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Sigma- and Pi-Conjugated Organosilicon Polymers

  • Chapter
Silicon-Containing Polymers

Abstract

Organosilicon polymers with σ anEquationd π-conjugation along the main chain constitute an important class of new functional polymers, because of their potential applications, typically as preceramic materials, photoresists, electrical- and photo-conductive materials, nonlinear optical materials and materials for organic electroluminescent devices. When the silicon moiety attaches to π-electron systems, the silicon atom substantially perturbs the electronic structure of the π-system through peculiar orbital interactions, i.e. σ-π, σ*-π, and σ*-π* conjugation [1–3], giving rise to unique properties. In the past decade, there have been extensive investigations of this field. This chapter will review the recent developments of the chemistry of σ — and π -conjugated organosilicon polymers, especially focusing on the polymers consisting of oligosilylene units and π -electron systems alternately in the main chain [4] and the polymers based on silicon-containing heterocycles such as siloles (silacyclopentadienes) [5].

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  1. Institute for Chemical Research, Kyoto University, Uji, Kyoto, 611-0011, Japan

    Shigehiro Yamaguchi & Kohei Tamao

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  1. Shigehiro Yamaguchi
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  1. University of Kent, Canterbury, UK

    Richard G. Jones

  2. Dow Corning Asia Ltd., Kanagawa, Japan

    Wataru Ando

  3. Polish Academy of Sciences, Lódz, Poland

    Julian Chojnowski

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Yamaguchi, S., Tamao, K. (2000). Sigma- and Pi-Conjugated Organosilicon Polymers. In: Jones, R.G., Ando, W., Chojnowski, J. (eds) Silicon-Containing Polymers. Springer, Dordrecht. https://doi.org/10.1007/978-94-011-3939-7_17

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