Skip to main content

Coherent Control of Atomic Photoionization and Autoionization

  • Chapter
Coherent Control in Atoms, Molecules, and Semiconductors

Abstract

The control of the products of photoabsorption through the relative phase of two fields represents one of the schemes of coherent control which has been under continuing study and evolution over the last few years [1-8]. Its general aspects as well as a number of specific issues pertaining to small molecules are usefully reviewed and summarized in this volume by Gordon et al. With the intention of avoiding duplication of discussion and minimizing the overlap with their article, we focus our review and remarks on certain aspects of phase control in atoms. There are we believe two main motivations for studying phase control in photoabsorption. One has to do with the desire to control branching ratios of products, as amply illustrated experimentally and theoretically by Gordon et al. The other has to do with the possibility of probing atomic and molecular properties and interactions with radiation. We emphasize here the second.

This is a preview of subscription content, log in via an institution to check access.

Access this chapter

Chapter
USD 29.95
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
eBook
USD 84.99
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
Softcover Book
USD 109.99
Price excludes VAT (USA)
  • Compact, lightweight edition
  • Dispatched in 3 to 5 business days
  • Free shipping worldwide - see info
Hardcover Book
USD 109.99
Price excludes VAT (USA)
  • Durable hardcover edition
  • Dispatched in 3 to 5 business days
  • Free shipping worldwide - see info

Tax calculation will be finalised at checkout

Purchases are for personal use only

Institutional subscriptions

Preview

Unable to display preview. Download preview PDF.

Unable to display preview. Download preview PDF.

References

  1. Gordon, R.J. and Rice, S.A. (1997) Active Control of the Dynamics of Atoms and Molecules, Ann. Rev. Phys. Chem. 48, 601–641.

    Article  ADS  Google Scholar 

  2. Chen C., Yin, Y.-Y., and Elliott, D.S. (1990) Interference between Optical Transitions, Phys. Rev. Lett. 64, 507–510.

    Article  ADS  Google Scholar 

  3. Park, S.M., Lu, S.-P., and Gordon, R.J. (1991) Coherent laser control of the resonance-enhanced multiphoton ionization, J. Chem. Phys. 94, 8622–8624.

    Article  ADS  Google Scholar 

  4. Nakajima T., Lambropoulos, R, Cavalieri S., and Matera, M. (1992) Modulating ionization through phase control, Phys. Rev. A 46, 7315–7318.

    Article  ADS  Google Scholar 

  5. Nakajima, T. and Lambropoulos, P. (1993) Manipulation of the Line Shape and Final Products of Autoionization through the Phase of Electric Fields, Phys. Rev. Lett. 70, 1081–1084.

    Article  ADS  Google Scholar 

  6. Nakajima, T. and Lambropoulos, P. (1994) Effects of the phase of laser fields on autoionization, Phys. Rev. A 50, 595–610.

    Article  ADS  Google Scholar 

  7. Nakajima T., Zhang, J. and Lambropoulos, P. (1997) Phase control through channels involving multiple continua and multiple thresholds, J. Phys. B 30, 1077–1095.

    Article  ADS  Google Scholar 

  8. Shapiro M., Hepburn, J.W. and Brumer, P. (1988) Simplified laser control of unimolecular reactions simultaneous 62-1 excitation, Chem. Phys. Lett. 149, 451–454.

    Article  ADS  Google Scholar 

  9. Lefebvre-Brion, H. (1997) Study of the origin of the phase lag between signals in coherent laser control, J. Chem. Phys. 106, 2544–2546.

    Article  ADS  Google Scholar 

  10. Zhu L., Suto K., Fiss, J.A., Wada R., Seideman, T. and Gordon, R.J. (1997) Effect of Resonances on the Coherent Control of the Photoionization and Photodissociation of HI and Di, Phys. Rev. Lett. 79, 4108–4111.

    Article  ADS  Google Scholar 

  11. Seideman, T. (1998) The role of a molecular phase in two-pathway excitation schemes, J. Chem. Phys. 108, 1915–1923.

    Article  ADS  Google Scholar 

  12. Zhu L., Kleiman V., Li, X., Lu S., Trentelman, K. and Gordon, R.J. (1995) Coherent Laser Control of the Product Distribution Obtained in the Photoexcitation on Hi, Science 270, 77–80.

    Article  ADS  Google Scholar 

  13. Lambropoulos P., Maragakis, P. and Zhang, J. Two-Electron Atoms in Strong Fields, Physics Reports (to be published).

    Google Scholar 

  14. Bar-Ad S., Kner P., Marquezini, M.V., Mukamel S., and Chemla, D.S. (1997) Quantum Confined Fano Interference, Phys. Rev. Lett. 78, 1363–1366

    Article  ADS  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Editor information

Editors and Affiliations

Rights and permissions

Reprints and permissions

Copyright information

© 1999 Springer Science+Business Media Dordrecht

About this chapter

Cite this chapter

Lambropoulos, P., Nakajima, T. (1999). Coherent Control of Atomic Photoionization and Autoionization. In: Pötz, W., Schroeder, W.A. (eds) Coherent Control in Atoms, Molecules, and Semiconductors. Springer, Dordrecht. https://doi.org/10.1007/978-94-011-4552-7_5

Download citation

  • DOI: https://doi.org/10.1007/978-94-011-4552-7_5

  • Publisher Name: Springer, Dordrecht

  • Print ISBN: 978-94-010-5932-9

  • Online ISBN: 978-94-011-4552-7

  • eBook Packages: Springer Book Archive

Publish with us

Policies and ethics