Abstract
Because of its sensitivity to point defects atomically close to probe nuclei, it is reasonable to expect that perturbed angular correlation (PAC) spectroscopy has the potential to assist in the identification of diffusion mechanisms. It is of interest to characterize under what conditions diffusing defects are visible and how the defects affect relaxation in PAC spectra. This was investigated using a stochastic model to simulate PAC spectra for the special case of non-impurity PAC probes diffusing via a simple vacancy mechanism on the Cu-sublattice in Cu3Au-structured compounds.
This work is funded in part by NSF grant DMR 06-06006 (Metals Program) and by KY EPSCoR grant RSF 012-03.
Access this chapter
Tax calculation will be finalised at checkout
Purchases are for personal use only
Preview
Unable to display preview. Download preview PDF.
References
Zacate, M.O., Favrot, A., Collins, G.S.: Atom movement in In3La studied via nuclear quadrupole relaxation. Phys. Rev. Lett. 92, 225901 (2004); Erratum. Phys. Rev. Lett. 93, 049903 (2004)
Winkler, H., Gerdau, E.: γγ-angular correlations perturbed by stochastic fluctuating fields. Z. Phys. 262, 363–376 (1973)
Philibert, J.: Atom Movements: Diffusion and Transport in Solids. Les Éditions de Physique, Les UIis (1991)
Evenson, W.E., Gardner, J.A., Wang, R., Su, H.-T., McKale, A.G.: PAC analysis of defect motion by Blume’s Stochastic Model for I=5/2 electric quadrupole interactions. Hyperfine Interact. 62, 283–300 (1990)
Author information
Authors and Affiliations
Corresponding author
Editor information
Editors and Affiliations
Rights and permissions
Copyright information
© 2008 Springer Science + Business Media B.V.
About this paper
Cite this paper
Muhammed, H., Zacate, M.O., Evenson, W.E. (2008). Simulation of PAC spectra for spin 5/2 probes diffusing via a simple vacancy mechanism in Cu3Au-structured intermetallic compounds. In: Pasquevich, A., RenterÃa, M., Saitovitch, E.B., Petrilli, H. (eds) HFI/NQI 2007. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-540-85320-6_27
Download citation
DOI: https://doi.org/10.1007/978-3-540-85320-6_27
Published:
Publisher Name: Springer, Berlin, Heidelberg
Print ISBN: 978-3-540-85319-0
Online ISBN: 978-3-540-85320-6
eBook Packages: Physics and AstronomyPhysics and Astronomy (R0)