Abstract
In this chapter the reader will find a detailed analysis of the behavior of populations and the real and imaginary parts of molecular nonlinear resonant polarization. There is a discussion of the relation between contributions produced by the difference in the values of polarizability of resonant levels, the saturation of populations, the dynamic Stark effect, into nonlinear dielectric polarizability, with special attention paid to single- and two-photon resonances.
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Butylkin, V.S., Khronopulo, Y.G., Kaplan, A.E., Yakubovich, E.I. (1989). The Molecular Response to the Resonant Effects of Quasimonochromatic Fields. In: Resonant Nonlinear Interactions of Light with Matter. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-642-68891-1_2
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