Abstract
Results of picosecond photon echo and pump-probe experiments on pentacene in naphthalene and p-terphenyl are reported. The photon echoes are detected by optical mixing of the echo with a synchronized probe pulse in an ADP crystal. From the temperature dependence of the photon echo it is concluded that the pure electronic transition of pentacene in both naphthalene and p-terphenyl is relaxed by phonon scattering off a resonant phonon. Time-resolved absorption measurements on some selected excited state vibrations of pentacene in naphthalene show that drastic differences exist in vibrational relaxation times.
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References
S.L. Shapiro (ed): Ultrashort Light Pulses, Topics in Appl.Phys., Vol.18 (Springer, Berlin, Heidelberg, New York 1977)
A. Laubereau, G. Wochner, W. Kaiser: Phys. Rev. A13, 2212 (1976)
D.M. Burland, D.E. Cooper, M.D. Fayer, C.R. Gochanour: Chem. Phys. Lett. 52, 279 (1977)
S.L. Robinette, G.J. Small: J. Chem. Phys. 65, 837 (1976)
W.H. Hesslink, D.A. Wiersma: Chem. Phys. Lett. June 1 issue (1978): Picosecond Phenomena meeting, Hilton Head, South Carolina, May 1978.
N.A. Kurnit, I.D. Abella, S.R. Hartmann: Phys. Rev. Lett. 13, 567 (1964),
N.A. Kurnit, I.D. Abella, S.R. Hartmann Phys. Rev. 141, 391 (1966)
T.J. Aartsma, D.A. Wiersma: Opt. Commun. 18, 201 (1976),
T.J. Aartsma, D.A. Wiersma Chem. Phys. Lett. 42, 520 (1976)
T.E. Orlowski, K.E. Jones, A.H. Zewail: Chem. Phys. Lett. 54, 197 (1978)
H. de Vries, D.A. Wiersma: J. Chem. Phys. to be published
A. Brillante, D.P. Craig: J. Chem. Soc., Faraday Trans 2, 71, 1457 (1975)
H.P. Weber, H.G. Danielmeyer: Phys. Rev. A2, 2074 (1970)
N. Takeuchi, IEEE J.QE-11 236, (1975)
S. Voelker, R.M. Macfarlane, J.H. v.d. Waals: Chem. Phys. Lett. 53, 8 (1978)
T.J. Aartsma, J.B.W. Morsink, D.A. Wiersma: Chem. Phys. Lett. 47, 425 (1977)
M.A. Krivoglaz: Sov. Phys. Jetp. 21, 204 (1965)
C.B. Harris: J. Chem. Phys. 12, 5607 (1977)
R. Kubo: Adv. Chem. Phys. XV, 101 (1969) and References therein
P. de Bree, D.A. Wiersma: to be published
A.G. Redfield: Adv. Magn. Res. vol I (ed. J.S. Waugh, Acad.Press, 1965)
D. von der Linde, A. Laubereau, W. Kaiser: Phys. Rev. Lett. 26, 954 (1971)
E.P. Ippen, C.V. Shank, A. Bergman: Chem. Phys. Lett 38, 611 (1976)
C.V. Shank, D.H. Auston: Phys. Rev. Lett 34, 479 (1975)
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Hesselink, W.H., Wiersma, D.A. (1978). Picosecond (Coherent) Transients in Molecular Mixed Crystals. In: Shank, C.V., Ippen, E.P., Shapiro, S.L. (eds) Picosecond Phenomena. Springer Series in Chemical Physics, vol 4. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-642-67099-2_37
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DOI: https://doi.org/10.1007/978-3-642-67099-2_37
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