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Hydrocarbon Radical Cations in Condensed Phases

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Molecules in Physics, Chemistry, and Biology

Part of the book series: Topics in Molecular Organization and Engineering ((MOOE,volume 3))

Abstract

Radical cations are formed by one-electron loss from closed-shell molecules. They are generally very reactive, and special techniques are often required for their characterization. In this paper the emphasis is on studies in the condensed phase. Other authors have dealt with spectroscopy, structure and chemistry in the gas phase [1]. Radical cations were observed early as intermediates in γ-irradiated frozen matrices with optical absorption [2]. The early ESR work on relatively stable aromatic cations in solution aiming at elucidating their electronic structure has been summarized [3, 4]. Shida and coworkers made an important contribution by developing suitable techniques to generate and stabilize organic cations in rigid halogenated matrices at low temperature so that ESR measurements could be carried out. Their work has been reviewed [5].

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Authors and Affiliations

  1. Department of Physics, IFM, Linköping University, S-581 83, Linköping, Sweden

    A. Lund & M. Lindgren

  2. Department of Quantum Chemistry, Uppsala University, Box 518, S-751 20, Uppsala, Sweden

    S. Lunell

  3. Laboratoire de Chimie Physique, 11, rue Pierre et Marie Curie, 75005, Paris, France

    J. Maruani

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  1. Centre de Mécanique Ondulatoire Appliquée, Laboratoire de Chimie Physique, CNRS and University of Paris, France

    Jean Maruani

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© 1989 Kluwer Academic Publishers, Dordrecht, The Netherlands

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Lund, A., Lindgren, M., Lunell, S., Maruani, J. (1989). Hydrocarbon Radical Cations in Condensed Phases. In: Maruani, J. (eds) Molecules in Physics, Chemistry, and Biology. Topics in Molecular Organization and Engineering, vol 3. Springer, Dordrecht. https://doi.org/10.1007/978-94-009-2853-4_11

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