhang, and J. Tejada (1995) J. Appl. Phys. 79, 4686.
E.M. Chudnovsky and L. Gunther (1988) Phys. Rev. Lett. 60, 661; Phys. Rev. B 37, 9455.
E.M. Chudnovsky, D.P. DiVincenzo (1993) Phys. Rev. B 48, 10548.
J.R. Friedman, M. Sarachick, J. Tejada, and R. Ziolo (1996), J. Appl. Phys. 79, 6031;
J.R. Friedman, M. Sarachick, J. Tejada, and R. Ziolo (1996) Phys. Rev. Lett. 76 3830.
B. Barbara et al. (1995) J. Magn. Magn. Mater. 140–144, 1825.
C. Paulsen and J.-G. Park in Quantum Tunneling of Magnetization, edited by L. Gunther and B. Barbara (Kluwer, 1995), p. 189.
C. Paulsen, J.-G. Park, B. Barbara, R. Sessoli and A. Canesehi (1995) J. Magn. Magn. Mater. 140–144, 379.
M.A. Novak and R. Sessoli in Quantum Tunneling of Magnetization, edited by L. Gunther and B. Barbara (Kluwer, 1995), p. 171.
A. Canesehi, et al. (1991) J. Am. Chem. Soc. 113, 5873.
R. Sessoli, et al. (1993) J. Am. Chem. Soc. 115, 1804.
R. Sessoli, D. Gatteschi, A. Canesehi, and M.A. Novak (1993) Nature 365, 141.
C. Paulsen, et al. (1995) J. Magn. Magn. Mater. 140–144, 1891.
M.A. Novak, R. Sessoli, A. Canesehi, and D. Gatteschi (1995) J. Magn. Magn. Mater. 146, 211.
J. Villain, F. Hartman-Boutron, R. Sessoli, and A. Rettori (1994) EuroPhys. Lett. 27, 159.
P. Politti, A. Rettori, F. Hartman-Boutron, J. Villain (1995), Phys. Rev. Lett. 75, 537.
T. Lis (1980) Acta Cryst. B 36, 2042.
J.M. Hernandez, X.X. Zhang, F. Luis, J. Bartolome, J. Tejada, and R. Ziolo, Europhys. Lett., 35, 301 (1996);
J.M. Hernandez, X.X. Zhang, J. Tejada, J.R. Friedman, and M.P. Sarachick (unpublished).
D.A. Garanin (1991) J. Phys. A: Math Gen. 24, L61.
Author information
Authors and Affiliations
Editor information
Editors and Affiliations
Rights and permissions
Copyright information
© 1997 Springer Science+Business Media Dordrecht
About this chapter
Cite this chapter
Tejada, J., Zhang, X.X., Hernandez, J.M., Friedman, J.R., Sarachik, M.P., Ziolo, R.F. (1997). Quantum Hysteretic Phenomena in Mn12-Acetate Magnetic Clusters. In: Hadjipanayis, G.C. (eds) Magnetic Hysteresis in Novel Magnetic Materials. NATO ASI Series, vol 338. Springer, Dordrecht. https://doi.org/10.1007/978-94-011-5478-9_23
Download citation
DOI: https://doi.org/10.1007/978-94-011-5478-9_23
Publisher Name: Springer, Dordrecht
Print ISBN: 978-94-010-6304-3
Online ISBN: 978-94-011-5478-9
eBook Packages: Springer Book Archive