Abstract
Simulated and experimental broadened Mössbauer spectra are analyzed using several distribution functions. The resolution Hesse and Rübartsch data are reproduced in order to analyze the origin of the oscillations appearing in the recovered distribution function. The lined triangular distribution is used and some of its properties are described. The no implicit nth-nomial distribution function P(x) = (aCos (πx) + bSin (πx))n is introduced, complementing the Window and Hesse and Rübartasch no implicit distribution functions. This new no implicit distribution function gives similar results of those of Window’s method. In addition, the Window method has also been modified by inserting a smoothing factor λC. For 0 < λC < 1 a hyperfine distribution with low resolution may be obtained; for λC > 1, the opposite is obtained. The Levenberg-Marquardt algorithm is used to solve the involved Fredholm integral equation rather than the typical second order regularized algorithm. From the extracted hyperfine field distribution functions of the Mössbauer spectra of the amorphous and crystallized Fe70Cr2Si5B16 magnetic alloy the short range atomic order for the amorphous state of this alloy can be inferred.
Proceedings of the Thirteenth Latin American Conference on the Applications of the Mössbauer Effect, (LACAME 2012), Medellín, Colombia, 11–16 November 2012.
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Cabral-Prieto, A. (2013). Analysis of broadened Mössbauer spectra using simple mathematical functions. In: Meneses, C.A.B., Caetano, E.P., Torres, C.E.R., Pizarro, C., Alfonso, L.E.Z. (eds) LACAME 2012. Springer, Dordrecht. https://doi.org/10.1007/978-94-007-6482-8_2
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DOI: https://doi.org/10.1007/978-94-007-6482-8_2
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