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Spin-Orbit Effects in Chemical Reactions

  • Chapter
Selectivity in Chemical Reactions

Part of the book series: NATO ASI Series ((ASIC,volume 245))

Abstract

It is well known that forms of reagent energy, for example translational, vibrational, rotational excitation, can have drastically different effects on the rate of a chemical reaction. In this paper, we review investigations of spin-orbit effects in reactions involving atoms with both nonzero electronic orbital and spin angular momenta. There has been increasing interest in reactions of individual atomic spin-orbit levels because of the importance of nonadiabatic transitions in controlling the magnitude of spin-orbit dependences. Experimental methods for the study of reactions of individual reagent spin-orbit levels and for the detection of such states in atomic products will be briefly discussed. Observations for reactions of representative classes of atoms, including halogen atoms, electronically excited and ionized inert gases, and electronically excited alkaline earth and mercury atoms, are presented. The approaches taken for a theoretical modelling of such reactions are also outlined.

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  1. Department of Chemistry, The Johns Hopkins University, Baltimore, Maryland, 21218, USA

    Paul J. Dagdigian

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  1. Department of Chemistry, University of Manchester, Manchester, UK

    J. C. Whitehead

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Dagdigian, P.J. (1988). Spin-Orbit Effects in Chemical Reactions. In: Whitehead, J.C. (eds) Selectivity in Chemical Reactions. NATO ASI Series, vol 245. Springer, Dordrecht. https://doi.org/10.1007/978-94-009-3047-6_9

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