Abstract
Passage from the quasiperiodic into the chaotic regime in a quantum system (a radiative active mode coupled to a laser field and in turn, intramolecularly coupled to radiatively inert background modes) is studied. Three main parameters are considered to be crucial in this passage: the radiative/intramolecular relative coupling strength, the effectiveness of the background as a bath, and the nature of the background detuning and coupling to the radiative pump mode.
This is a preview of subscription content, log in via an institution to check access.
Access this chapter
Tax calculation will be finalised at checkout
Purchases are for personal use only
Preview
Unable to display preview. Download preview PDF.
References
W. B. Miller, S. A. Safron and D. R. Herschbach, J. Chem. Phys. 56, 358 (1972).
P. J. Robinson and K. A. Holbrook, “Unimolecular Reactions,” Wiley, New York (1972).
P. A. Schultz, A. S. Sudbø, E. R. Grant, Y. R. Shen, and Y. T. Lee, J. Chem. Phys. 72, 4985 (1980).
D. W. Noid, M. L. Koszykowski and R. A. Marcus, in “Ann. Rev. of Phys. Chem.,” Vol. 32, eds. B. S. Rabinovitch, J. M. Schurr and H. L. Strauss (1981).
S. A. Rice, Adv. Chem. Phys. 24, 155 (1973).
K. S. J. Nordholm and S. A. Rice, J. Chem. Phys. 61, 203 (1974); ibid., 61, 768 (1974); ibid., 62, 157 (1975).
D. W. Noid and R. A. Marcus, J. Chem. Phys. 67, 559 (1977).
I. C. Percival, J. Phys. B. 6, L229 (1973).
M. Feingold and A. Peres, Physica B9, 433 (1983).
C. D. Cantrell, H.W. Galbraith, and J. R. Ackerhalt, in “Multiphoton Processes,” edited by J. H. Eberly and P. Lambropoulos, ( Wiley, New York, 1978 ), p. 331.
A. Nauts and R. E. Wyatt, Phys. Rev. Lett, 51, 2238 (1983).
A. Nauts and R. E. Wyatt, Phys. Rev. A, 30, 872 (1984).
C. J. Lanczos, J. Res. Nat. Bur. Stand., 45, 255 (1950).
C. C. Paige, J. Ins. Math. Appl., 10, 373 (1972).
R. Haydock, Comp. Phys. Commun., 20, 11 (1980).
R. Haydock, in “Solid State Physics,” H. Ehrenreich, F. Seitz, and D. Turnbull, eds. ( Academic, New York, 1980 ).
R. Haydock, in “Excitations in Disordered Systems” M. F. Thorpe, ed., ( Plenum, New York, 1981 ).
R. R. Whitehead, A. Watt, B. J. Cole and I. Morrison, in “Advances in Nuclear Physics,” Vol. 9, ed. M. Baranger and E. Vogt ( Plenum, New York, 1977 ), p. 123.
I. Schek and R. E. Wyatt, J. Chem. Phys. 83, 3028 (1985).
I. Schek and R. E. Wyatt, J. Chem. Phys. 83, 4650 (1985).
P. Lambin and J.-P. Gaspard, Phys. Rev. B., 26, 4356 (1982).
J.-P. Gaspard and P. Lambin, in “The Recursion Method and its Applications,” D. G. Pettifor and D. L. Wearie, eds. ( Springer, Berlin 1984 ), p. 72.
I. Schek and R. E. Wyatt, J. Chem. Phys., 84, 4497 (1986).
N. Moiseyev, I. Schek and R. E. Wyatt, Chem. Phys. Lett (submitted).
I. Schek and R. E. Wyatt, Chem. Phys. Lett. 129, 99 (1986).
R. Haydock, V. Heine and M. J. Kelley, J. Phys. C., 8, 2591 (1975).
I. Schek, N. Moiseyev and R. E. Wyatt, J. Chem. Phys. (submitted).
I. Schek and J. Jortner, J. Chem. Phys. 70, 3016 (1979).
B. Carmeli, I. Schek, A. Nitzan and J. Jortner, J. Chem. Phys. 72, 1928 (1980).
I. Schek and J. Jortner, Theor. Chem. Acta 69, 323 (1986).
Author information
Authors and Affiliations
Editor information
Editors and Affiliations
Rights and permissions
Copyright information
© 1987 D. Reidel Publishing Company
About this chapter
Cite this chapter
Schek, I., Wyatt, R.E. (1987). Effect of Diagonal and Off-Diagonal Disorder in the Multiphoton Excitation of an Active Mode Coupled to a Bath: Use of the Irreducible Recursive Residue Generation Method. In: Lefebvre, R., Mukamel, S. (eds) Stochasticity and Intramolecular Redistribution of Energy. NATO ASI Series, vol 200. Springer, Dordrecht. https://doi.org/10.1007/978-94-009-3837-3_7
Download citation
DOI: https://doi.org/10.1007/978-94-009-3837-3_7
Publisher Name: Springer, Dordrecht
Print ISBN: 978-94-010-8208-2
Online ISBN: 978-94-009-3837-3
eBook Packages: Springer Book Archive