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Dynamics of Gas-Surface Interactions pp 101–129Cite as

Hydrogen Dissociation on Stepped Pt Surfaces

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Part of the book series: Springer Series in Surface Sciences ((SSSUR,volume 50))

Abstract

A short historical perspective outlines how interest in a physisorbed molecular state of hydrogen led to studies of a chemisorbed molecular state. Increasing evidence for such a state sparked interest in the dissociation dynamics at lower coordinated sites on surfaces, which also serve as models for active sites on particles used in industrial catalysis. As the Pt[n(111) ×(100)] has become the most intensely studied model system, we discuss results of molecular beam and theoretical dynamical studies in detail. We close by reviewing the most recent model for separating step and terrace reactivity and provide an outlook for this field of research.

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Authors and Affiliations

  1. SINTEF Materials and Chemistry, 124, Blindern, N-0314, Oslo, Norway

    Roar A. Olsen

  2. Leiden Institute of Chemistry, Leiden University, 9502, 2300 RA, Leiden, The Netherlands

    Ludo B. F. Juurlink

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  1. Roar A. Olsen
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  1. , Centro de Física de Materiales, CSIC-UPV/EHU, Paseo Manuel de Lardizabal 5, Donostia-San Sebastián, 20018, Spain

    Ricardo Díez Muiño

  2. , Instituto de Física Rosario, CONICET-UNR, 27 de Febrero 210, Rosario, 2000, Argentina

    Heriberto Fabio Busnengo

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Olsen, R.A., Juurlink, L.B.F. (2013). Hydrogen Dissociation on Stepped Pt Surfaces. In: Díez Muiño, R., Busnengo, H. (eds) Dynamics of Gas-Surface Interactions. Springer Series in Surface Sciences, vol 50. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-642-32955-5_5

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