Abstract
High resolution spectroscopy utilising a Bruker IFS 120 HR spectrometer was established at DLR during the end of the 80s. Since then extensive infrastructure has been built up regarding laboratory equipment as well as software tools. This includes cooleable/heatable single and multi-pass absorption cells (temperature range 190 — 1000 K, length 0.15 – 100 m), a flow system for generation of unstable species, capability for atmospheric absorption and emission measurements. For data reduction, among other utilities, the flexible line parameter retrieval code FitMAS (Fit Molecular Absorption Spectra) was developed. The work is focused on the generation of a quality-assured spectroscopic database of atmospheric constituents. Within nationally and internationally funded projects numerous species were investigated in the region from 10 to 3000 cm-1: CO, CO2, O3, ClO, Cl2O2, HOC1, ClONO2, BrO, OH, H2O, HO2, H2O2, NO, NO2, N2O5. Validated accuracies for line strengths of 1% and for pressure broadening parameters of 2% have been established.
Access this chapter
Tax calculation will be finalised at checkout
Purchases are for personal use only
Preview
Unable to display preview. Download preview PDF.
References
Birk, M., Hausamann, D., Wagner, G., and Johns, J.W. (1996) Determination of line strengths by Fourier transform spectroscopy, Appl. Opt. 35, 2971–2985.
Rothman, L. S., Rinsland, C.P., Goldman, A., Massie, S.T., Edwards, D.P., Flaud, J.-M., Perrin, A., Camy-Peyret, C., Dana, V., Mandin, J.Y., Schroeder, J., Mc Cann, A., Gamache, R.R., Watson, R.B., Yoshino, K., Chance, K.V., Jucks, K.W., Brown, L.R., Nemtchinov, V., and Varanasi, P. (1996) The HITRAN molecular spectroscopic data base and HAWKS (HITRAN atmospheric Work Station): 1996 edition, J. Quant. Spectrosc. Radiat. Transfer 60, 665–710.
Jacquinet-Husson, N, Arié, E., Ballard, J., Barbe, A., Bjoraker, G., Bonnet, B., Brown, L.R., Camy-Peyret, C., Champion, J.P., Chédin, A., Chursin, A., Clerbaux, C., Duxbury, G., Flaud, J.-M., Fourrié, N., Fayt, A., Graner, G., Gamache, R., Goldman, A., Golovko, VI., Guelachvili, G., Hartmann, J.M., Hilico, J.C., Hillman, J., Lefèvre, G., Lellouch, E., Mikhailenko, S.N., Naumenko, O.V., Nemtchinov, V., Newnham, D.A., Nikitin, A., Orphal, J., Perrin, A., Reuter, D.C., Rinsland, C.P., Rosenmann, L., Rothman, L.S., Scott, N.A., Selby, J., Sinitsa, L.N., Sirota, J.M., Smith, A.M., Smith, K.M., Tyuterev, Vl.G., Tipping, R.H., Urban, S., Varanasi, P., and Weber, M. (1999) The 1997 spectroscopic GEISA databank. J. Quant. Spectrosc. Radiat. Transfer 62, 205–254.
Pickett, H.M., Poynter, R.L., and Cohen, E.A. (1992) Submillimeter, Millimeter, and Microwave Spectral Line Catalogue, JPL Publication 80-23, Rev. 3, Jet Propulsion Laboratory, Pasadena, CA, USA.
Brown, L.R., Gunson, M.M., Toth, R.A., Irion, F.W., Rinsland, C.P., and Goldman, A. (1996) 1995 Atmospheric Trace Molecule Spectroscopy (ATMOS) Linelist, Appl. Opt. 35, 2828.
Chance, K.V., Jucks, K.W., Johnson, D.G., and Traub, W.A. (1994) The Smithsonian Astrophysical Observatory Database 1992, J. Quant. Spectrosc. Radiat. Transfer 52, 447–457.
Schreier, F., Schimpf, B., and Birk, M. (1993) FitMAS — Least-squares fitting of molecular line parameters from high resolution Fourier transform spectra (1993) In 13. Colloquium on High Resolution Molecular Spectroscopy, Riccione, Italy.
Dennis, J.E. and Schnabel, R.B. (1983) Numerical Methods for Unconstrained Optimization and Nonlinear Equations Prentice-Hall.
Varghese, P.L. and Hanson, R.K. (1984) Collisional narrowing effects on spectral line shapes measured at high resolution, Appl. Opt. 23, 2376–2385.
Schreier, F. (1992) The Voigt and Complex Error Function: A Comparison of Computational Methods, J. Quant. Spectrosc. Radiat. Transfer 48, 743–762.
Anderson, E., Bai, Z., Bischof, C., Demmel, J., Dongarra, J.J., Du Croz, J., Greenbaum, A., Hammarling, S., McKenney, A., Ostrouchov, S., and Sorensen, D. (1995) LAPACK Users’ Guide (2nd edition), SIAM.
Johns, J.W.C., Schreier, F., Schimpf, B., and Birk, M. (1994) Analysis of High-Resolution Fourier Transform Molecular Spectra, In The Future of Spectroscopy: From Astrophysics to Biology, Sainte-Adèle, Quebec, Canada.
Birk, M., Wagner, G., and Flaud, J.-M. (1994) Experimental Line strengths of Far-Infrared Pure Rotational Transitions of Ozone, J. Molec. Spectrosc. 163, 245–261.
Birk, M. and Wagner, G. (1997) Study on Spectroscopic Database for Millimeter and Submillimeter Wavelength, Final Report to ESTEC, Contract No. 11581/95/NL/CN, edited by Agnes Bauer, ESTEC, The Netherlands.
Birk, M. and Wagner, G. (1994) Vorrichtung zur Erzeugung eines definierten Ozon-Fremdgas-Gemisches und Verfahren zum Bereitstellen eines definierten Ozon-Fremdgas-Gemisches in einem geschlossenen Behälter, Deutsches Patent Nr. 43 42 624.7–52.
Birk, M., Wagner, G. (1997) Experimental line strengths of the CIO fundamental, J. Geophys. Res. 102, 19199–19206.
Wagner, G. and Birk, M. (2000) Erweiterung der spektroskopischen Datenbasis von C1O-NO2, C1OOC1, O3, N2O5 im Hinblick auf die Nutzung durch die MIPAS Instrumente, Ozone Research Program KKZ 07DLR05, German Ministery for Education and Research, Germany.
Birk, M., Wagner, G., Flaud, J.-M., and Hausamann, D. (1994) Line strengths in the v3-v2 Hot Band of Ozone, J. Mol. Spectrosc. 163, 262–275.
Wagner, G., Birk, M., Schreier, F., and Flaud, J.-M. (2000) Spectroscopic database of the three ozone fundamentals, subm. to JGR.
Oelhaf, H., Wetzel, G., Höpmer, M., Friedl-Vallon, F., Glatthor, N., Maucher, G., Stiller, G., Trieschmarm, O., von Clarmann, Th., Birk, M., and Wagner, G. (2000) Interconsistency checks of C1ONO2 retrievals from MIPAS-B spectra by using different bands and spectroscopic parameter sources, Proceedings IRS 2000, Petersburg, Russia.
Birk, M. and Wagner, G. (2000) A new spectroscopic database for chlorine nitrate, Poster, 6th HITRAN Conference, Cambridge, USA.
von Bargen, A., Birk, M., and Wagner, G. (1997) The HO2 Radical: The pure rotational FIR Spectrum Measured by FTS and the Molecular Constants, Poster Q1, 15th Colloquium on High Resolution Molecular Spectroscopy, Glasgow, UK, and Hochauflösende Fourier-Transform-Spektroskopie an den Radikalen Hydroperoxyl und Hydroxyl, PhD Thesis, University of Gießen, Germany.
Wagner, G. and Birk, M. (1997) Line Positions and Air Broadening of Pure Rotational Transitions of BrO From FTS Measurements, Poster B6, 15th Colloquium on High Resolution Molecular Spectroscopy, Glasgow, UK.
Flaud, J.-M., Birk, M., Wagner, G., Orphal, J., Klee, S., and Lafferty, W.J. (1998) The Far Infrared Spectrum of HOC1: Line Positions and Intensities, J. Mol. Spectrosc. 191, 362–367.
Schäfer, K. (ed.) (1998) Non-Intrusive Measurement of Aircraft Engine Exhaust Emissions (AEROJET), Final Technical Report, Commission of the European Communities Contract No. BRPR-CT96-0142.
Birk, M., Colmont, J.-M., Priem, D., Wagner, G., and Wlodarczak, G. (1997) N2-, O2-, and Air-Broadening Coefficients of the J=3→2 Line of CO and the J=342, 32→341, 33 Line of O3, Measured with Two Techniques: Tunable Microwave Source and Fourier-Transform Spectroscopy, Poster F4, 15th Colloquium on High Resolution Molecular Spectroscopy, Glasgow, UK.
Author information
Authors and Affiliations
Editor information
Editors and Affiliations
Rights and permissions
Copyright information
© 2001 Springer Science+Business Media Dordrecht
About this chapter
Cite this chapter
Birk, M., Hausamann, D., Schreier, F., Wagner, G. (2001). High Resolution Infrared Laboratory Spectroscopy of Atmospheric Constituents at DLR. In: Demaison, J., Sarka, K., Cohen, E.A. (eds) Spectroscopy from Space. NATO Science Series, vol 20. Springer, Dordrecht. https://doi.org/10.1007/978-94-010-0832-7_14
Download citation
DOI: https://doi.org/10.1007/978-94-010-0832-7_14
Publisher Name: Springer, Dordrecht
Print ISBN: 978-0-7923-6993-6
Online ISBN: 978-94-010-0832-7
eBook Packages: Springer Book Archive