Abstract
Femtosecond pump-probe measurements at room temperature reveal coherent nuclear motion and ultrafast depolarization within the dimeric subunit of a bacterial light-harvesting complex, and spectral evolution within the re-assembled aggregate. The results establish a sub-50 fs timescale for dephasing between dimer exciton levels and support a stochastic hopping model for energy transfer within antenna complexes.
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References
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© 1996 Springer-Verlag Berlin Heidelberg
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Kumble, R., Palese, S., Visschers, R.W., Dutton, P.L., Hochstrasser, R.M. (1996). Femtosecond Dynamics Within the B820 Dimeric Subunit from the Core Antenna Complex of Rs. rubrum . In: Barbara, P.F., Fujimoto, J.G., Knox, W.H., Zinth, W. (eds) Ultrafast Phenomena X. Springer Series in Chemical Physics, vol 62. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-642-80314-7_139
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DOI: https://doi.org/10.1007/978-3-642-80314-7_139
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