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Ultrafast Phenomena XVI pp 63–65Cite as

Probing Dynamics in Polyatomic Molecules Using High Harmonic Generation: the Role of Ionization Continua

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Part of the book series: Springer Series in Chemical Physics ((CHEMICAL,volume 92))

Abstract

We show that to understand harmonic generation from molecules undergoing a large change in configuration, multiple ionization continua must be considered. After exciting large amplitude vibrations in an N2O4 dimer, bright bursts of harmonics are emitted at the outer turning point of the vibration.

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References

  • J. Itatani, D. Zeidler, J. Levesque, D. M. Villeneuve, and P. B. Corkum, Phys. Rev. Lett., Vol. 94, 123902, 2005.

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  • N. L. Wagner, A. Wuest, I. P. Christov, T. Popmintchev, X. B. Zhou, M. M. Murnane, H. C. Kapteyn, Proc. Natl. Acad. Sci., Vol. 103, 13279, 2006.

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Author information

Authors and Affiliations

  1. JILA and Dept. of Physics, University of Colorado, Boulder, CO, 80309, USA

    Wen Li, Xibin Zhou, Robynne Lock, Margaret Murnane & Henry Kapteyn

  2. Steacie Institute of Molecular Sciences, National Research Council, Ottawa, ON, K1A0R6, Canada

    Serguei Patchkovskii, Olga Smirnova & Albert Stolow

Authors
  1. Wen Li
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  2. Xibin Zhou
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  3. Robynne Lock
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  4. Serguei Patchkovskii
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  5. Olga Smirnova
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  6. Albert Stolow
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  7. Margaret Murnane
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  8. Henry Kapteyn
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Corresponding author

Correspondence to Wen Li .

Editor information

Editors and Affiliations

  1. National Research Council Canada, Sussex Drive 100, Ottawa, K1A 0R6, Canada

    Paul Corkum

  2. Dipto. Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, Milano, 20133, Italy

    Sandro Silvestri

  3. Technology (MIT), Massachusetts Institute of, Massachusetts Ave. 77, Cambridge, 02139, USA

    Keith A. Nelson

  4. Sektion Physik, Univ. München, Oettingenstr. 67, München, 80538, Germany

    Eberhard Riedle

  5. Lawrence Berkeley National Laboratory, University of California, Cyclotron Road 1, Berkeley, 94720, USA

    Robert W. Schoenlein

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© 2009 Springer-Verlag Berlin Heidelberg

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Li, W. et al. (2009). Probing Dynamics in Polyatomic Molecules Using High Harmonic Generation: the Role of Ionization Continua. In: Corkum, P., Silvestri, S., Nelson, K., Riedle, E., Schoenlein, R. (eds) Ultrafast Phenomena XVI. Springer Series in Chemical Physics, vol 92. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-540-95946-5_21

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  • DOI: https://doi.org/10.1007/978-3-540-95946-5_21

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  • Publisher Name: Springer, Berlin, Heidelberg

  • Print ISBN: 978-3-540-95945-8

  • Online ISBN: 978-3-540-95946-5

  • eBook Packages: Physics and AstronomyPhysics and Astronomy (R0)

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