Abstract
In their role as cloud condensation nuclei (CCN), aerosols are linked to, and often control, the hydrologic cycle and therefore major fluxes of the Earth’s radiation balance. Clouds, in tum, affect the levels and geographical distribution of aerosols by removing them in precipitation and by driving the general circulation. Aerosols are formed, evolve, and are eventually removed within the general circulation of the atmosphere. The characteristic time of many of the microphysical aerosol processes is days up to several weeks, hence longer than the residence time of the aerosol within a typical atmospheric compartment (e.g. the marine boundary layer, the free troposphere etc. …).To understand aerosol properties, one cannot confine the discussion to such compartments, but one needs to view aerosol microphysical phenomena within the context of atmospheric dynamics that connects those compartments. This paper attempts to present an integrated microphysical and dynamical picture of the global tropospher ic aerosol system. It does so by reviewing the microphysical processes and those elements of the general circulation that determine the size distribution and chemical composition of the aerosol
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References
Ammann M., Kalberer, M., Jost D.T., Tobler L., Rossler E., Piguet D., Gaggeler, H.W., and Baltensperger U., (1998) Heterogeneous production of nitrous acid on soot in polluted air masses, Nature, 395, 157–160.
Charlson R.J., Langner, J., Rodhe, H., Leovy, C.B., and Warren S.G., (1991) Perturbation of the nothern hemisphere radiative balance by backscattering from anthropogenic sulfate aerosols, Tellus, 43AB, 152–163.
Clarke, A.D., Porter, J.N., Valero, F.PJ., and P. Pilewskie, P., (1996) Vertical profiles, aerosol microphysics, and optical closure during ASTEX: measured and modeled column optical properties, Journal of Geophysical Research, 101, 4443–4453.
Clarke, A.D., Uehara, T., and Porter J.N., (1996) Lagrangian evolution of an aerosol column during the Atlantic Stratocumulus Transition Experiment, Journal of Geophysical Research, 101, 4351–4362.
Feichter J., and Crutzen, PJ., (1990) Parameterization of vertical tracer transport due to deep cumulus convection in a global transport model and evaluation with radon measurements, Tellus 42 B, 100–117.
Friedlander, S.K. (1977) Smoke, Dust and Haze: fundamentals of aerosol behaviour, John Wiley & Sons, New York.
Heimann, M., Monfray P., and Polian, G., (1990) Modeling the long-range transport of Rn-222 to subantarctic and antarctic areas, Tellus, 42B, 83–99. 1990.
Hoppel W.A., Frick, F.M., and Larson, R.E., (1986) Effect of nonprecipitating clouds on the aerosol size distribution in the marine boundary layer, Geophysical Research Letters, 13, 125–128.
Hoppel W.A., Frick G.M., Fitzgerald J.W., and Wattle B.J. (1994) A cloud chamber study of the effect that nonprecipitating water clouds have on the aerosol size distribution, Aerosol Science and Technol., 20, 1–30
Jacob D.J., Heikes, B.G., Fan, S.-M., Logan, J.A., Mauzerall, D.L., Bradshaw, J.D., Singh, H.B., Gregory, G.L., Talbot, R.W., Blake, D.E., and Sachse, G.W., (1996) Origin of ozone and NOx in the tropical troposphere: A photochemical analysis of aircraft observations over the South Atlantic basin, Journal of Geophysical Research, 101, 24235–24250.
Langner, J., and Rodhe, H., (1991) A global three-dimensional model of the tropospheric sulfur cycle, Journal of Atmospheric Chemistry, 13, 225–263.
Lelieveld, J., and Crutzen, PJ., (1994) Role of deep cloud convection in the ozone budget of the troposphere, Science, 264, 1759–1761.
Mason B. J. (1971) The physics of clouds, Clarendon Press, Oxford.
Murphy D.M., Thomson, D.S., and Mahoney M.I., (1998) In situ measurements of organics, meteoritic material, mercury, and other elements in aerosols at 5 to 19 kilometers, Science, 282, 1664–1669.
Newell R.E., Zhu, Y., Browell, E.V., Read, W.G., and Waters, J.W., (1996) Walker circulation and tropical upper tropospheric water vapor, Journal of Geophysical Research, 101, 1961–1974.
Newell R.E., V. Thouret, V., Cho, J.Y.N., Stoller, P., Marenco, A., and Smit, H.G., (1999) Ubiquity of quasihorizontal layers in the tropophere, Nature, 398, 316–319.
Novakov T., Hegg, D.A., and Hobbs, P.V., (1997) Airborne measurements of carbonaceous aerosols on the East Coast of the United States, Journal of Geophysical Research, 102, 30023–30030.
O’Dowd, C.D. and Smith, M.H., (1993) Physicochemical properties of aerosols over the Northeast Atlantic: Evidence for wind-speed-related submicron sea-salt aerosol production, Journal of Geophysical Research, 98, 1137–1149.
Pruppacher, H.R. and Klett, J.D., (1980) Microphysics of Clouds and Precipitation, D. Reidel Publishing Company
Putaud J.-P., Van Dingenen, R., Mangoni, M., Virkkula, A., Raes, F., Maring, H., Prospero, J., Swietlicki, E., Berg, O., Hillamo, R., and Makela, T., (2000) Chemical mass closure and assessment of the origin of the submicron aerosol in the marine boundary layer and the free troposphere at Tenerife during ACE-2, Tellus, 52B, 141–168.
Raes F., Wilson, J., and Van Dingenen, R., (1995) Aerosol’ dynamics and its implication for the global aerosol climatology, in “Aerosol Forcing of Climate”, (Eds. R.I. Charson and J. Heintzenberg), John Wiley & Sons.
Raes, F., (1995) Entrainment of free tropospheric aerosols as a regulating mechanism for cloud condensation nuclei in the remote marine boundary layer, Journal of Geophysical Research, 100, 2893–2903.
Rodhe H., (1983) Precipitation scavenging and tropospheric mixing, in Precipitation Scavenging, Dry Deposition, and Resuspension (Pruppacher et al., Eds), 719–728..
Schulz M., Balkanski, Y.I., Guelle, W., and Dulac F., (1998) Role of aerosol size distribution and source location in a three-dimensional simulation of a Saharan dust episode tested against satellite-derived optical thickness, Journal of Geophysical Research, 103, 10579–10592.
Vogt R., Crutzen, P.I., and Sander, R., (1996) A mechanism for halogen release from sea-salt aerosol in the remote marine boundary layer, Nature, 383, 327–330.
Wang P.-H., Rind, D., Trepte, C.R., Kent, G.S., Yue, G.K., and Skeens., K.M., (1998) An empirical model study of the tropospheric meridional circulation based on SAGE II observations, Journal of Geophysical Research, 103, 13801–13818.
Wu Z., R.N. Newell, Y. Zhu, Y., Anderson, B.E., Browell, E.V., Gregory, G.L., Sachse, G.W., Collins Jr., J.E., (1997) Atmospheric layers measured from the NASA DC-8 during PEM-West B and comparison with PEM-West A., Journal of Geophysical Research, 102, 28353–28365.
Zimmermann P.H. (1984) Ein dreidimensionales numerisches Transportmodell fur atmospharische Spurenstoffe, Thesis, Univeristy of Mainz, FRG.
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Raes, F. (2002). Formation and Cycling of Aerosols in the Global Troposphere. In: Barnes, I. (eds) Global Atmospheric Change and its Impact on Regional Air Quality. NATO Science Series, vol 16. Springer, Dordrecht. https://doi.org/10.1007/978-94-010-0082-6_3
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DOI: https://doi.org/10.1007/978-94-010-0082-6_3
Publisher Name: Springer, Dordrecht
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