Abstract
The main objectives of this study were to quantify the distribution of polycyclic aromatic hydrocarbons (PAHs) and polychlorinated biphenyls (PCBs) between air, water and sediments and to estimate the most important fluxes between these compartments by synthesizing all data in a semi-empirical mass balance of PAHs and PCBs for the Baltic Sea.
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References
Anonymous (1986) Water balance of the Baltic Sea. Helsinki Commission, Helsinki
Axelman J, Bandh C, Broman D, Carman R, Jonsson P, Larsson H, Linder H, Näf C, Pettersen H (1995) Time-trend analysis of PAH and PCB sediment fluxes in the northern Baltic proper using different dating methods. Mar Freshwater Res 46: 137–144
Axelman J, Broman D, Näf C (1997) Field measurements of the partitioning of PCBs in planktonic organisms–effects of growth, particle size and solvent-solute interactions. Environ Sci Technol 31: 665–669
Axelman J, Näf C, Broman D (2000) Vertical flux and particulate/water dynamics of polychlorinated biphenyls ( PCBs) in the open Baltic Sea. Ambio 29: 210–216
Baker JE, Eisenreich SJ (1990) Concentrations and fluxes of polycyclic aromatic hydrocarbons and polychlorinated biphenyls across the air-water interface of Lake Superior. Environ Sci Technol 24: 342–352
Baker JE, Eisenreich SJ, Eadie BJ (1991) Sediment trap fluxes and benthic recycling of organic carbon, polycyclic aromatic hydrocarbons, and polychlorobiphenyl congeners in Lake Superior. Environ Sci Technol 25: 500–509
Bandh C, Ishaq R, Broman D, Näf C, Rönnqvist-Nii Y, Zebühr Y (1994) Separation for subsequent analysis of PCBs, PCDD/Fs, and PAHs according to aromaticity and planarity using a two-dimensional HPLC-system. Environ Sci Technol 30: 214–219
Baron JA, Thibodeaux LJ, Reible DD, Templet P-H, Henry CB Jr (1990) Laboratory simulation of diffusion in contaminated sediments. Estuaries 13: 81–88
Bergström S, Carlsson B (1994) River runoff to the Baltic Sea: 1950–1990. Ambio 23: 280–287
Bidleman TF (1984) Estimation of vapor pressures nonpolar organic compounds by capillary gas chromatography. Anal Chem 56: 2490–2496
Bidleman TF (1988) Atmospheric processes. Environ Sci Technol 22: 361–367
Bignert A, Göthberg A, Jensen S, Litzén K, Odsjö T, Olsson M, Reutergsrdh L (1993) The need for adequate biological sampling in ecotoxicological investigations: a retrospective study of twenty years’ pollution monitoring. Sci Total Environ 128: 121–139
Blomqvist S, Larsson U (1994) Detrital bedrock elements as tracers of settling resuspended particulate matter in a coastal area of the Baltic Sea. Limnol Oceanogr 39: 880–896
Booij K, Achterberg EP, Sundby B (1992) Release rates of chlorinated hydrocarbons from contaminated sediments. Neth J Sea Res 29: 297–310
Broman D, Näf C, Lundbergh I, Zebühr Y (1990a) An in-situ on the distribution, biotransformation and flux of polycyclic aromatic hydrocarbons (PAHs) in an aquatic food chain (seston-Mytilus edulis L.-Somateria mollissima L.) from the Baltic: an ecotoxicological perspective. Environ Tox Chem 9: 429–442
Broman D, Kugelberg J, Näf C (1990b) Two hydrodynamically stable self-suspended buoyant sediment traps. Estuar Coast Shelf Sci 30: 429–436
Broman D, Näf C, Zebühr Y (1991a) Long term high-and low-volume air sampling of polychlorinated dibenzo-p-dioxins and dibenzofurans and polycyclic aromatic hydrocarbons along a transect from urban to remote areas on the Swedish Baltic coast. Environ Sci Technol 25: 1841–1850
Broman D, Näf C, Rolff C, Zebühr Y (1991b) Occurrence and dynamics of polychlorinated dibenzo-p-dioxins and dibenzofurans and polycyclic aromatic hydrocarbons in the mixed surface layer of remote coastal and offshore waters of the Baltic. Environ Sci Technol 25: 1850–1864
Brunner S, Hornung E, Santi H, Wolff E, Piringer OG, Altschuh J, Brüggemann R (1990) Henry’s law constants for polychlorinated biphenyls: experimental determination and structure-property relationships. Environ Sci Technol 24: 1751–1754
Chen H-W (1993) Fluxes of organic pollutants from the sediments in the Boston Harbour. Massachusetts Institute of Technology, Boston
Chin Y-P, McNichol AP, Gschwend P (1991) Quantification and characterization of pore-water organic colloids. In: Baker RA (ed) Organic substances in sediments and water. Lewis, Chelsea, MI
De Bruijn J, Busser F, Seinen W, Hermens J (1989) Determination of octanol/water partition coefficients for hydrophobic organic chemicals with the “slow-stirring” method. Environ Tox Chem 8: 499–512
Dickhut RM, Gustafson KE (1995) Atmospheric washout of polycyclic aromatic hydrocarbons in the southern Chesapeake Bay region. Environ Sci Technol 29: 1518–1525
Eisenreich SJ (1987) The chemical limnology of nonpolar organic contaminants: polychlorinated biphenyls in Lake Superior. In: Hites RA (ed) Source and fates of aquatic pollutants. American Chemical Society, Washington, DC
Eisenreich SJ, Looney BB, Thornton JD (1981) Airborne organic contaminants in the Great Lakes ecosystem. Environ Sci Technol 15: 30–38
Elmgren R (1984) Trophic dynamics in the enclosed, brackish Baltic Sea. Rapp P-v Réun Cons Int Explor Mer 183: 152–163
Foreman WT, Bidleman TF (1985) Vapor pressure estimates of individual polychlorinated biphenyls and commercial fluids using gas chromatographic data. J Chromatogr 330: 203–216
Formica SJ, Baron JA, Thibodeaux LJ, Valsaraj KT (1988) PCB transport into lake sediments. Conceptual model and laboratory simulation. Environ Sci Technol 22: 1435–1440
Gustafsson O, Gschwend PM (1997) Soot as strong partition medium for polycyclic aromatic hydrocarbons in aquatic systems. In: Eganhouse R (ed) Molecular markers in environmental geochemistry. American Chemical Society, Washington, DC
Hawker DW, Connell DW (1988) Octanol-water partition coefficients of polychlorinated biphenyl congeners. Environ Sci Technol 22: 382–387
Hoff RM, Muir DCG, Grift NP (1992) Annual cycle of polychlorinated biphenyls and organohalogen pesticides in air in southern Ontario. 1. Air concentration data. Environ Sci Technol 26: 266–275
Hornbuckle KC, Sweet CW, Pearson RF, Swackhamer DH, Eisenreich SJ (1995) Assessing annual water-air fluxes of polychlorinated biphenyls in Lake Michigan. Environ Sci Technol 29: 869–877
Jonsson P (1992) Large-scale changes of contaminants in Baltic Sea sediments during the twentieth century. Doctoral Thesis, Uppsala University
Junge CE (1974) Residence time and variability of tropospheric trace gases. Tellus 26: 477–488
Junge CE (1977) Basic considerations about trace constituents in the atmosphere as related to the fate of global pollutants. In: Suffet IH (ed) Fate of pollutants in the air and water environments. Wiley-Interscience, New York, pp 7–25
Karickhoff SW (1981) Semi-empirical estimation of sorption of hydrophobic pollutants on natural sediments and soils. Chemosphere 10: 833–846
Kjeller L-O, Rappe C (1995) Time trends in levels, patterns, and profiles for polychlorinated dibenzo-p-dioxins, dibenzofurans, and biphenyls in a sediment core from the Baltic proper. Environ Sci Technol 29: 346–355
Karickhoff SW, Brown DS, Scott A (1979) Sorption of hydrophobic pollutants on natural water sediments. Water Res 13: 241–248
Leppänen J-M, Alenius P (1988) Cycling of organic matter during the vernal growth period in the open northern Baltic proper. I. Hydrography, currents and related factors. Finn Mar Res 255: 3–18
Mackay D (1989) Modeling the long-term behavior of a contaminant in a large lake. J Great Lakes Res 15: 183–297
Mackay D, Shiu WY, Ma KC (1991) Illustrated handbook of physical-chemical properties and environmental fate for organic chemicals, vols I-II. Lewis, Chelsea, MI
McGroddy SE, Farrington JW, Gschwend PM (1996) Comparison of the in-situ and desorption sediment-water partitioning of polycyclic aromatic hydrocarbons and polychlorinated biphenyls. Environ Sci Technol 30: 172–177
McVeety BD, Hites RA (1988) Atmospheric deposition of polycyclic aromatic hydrocarbons to water surfaces: a mass balance approach. Atmos Environ 22:511–536
National Academy of Science (1979) Polychlorinated biphenyls. National Academy of Science, Washington, DC
Neumann T, Christiansen C, Clasen S, Emeis K-C, Kunzendorf H (1997) Geochemical records of salt-water inflows into deep basins of the Baltic Sea. Cont Shelf Res 17: 95–115
Ott WR (1990) A physical explanation of the log normality of pollutant concentrations. J Air Waste Manage Assoc 40: 1378–1383
Panshin SY, Hites RA (1994) Atmospheric concentrations of polychlorinated biphenyls at Bermuda. Environ Sci Technol 28: 2001–2007
Pearlman RS, Yalkowsky SH, Banerjee S (1984) Water solubilities of polynuclear aromatic and heteroaromatic compounds. J Phys Chem Ref Data 13: 555–562
Rekker RF, De Kort NN (1979) The hydrophobic fragment constant; an extension to a 1000 point data set. Eur J Med Chem Chim Ther 14: 479–488
Schulz DE, Petrick G, Duinker JC (1989) Complete characterization of polychlorinated biphenyl congeners in commercial Aroclor and Clophen mixtures by multidimensional gas chromatography-electron capture detection. Environ Sci Technol 23: 852–859
Schulz-Bull DE, Petrick G, Kannan N, Duinker JC (1995) Distribution of individual chlorobiphenyls ( PCB) in solution and suspension in the Baltic Sea. Mar Chem 48: 245–270
Schwartzenbach RP, Gschwend PM, Imboden DM (1993) Environmental organic chemistry. Wiley Interscience, New York
Slinn WNG, Hasse L, Hicks BB, Hogan AW, Lal D, Liss PS, Munnich KO, Sehmel GA,Vittor O (1978) Some aspects of the transfer of atmospheric trace constituents past the air-sea interface. Atmos Environ 12: 2055–2087
Swackhamer DL, Skoglund RS (1993) Bioaccumulation of PCBs by algae: kinetics versus equilibrium. Environ Tox Chem 12: 831–838
ten Hulscher TEM, van der Velde LE, Bruggeman WA (1992) Temperature dependence of Henry’s law constants for selected chlorobenzenes, polychlorinated biphenyls and polycyclic aromatic hydrocarbons. Environ Tox Chem 11: 1595–1603
Ullman WJ, Aller RC (1982) Diffusion coefficients in nearshore marine sediments. Limnol Oceanogr 27: 552–556
Whitby KT (1978) The physical characteristics of sulfur aerosols. Atmos Environ 12: 135–159
Wu S, Gschwend PM (1986) Sorption kinetics of hydrophobic organic compounds to natural sediments and soils. Environ Sci Technol 20: 717–725
Zebühr Y, Näf C, Broman D, Lexén K, Colmsjö A, Östman C (1989) Sampling techniques and clean up procedures for some complex environmental samples with respect to PCDDs and PCDFs and other organic contaminants. Chemosphere 19: 34–44
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Axelman, J. et al. (2001). Dynamics and Distribution of Hydrophobic Organic Compounds in the Baltic Sea. In: Wulff, F.V., Rahm, L.A., Larsson, P. (eds) A Systems Analysis of the Baltic Sea. Ecological Studies, vol 148. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-662-04453-7_10
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DOI: https://doi.org/10.1007/978-3-662-04453-7_10
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