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Real-Time Monitoring of Structural Evolution in Cis-Stilbene Photoisomerization Time-Domain Raman Spectroscopy

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Ultrafast Phenomena XVI

Part of the book series: Springer Series in Chemical Physics ((CHEMICAL,volume 92))

Abstract

We studied the vibrational structure of reactive S1 cis-stilbene through wavepacket motions generated impulsively at various delay-times. They showed gradual frequency downshift, demonstrating highly anharmonic nature of the excited-state potential and structural evolution with photoisomerization

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References

  1. K. Ishii, S. Takeuchi, and T. Tahara, “A 40-fs time-resolved absorption study on cis-stilbene in solution: observation of wavepacket motion on the reactive excited state”, Chem. Phys. Lett. 398, 400, 2004.

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  2. S. Fujiyoshi, S. Takeuchi, and T. Tahara, “Time-resolved impulsive stimulated Raman scattering from excited-state polyatomic molecules in solution”, J. Phys. Chem. A 107, 494, 2003.

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Authors and Affiliations

  1. Molecular Spectroscopy Laboratory, RIKEN 2-1, Hirosawa, 351-0198, Wako, Japan

    Satoshi Takeuchi & Tahei Tahara

  2. Department of Physical Chemistry, Hebrew University, Jerusalem, 91904, Israel

    Sanford Ruhman

  3. School of Engineering, The University of Tokyo, Tokyo, 113-8656, Japan

    Takao Tsuneda

  4. National Institute of Advanced Industrial Science and Technology, 305-8568, Tsukuba, Japan

    Mahito Chiba

  5. Graduate School of Science, Hokkaido University, Sapporo, 060-0810, Japan

    Tetsuya Taketsugu

Authors
  1. Satoshi Takeuchi
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  2. Sanford Ruhman
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  3. Takao Tsuneda
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  4. Mahito Chiba
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  5. Tetsuya Taketsugu
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  6. Tahei Tahara
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Corresponding author

Correspondence to Satoshi Takeuchi .

Editor information

Editors and Affiliations

  1. National Research Council Canada, Sussex Drive 100, Ottawa, K1A 0R6, Canada

    Paul Corkum

  2. Dipto. Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, Milano, 20133, Italy

    Sandro Silvestri

  3. Technology (MIT), Massachusetts Institute of, Massachusetts Ave. 77, Cambridge, 02139, USA

    Keith A. Nelson

  4. Sektion Physik, Univ. München, Oettingenstr. 67, München, 80538, Germany

    Eberhard Riedle

  5. Lawrence Berkeley National Laboratory, University of California, Cyclotron Road 1, Berkeley, 94720, USA

    Robert W. Schoenlein

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© 2009 Springer-Verlag Berlin Heidelberg

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Takeuchi, S., Ruhman, S., Tsuneda, T., Chiba, M., Taketsugu, T., Tahara, T. (2009). Real-Time Monitoring of Structural Evolution in Cis-Stilbene Photoisomerization Time-Domain Raman Spectroscopy. In: Corkum, P., Silvestri, S., Nelson, K., Riedle, E., Schoenlein, R. (eds) Ultrafast Phenomena XVI. Springer Series in Chemical Physics, vol 92. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-540-95946-5_99

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  • DOI: https://doi.org/10.1007/978-3-540-95946-5_99

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  • Publisher Name: Springer, Berlin, Heidelberg

  • Print ISBN: 978-3-540-95945-8

  • Online ISBN: 978-3-540-95946-5

  • eBook Packages: Physics and AstronomyPhysics and Astronomy (R0)

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