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Plutonium, Americtum and Radiocaesium in Sea Water, Sediments and Coastal Soils in Carlingford Lough

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Radionuclides in the Study of Marine Processes

Abstract

Artificial radioactivity within the sediment-water system in Carlingford Lough has been studied and the extent of transport of plutonium from sea to land has been assessed by analysing soil samples taken at selected inland sites close to the shore of the Lough. Samples of sea water, suspended particulate and sediment have been analysed for 134Cs, 137Cs, 238Pu, 239,240Pu and 241Am and the speciation of both plutonium and americium determined in Lough waters. The association of transuranium nuclides with colloids has also been examined and it has been shown that a significant proportion of the plutonium and almost all of the americium in the filtrate fraction (<0.22 µm) is in a colloidal form. In general, concentrations of radiocaesium and the transuranics were found to be very low and showed little or no enhancement when compared to similar materials sampled elsewhere near the north-east coast of Ireland. Finally, the sea-to-land transfer of plutonium and, by inference, other actinides was found to be insignificant in the vicinity of the Lough and the adjacent coastline.

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References

  1. Douglas, D.J. and Conlon, J., Physico-chemical analysis of the water in Carlingford Lough. In Carlingford Lough Marine Laboratory, Bulletin No. 6, Nov. 1990, Published by Carlingford Lough Aquaculture Association., Omeath, Ireland, ISSN 0791-4512, pp. 20–8.

    Google Scholar 

  2. Douglas, D.J., Conlon, J. and McQuaid, S., Water analysis in Carlingford Lough. In Carlingford Lough Marine Laboratory, Bulletin No. 3, May 1990, Published by Carlingford Lough Aquaculture Association, Omeath, Ireland, ISSN 0791-4512, pp. 14–23.

    Google Scholar 

  3. Caulfield, J.J. and Ledgerwood, F.K., Terrestrial gamma-ray dose rates out of doors in Northern Ireland. Environmental Monitoring Report No. 2, Department of the Environment (Northern Ireland), Belfast, November 1989, 23 pp.

    Google Scholar 

  4. O’Grady, J. and Currivan, L., Radioactivity monitoring of the Irish marine environment, 1987. Nuclear Energy Board, Dublin, Ireland, 1990, 28 pp.

    Google Scholar 

  5. Crowley, M., Mitchell, P.I., O’Grady, J., Vives, J., Sanchez-Cabeza, J.A., Vidal-Quadras, A. and Ryan, T.P., Radiocaesium and plutonium concentrations in Mytilus edulis (L.) and potential dose implications for Irish Critical Groups. Ocean and Shoreline Management, 1990, 13, 149–61.

    Article  Google Scholar 

  6. Mitchell, P.I., Sanchez-Cabeza, J. Ryan, T.P., McGarry, A.T. and Vidal-Quadras, A., Preliminary estimates of cumulative caesium and plutonium deposition in the Irish terrestrial environment. J. Radioanal. Nucl. Chem. (Articles), 1990, 138, No. 2, 241–56.

    Article  CAS  Google Scholar 

  7. Mitchell, P.I., Vives Batlle, J., O’Grady, J., Sanchez-Cabeza, J.A. and Vidal-Quadras, A., Critical group doses arising from the consumption of fish and shellfish from the western Irish Sea. In New Developments in Fundamental and Applied Radiobiology: Proc. 23rd Annual Meeting of the European Society for Radiation Biology, Dublin, 23–26 September 1990 (Eds. C.B. Seymour and Carmel Mothersill), Publ. Taylor and Francis, 1991, 380–91.

    Google Scholar 

  8. Lovett, M.B. and Nelson, D.M., Determination of some oxidation states of plutonium in sea water and associated particulate matter. In Techniques for Identifying Transuranic Speciation in Aquatic Environments, Panel Proc. Ser., Ispra, IAEA, Vienna (STI/PUB/613), 1981, pp. 27–35.

    Google Scholar 

  9. Nevissi, A. and Schell, W.R., Distribution of plutonium and americium in Bikini Atoll Lagoon. Health Phys., 1975, 28, 539–47.

    Article  CAS  Google Scholar 

  10. Nevissi, A. and Schell, W.R., Efficiency of a large volume water sampler for some radionuclides in salt and freshwater. In Proc. Fourth National Symposium on Radioecology, Corvallis, Oregon, 12–14 May 1975, The Ecological Society of America, Spec. Publ. No. 1, (Ed. CE. Cushing Jr.), Dowden, Hutchinson and Ross Inc., Stroudsburg, Pennsylvania, 1976, pp. 277–82.

    Google Scholar 

  11. Mitchell, P.I., Vives Batlle, J., Ryan, T.P., Schell, W.R., Sanchez-Cabeza, J.A. and Vidal-Quadras, A., Studies on the speciation of plutonium and americium in the western Irish Sea. These Proceedings.

    Google Scholar 

  12. Pentreath, R.J., Harvey, B.R.. and Lovett, M.B., Chemical speciation of transuranium nuclides discharged into the marine environment. In Speciation of Fission and Activation Products in the Environment (Eds. R.A. Bulman and J.R. Cooper), Elsevier, 1986, pp. 312–25.

    Google Scholar 

  13. Nelson, D.M., Larsen, R.P. and Penrose, W.R., Chemical speciation of plutonium in natural waters. In Proc. Symposium on Environmental Research on Actinide Elements, Hilton Head, South Carolina, November 7–11, 1983. US Department of Energy, August 1987, CONF-841142, pp. 27–48.

    Google Scholar 

  14. Hunt, G.J., Radioactivity in surface and coastal waters of the British Isles, 1989. Aquatic Environment Monitoring Report, No. 23, Ministry of Agriculture, Fisheries and Food Directorate of Fisheries Research, Lowestoft, 1990, 66 pp.

    Google Scholar 

  15. Garland, J.A., McKay, W.A., Burton, P.J. and Cambray, R.S., Studies of environmental radioactivity on the coasts of Northern Ireland. Nucl. Energy, 1990, 29, No. 3, 205–23.

    CAS  Google Scholar 

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© 1991 Elsevier Science Publishers Ltd

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Mitchell, P.I. et al. (1991). Plutonium, Americtum and Radiocaesium in Sea Water, Sediments and Coastal Soils in Carlingford Lough. In: Kershaw, P.J., Woodhead, D.S. (eds) Radionuclides in the Study of Marine Processes. Springer, Dordrecht. https://doi.org/10.1007/978-94-011-3686-0_28

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  • DOI: https://doi.org/10.1007/978-94-011-3686-0_28

  • Publisher Name: Springer, Dordrecht

  • Print ISBN: 978-1-85166-707-9

  • Online ISBN: 978-94-011-3686-0

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