Abstract
Ambient concentrations and dry deposition fluxes of Hg in the gas and particle phase to Lakes St. Clair, Erie and Huron were estimated with a hybrid receptor-deposition model (HRD). The ambient gas and particulate phase Hg concentrations were predicted to vary by a factor of 12 to 18 during the transport of air masses traversing the lakes. The ensemble average deposition fluxes of fine particle Hg ranged from 7 pg/m2-h to 15.3 pg/m2-h over Lake St. Clair, 0.5 to 4.2 pg/m2-h over Lake Huron and 5.1 to 20.6 pg/m2-h over Lake Erie. The deposition flux of coarse particle Hg, was in the range of 50 to 84 pg/m2-h over Lake St. Clair, 4.7 to 24.2 pg/m2-h over Lake Huron and 5.1 to 20.6 pg/m2-:h over Lake Erie. Gaseous Hg volatilized at a rate of 0.21 to 0.52 ng/m2-h from Lake Huron and 0.13 to 0.36 from Lake Erie. Gas phase Hg was deposited at a rate of 5.9 ng/m2-h and/or volatilized at a rate of 0.5 ng/m2-h from Lake St. Clair depending upon the location of the sampling site used in the HRD model. The effect of meteorological conditions, particle size distributions and type and location of the sampling sites played an important role in the transfer of atmospheric Hg to and/or from the lakes.
Access this chapter
Tax calculation will be finalised at checkout
Purchases are for personal use only
Preview
Unable to display preview. Download preview PDF.
References
Burke, J., Hoyer, M., Keeler, G.J. and Scherbatskoy, T.:1994, Water Air and Soil Pollut., in this volume.
EPA, Locating and Estimating Air Emissions from Sources of Mercury and Mercury Compounds, Midwest Research Institute, North Caroline, Interim Report, January 1993.
Fitzgerald, W.F, Gill, G A.:1979, Anal. Chem, 51, 11: 1714–1720.
Gill, G.A. and Bruland, K.W.: 1990, Environ. Sci. Technol. 24, 1392–1397.
Keeler, G.J, Hoyer, M.E. and Lamborg, C.H.: 1994a, In: Mercury Pollution: Integration and Synthesis, Watras, C.J. and Huckabee, W. (Eds), Lewis Publishers, Chelsea, MI.
Keeler, G.J., Glinsorn, G. and Pirrone, N.: 1994b, Water Air and Soil Pollut., in this volume.
Lindqvist, O., Johansson, K., Aastrup, M., Anderson, A.:1991, Water Air Soil Pollut. 55, 7–17.
Meger, S.A.:1986, Water Air Soil Pollut. 30, 411–19.
Nater, E.A. and Grigal, D.F.:1992, Nature 358, 139–41.
Norton, S.A., Dillon, P.J., Douglas E.R, Mierle, G. and Kahl, J.S. in Acidic Precipitation, Vol.3, 73, Springer, Berlin (1990).
Pirrone, N., Keeler, G.J. and Holsen, T.M.: 1994a, submitted to Environ. Sci. Technol.
Pirrone, N., Keeler, G.J. and Holsen, T.M.: 1994b, submitted to Environ. Sci. Technol.
Pirrone, N., Keeler, G.J. and Warner, P.O.: 1994, Sci. Tot. Environ, in press.
Rada, R.G., Wiener, J.G, Winfrey, M.R. and Powell, D.E.:1989, Arch. Envir. Contam. Toxicol. 18, 175–81.
Slemer, F. and Langer, E.:1992, Nature 355, 434–37.
Swain, E.B., Engstrom, D.R., Brigham, M.E., Henning, T.A., Brezonik, P.L.:1992, Science 257, 784–87.
Vandal, G.M., Mason, RP. and Fitzgerald, W.F.: 1991, Water Air and Soil Poll. 56, 791–803.
Author information
Authors and Affiliations
Editor information
Editors and Affiliations
Rights and permissions
Copyright information
© 1995 Springer Science+Business Media Dordrecht
About this chapter
Cite this chapter
Pirrone, N., Glinsorn, G., Keeler, G.J. (1995). Ambient Levels and Dry Deposition Fluxes of Mercury to Lakes Huron, Erie and St. Clair. In: Porcella, D.B., Huckabee, J.W., Wheatley, B. (eds) Mercury as a Global Pollutant. Springer, Dordrecht. https://doi.org/10.1007/978-94-011-0153-0_20
Download citation
DOI: https://doi.org/10.1007/978-94-011-0153-0_20
Publisher Name: Springer, Dordrecht
Print ISBN: 978-94-010-4069-3
Online ISBN: 978-94-011-0153-0
eBook Packages: Springer Book Archive