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Optimal Sequences for Chirped-Pulse-Stimulated Vibrational Motion

  • E. M. Hiller
  • J. A. Cina
Conference paper
Part of the Springer Series in Chemical Physics book series (CHEMICAL, volume 62)

Abstract

Calculations on impulsive Raman scattering with sequences of preresonant pulses show that variable chirp rate and center frequency can enhance vibrational amplification and decrease electronic absorption.

Keywords

Center Frequency Vibrational Energy Rabi Frequency Vibrational Motion Pulse Chirp 
These keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.

References

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    T.J. Smith and J.A. Cina, J. Chem. Phys. 104, 1272 (1996).CrossRefADSGoogle Scholar
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    For a survey of impulsive stimulated Raman scattering, see: L. Dhar, J.A. Rogers, and K.A. Nelson, Chem. Rev. 94, 157 (1994).CrossRefGoogle Scholar
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    See also: S. Ruhman and R. Kosloff, J. Opt. Soc. Am. B 7, 1748 (1990).ADSGoogle Scholar
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    Recent applications ultrashort chirped pulses include: M. Sterling, R. Zadoyan, and V.A. Apkarian, J. Chem. Phys. 104, 6497 (1996)CrossRefADSGoogle Scholar
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    C.J. Bardeen, Q. Wang, and C.V. Shank, Phys. Rev. Lett. 75, 3410 (1995)CrossRefADSGoogle Scholar
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    B. Kohler, V.V. Yakovlev, J. Chi, J.L. Krause, M. Messina, K.R. Wilson, N. Schwentner, R.M. Whitnell, and Y. Yan, Phys. Rev. Lett. 74, 3360 (1995).CrossRefADSGoogle Scholar

Copyright information

© Springer-Verlag Berlin Heidelberg 1996

Authors and Affiliations

  • E. M. Hiller
    • 1
  • J. A. Cina
    • 2
  1. 1.James Franck InstituteThe University of ChicagoChicagoUSA
  2. 2.Department of ChemistryUniversity of OregonEugeneUSA

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