Abstract
A general theory of second order optical process is developed on the basis of the damping theory. It is clarified that the competitive behavior between the Raman scattering and luminescence depends not only on the relax-ation phenomena in the material system but also on the properties of excitation light and observation method. A general theory of time-resolved emission spectrum is formulated on the basis of microscopic treatment of the photo-detection process. The time-dependent behaviors of the Raman scattering and luminescence under pulsed excitation are clarified. As an illustration light scattering from a localized electron-phonon system is studied both on the stationary and time-resolved emission spectra. Then the theory is applied to the analysis of the recent experiments on the emission spectra from excitonic molecules in CuCl crystal and qualitatively satisfactory agreement between the theory and experiments is obtained. Finally a new formulation of resonant Raman scattering is presented in terms of the Keldysh-Schwinger formalism. This is a complete generalization of our stochastic theory to include the frequency and wavevector dependence of the relaxation phenomena.
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Takagahara, T. (1980). Resonant Raman Scattering and Luminescence. In: Kubo, R., Hanamura, E. (eds) Relaxation of Elementary Excitations. Springer Series in Solid-State Sciences, vol 18. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-642-81482-2_4
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DOI: https://doi.org/10.1007/978-3-642-81482-2_4
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