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Time domain separation of the nuclear and electronic contributions to the third order nonlinearity in glasses

  • S. Montant
  • A. Le Calvez
  • E. Freysz
  • A. Ducasse
  • M. Couzi
Conference paper
Part of the Springer Series in Chemical Physics book series (CHEMICAL, volume 63)

Abstract

The electronic and nuclear contributions to the third order nonlinearity of glasses are separated using 100 fs pulses with a time-resolved heterodyne optical Kerr effect technique. The time evolution of the nuclear contribution is in very good agreement with results deduced from the Raman spectra. A direct estimate of the relative strengths of electronic and nuclear contributions is made. The ratio between the two response function is ∼5/1 in Tellurium oxide glass sample. The validity of our method to separate these two contributions has been confirmed in different glasses.

Keywords

Raman Spectrum Order Nonlinearity Boson Peak Nuclear Contribution Order Susceptibility 
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References

  1. 1.
    R. Heflwarth, J. Cherlow, T.T. Tang, Phys. Rev. B 11, 964 (1975).ADSCrossRefGoogle Scholar
  2. 2.
    I. Thomaseau, J. Etchepare, G. Grillon, A. Migus, Opt. Letters. 10, 223 (1985).ADSCrossRefGoogle Scholar
  3. 3.
    I. Kang, T. D. Krauss, F. W. Wise, B. G. Aitken, N. F. Borrelli, JOSA B 12, 2053 (1995).CrossRefGoogle Scholar
  4. 4.
    I. Kang, T. D. Krauss, F. W. Wise, B. G. Aitken, N. F. Borrelli, Phys. Rev. B 54, 641 (1996).Google Scholar
  5. 5.
    A Le Calvez et al., Chem. Phys. Letters, 258, 620 (1996).ADSCrossRefGoogle Scholar

Copyright information

© Springer-Verlag Berlin Heidelberg 1998

Authors and Affiliations

  • S. Montant
    • 1
  • A. Le Calvez
    • 1
  • E. Freysz
    • 1
  • A. Ducasse
    • 1
  • M. Couzi
    • 2
  1. 1.Centre de Physique Moleculaire Optique et HertzienneUniversite Bordeaux ITalence CedexFrance
  2. 2.Laboratoire de Physico-Chimie Moleculaire, UMR 5803Universite Bordeaux ITalence CedexFrance

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