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Organic Molecular Aggregates pp 76–87Cite as

Ensemble Averaged Spin Pair Dynamics of Doublet and Triplet Molecules

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Part of the book series: Springer Series in Solid-State Sciences ((SSSOL,volume 49))

Summary

The dynamics of the spin transitions governing the magnetic field dependence of radical pair processes, triplet quenching by radicals and triplet — triplet annihilation in condensed media is considered. The spin dynamics are induced by the hyperfine interaction and by the zero field splitting and include the Zee— mann interaction with an external magnetic field. The theory presented takes the average over all nuclear spin orientations as well as over all histories of either nuclear spin realignments by exchange or rotational diffusion.

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References

  1. For a most recent review on magnetic field effects on doublet processes in chemistry and biology see K. Schulten, Advances in Solid State Physics, XXII, 61, J. Treusch (ed.), Vieweg, Braunschweig (1982)

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  2. K. Schulten, H. Staerk, A. Weller, H.-J. Werner and B. Nickel, Z. Phys. Chem. NF1Q1, 371 (1976); M.E. Michel-Beyer 1e, et al. Chem. Phys. 17, 139 (1976)

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  3. K. Schulten and P.G. Wolynes, J.Chem.Phys. 68, 3292 (1978); E.-W. Knapp and K. Schulten, J.Chem.Phys. 71 1878 (1979)

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  4. A. Weller, F. Nolting, and H. Staerk, Chem. Phys. Lett. 96, 24 (1983)

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  5. The major part of this Section will be found in K. Schulten, J. Chem. Phys. (in press)

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  6. L.R. Faulkner and A.J. Bard, J.Am.Chem.Soc. 91 6497 (1969)

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  7. J. Spichtig, H. Bulska, and H. Labhard, Chem.Phys. 15, 279 (1976); K. Lendi, P. Gerber, and H. Labhard, ibid. 18 449 (1976)

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Author information

Authors and Affiliations

  1. Physik-Department, Technische Universität München, D-8046, Garching, Fed. Rep. of Germany

    Klaus Schulten

Authors
  1. Klaus Schulten
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Editor information

Editors and Affiliations

  1. Abteilung für Theoretische Physik, Universität Ulm, D-7900, Ulm, Fed. Rep. of Germany

    Peter Reineker

  2. Institut für Theoretische Physik der Universität Stuttgart, Pfaffenwaldring 57, D-7000, Stuttgart 80, Fed. Rep. of Germany

    Hermann Haken

  3. Physikalisches Institut der Universität Stuttgart, Pfaffenwaldring 57, D-7000, Stuttgart 80, Fed. Rep. of Germany

    Hans Christoph Wolf

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© 1983 Springer-Verlag Berlin Heidelberg

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Schulten, K. (1983). Ensemble Averaged Spin Pair Dynamics of Doublet and Triplet Molecules. In: Reineker, P., Haken, H., Wolf, H.C. (eds) Organic Molecular Aggregates. Springer Series in Solid-State Sciences, vol 49. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-642-82141-7_8

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  • DOI: https://doi.org/10.1007/978-3-642-82141-7_8

  • Publisher Name: Springer, Berlin, Heidelberg

  • Print ISBN: 978-3-642-82143-1

  • Online ISBN: 978-3-642-82141-7

  • eBook Packages: Springer Book Archive

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