Preparation and Interrogation of Vibronic Coherences in Condensed Media: I2 Isolated in Condensed Rare Gases
Time domain measurements using chirped pulses, and frequency domain spectroscopy of I2 isolated in rare gas solids is exploited to connect experimental observables to molecular dynamics through semiclassical simulations.
KeywordsVibrational Relaxation Chirp Pulse Time Domain Measurement Classical Coherence Stationary Phase Approximation
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