Skip to main content

Molecules in Strong Laser Fields

  • Chapter
  • 1269 Accesses

Part of the book series: Springer Series on Atomic, Optical, and Plasma Physics ((SSAOPP,volume 48))

Molecules, compared to atoms, have additional degrees of freedom. Not only do the electrons move around the nuclei, but also the nuclei move relative to each other. This allows for a multitude of new phenomena, already without the action of external fields.

By coupling an external electric field to the molecular dynamics, such diverse topics as femtosecond spectroscopy, control of molecular dynamics, and the realization of quantum logic operations emerge. Before entering that wide field, some basics of molecular theory will be repeated by discussing the simplest molecule, the hydrogen molecular ion.

This is a preview of subscription content, log in via an institution.

Buying options

Chapter
USD   29.95
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
eBook
USD   159.00
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
Softcover Book
USD   209.00
Price excludes VAT (USA)
  • Compact, lightweight edition
  • Dispatched in 3 to 5 business days
  • Free shipping worldwide - see info

Tax calculation will be finalised at checkout

Purchases are for personal use only

Learn about institutional subscriptions

Preview

Unable to display preview. Download preview PDF.

Unable to display preview. Download preview PDF.

References

  1. J.C. Slater, Quantum Mechanics of Molecules and Solids, vol. 1 (McGraw-Hill, New York, 1963)

    Google Scholar 

  2. B.H. Bransden, C.J. Joachain, Physics of Atoms and Molecules, 2nd edn. (Pearson Education, Harlow, 2003)

    Google Scholar 

  3. A. Szabo, N.S. Ostlund, Modern Quantum Chemistry (Dover, Mineola, 1996)

    Google Scholar 

  4. B.N. Finkelstein, G.E. Horowitz, Z. Phys. 48, 118 (1928)

    Article  ADS  Google Scholar 

  5. P.M. Morse, Phys. Rev. 34, 57 (1929)

    Article  ADS  MATH  Google Scholar 

  6. D. ter Haar, Phys. Rev. 70, 222 (1946)

    Article  ADS  MathSciNet  Google Scholar 

  7. G. Herzberg, Molecular Spectra and Molecular Structure: I. Spectra of Diatomic Molecules, 2nd edn. (Krieger, Malabar, 1989)

    Google Scholar 

  8. A. Giusti-Suzor, F.H. Mies, L.F. DiMauro, E. Charron, B. Yang, J. Phys. B 28, 309 (1995)

    Article  ADS  Google Scholar 

  9. S. Chelkowski, T. Zuo, A.D. Bandrauk, Phys. Rev. A 46, R5342 (1992)

    Article  ADS  Google Scholar 

  10. S. Chelkowski, T. Zuo, O. Atabek, A.D. Bandrauk, Phys. Rev. A 52, 2977 (1995)

    Article  ADS  Google Scholar 

  11. M. Uhlmann, T. Kunert, R. Schmidt, Phys. Rev. A 72, 045402 (2005)

    Article  ADS  Google Scholar 

  12. J.D. Jackson, Klassische Elektrodynamik (Walter de Gruyter, Berlin, 1983)

    Google Scholar 

  13. T. Zuo, A.D. Bandrauk, Phys. Rev. A 52, R2511 (1995)

    Article  ADS  Google Scholar 

  14. A.D. Bandrauk, in Molecules in Laser Fields, ed. by A.D. Bandrauk (Dekker, New York, 1994), Chap. 1, pp. 1–69

    Google Scholar 

  15. B. Feuerstein, U. Thumm, Phys. Rev. A 67, 043405 (2003)

    Article  ADS  Google Scholar 

  16. A. Palacios, H. Bachau, F. Martin, Phys. Rev. Lett. 96, 143001 (2006)

    Article  ADS  Google Scholar 

  17. D.J. Tannor, Introduction to Quantum Mechanics: A Time-dependent Perspective (University Science Books, Sausalito, 2007)

    Google Scholar 

  18. R. Schinke, Photodissociation Dynamics (Cambridge University Press, Cambridge, 1993)

    Book  Google Scholar 

  19. R.B. Walker, R.K. Preston, J. Chem. Phys. 67, 2017 (1977)

    Article  ADS  MathSciNet  Google Scholar 

  20. R. Mecke, Z. Elektrochemie 54, 38 (1950)

    Google Scholar 

  21. M.J. Davis, R.E. Wyatt, Chem. Phys. Lett. 86, 235 (1982)

    Article  ADS  Google Scholar 

  22. W. Jakubetz, J. Manz, V. Mohan, J. Chem. Phys. 90, 3683 (1989)

    Article  ADS  Google Scholar 

  23. S. Chelkowski, A.D. Bandrauk, P.B. Corkum, Phys. Rev. Lett. 65, 2355 (1990)

    Article  ADS  Google Scholar 

  24. S. Krempl, T. Eisenhammer, A. Hübler, G. Mayer-Kress, P.W. Milonni, Phys. Rev. Lett. 69, 430 (1992)

    Article  ADS  Google Scholar 

  25. S. Shi, H. Rabitz, J. Chem. Phys. 92, 364 (1990)

    Article  ADS  Google Scholar 

  26. B.M. Garraway, K.A. Suominen, Rep. Prog. Phys. 58, 365 (1995)

    Article  ADS  Google Scholar 

  27. J.C. Tully, J. Chem. Phys. 93, 1061 (1990)

    Article  ADS  Google Scholar 

  28. H.D. Meyer, W.H. Miller, J. Chem. Phys. 72, 2272 (1980)

    Article  ADS  Google Scholar 

  29. G. Stock, M. Thoss, Phys. Rev. Lett. 78, 578 (1997)

    Article  ADS  MathSciNet  MATH  Google Scholar 

  30. J.J. Sakurai, Modern Quantum Mechanics (Addison-Wesley, Reading, 1994)

    Google Scholar 

  31. K.A. Suominen, B.M. Garraway, S. Stenholm, Phys. Rev. A 45, 3060 (1992)

    Article  ADS  Google Scholar 

  32. I.S. Gradshteyn, I.M. Ryzhik, Table of Integrals Series and Products, 5th edn. (Academic, New York, 1994)

    MATH  Google Scholar 

  33. F. Grossmann, Phys. Rev. A 60, 1791 (1999)

    Article  ADS  MathSciNet  Google Scholar 

  34. A. Assion, M. Geisler, J. Helbing, V. Seyfried, T. Baumert, Phys. Rev. A 54, R4605 (1996)

    Article  ADS  Google Scholar 

  35. C. Meier, Ph.D. Thesis, Theoretische Untersuchungen zur Photoelektronenspektroskopie kleiner Moleküle mit kurzen und intensiven Laserpulsen (Universität Freiburg, 1995)

    Google Scholar 

  36. V. Engel, Comput. Phys. Commun. 63, 228 (1991)

    Article  ADS  MATH  Google Scholar 

  37. V. Engel, H. Metiu, J. Chem. Phys. 100, 5448 (1994)

    Article  ADS  Google Scholar 

  38. S.O. Williams, D.G. Imre, J. Phys. Chem. 92, 6648 (1988)

    Article  Google Scholar 

  39. M. Dantus, M.J. Rosker, A.H. Zewail, J. Chem. Phys. 87, 2395 (1987)

    Article  ADS  Google Scholar 

  40. F. Hund, Z. Phys. 43, 805 (1927)

    Article  ADS  Google Scholar 

  41. F. Grossmann, T. Dittrich, P. Jung, P. Hänggi, Phys. Rev. Lett. 67, 516 (1991)

    Article  ADS  Google Scholar 

  42. F. Grossmann, Ph.D. Thesis, Der Tunneleffekt in periodisch getriebenen Quantensystemen (Universität Augsburg, 1992)

    Google Scholar 

  43. F. Grossmann, P. Hänggi, Europhys. Lett. 18(1), (1992)

    Google Scholar 

  44. J.H. Shirley, Phys. Rev. 138, B979 (1965)

    Article  ADS  Google Scholar 

  45. M. Abramowitz, I.A. Stegun, Handbook of Mathematical Functions (Dover, New York, 1965)

    Google Scholar 

  46. Y. Kayanuma, Phys. Rev. A 50, 843 (1994)

    Article  ADS  Google Scholar 

  47. G.D. Valle, M. Ornigotti, E. Cianci, V. Foglietti, P. Laporta, S. Longhi, Phys. Rev. Lett. 98, 263601 (2007)

    Article  ADS  Google Scholar 

  48. E. Kierig, U. Schnorrberger, A. Schietinger, J. Tomkovic, M.K. Oberthaler, Phys. Rev. Lett. 100, 190405 (2008)

    Article  ADS  Google Scholar 

  49. V. Roudnev, B.D. Esry, I. Ben-Itzhak, Phys. Rev. Lett. 93, 163601 (2004)

    Article  ADS  Google Scholar 

  50. M.F. Kling, C. Siedschlag, A.J. Verhoef, J.I. Khan, M. Schultze, T. Uphues, Y. Ni, M. Uiberacker, M. Drescher, F. Krausz, M.J.J. Vrakking, Science 312, 246 (2006)

    Article  ADS  Google Scholar 

  51. K. Bergmann, H. Theuer, B.W. Shore, Rev. Mod. Phys. 70, 1003 (1998)

    Article  ADS  Google Scholar 

  52. D.J. Tannor, S.A. Rice, Adv. Chem. Phys. 70, 441 (1988)

    Article  Google Scholar 

  53. R. Kosloff, S.A. Rice, P. Gaspard, S. Tersigni, D.J. Tannor, Chem. Phys. 139, 201 (1986)

    Article  ADS  Google Scholar 

  54. D.J. Tannor, R. Kosloff, S.A. Rice, J. Chem. Phys. 85, 5805 (1986)

    Article  ADS  Google Scholar 

  55. V.F. Krotov, I.N. Feldman, Eng. Cybernetics 21, 123 (1984)

    MathSciNet  Google Scholar 

  56. S.A. Rice, M. Zhao, Optical Control of Molecular Dynamics (Wiley, New York, 2000)

    Google Scholar 

  57. F. Grossmann, L. Feng, G. Schmidt, T. Kunert, R. Schmidt, Europhys. Lett. 60, 201 (2002)

    Article  ADS  Google Scholar 

  58. D. Zeidler, S. Frey, K.L. Kompa, M. Motzkus, Phys. Rev. A 64, 023420 (2001)

    Article  ADS  Google Scholar 

  59. R.S. Judson, H. Rabitz, Phys. Rev. Lett. 68, 1500 (1992)

    Article  ADS  Google Scholar 

  60. A. Assion, T. Baumert, M. Bergt, T. Brixner, B. Kiefer, V. Seyfried, M. Strehle, G. Gerber, Science 282, 919 (1998)

    Article  ADS  Google Scholar 

  61. D. Babikov, J. Chem. Phys. 121, 7577 (2004)

    Article  ADS  Google Scholar 

  62. T. Cheng, A. Brown, J. Chem. Phys. 124, 034111 (2006)

    Article  ADS  Google Scholar 

  63. J.R. Hiskes, Phys. Rev. 122, 1207 (1961)

    Article  ADS  Google Scholar 

  64. U. Weiss, W. Häffner, Phys. Rev. D 27, 2916 (1983)

    Article  ADS  Google Scholar 

  65. D.W. Hone, R. Ketzmerick, W. Kohn, Phys. Rev. A 56, 4045 (1997)

    Article  ADS  Google Scholar 

  66. D. Kohen, D.J. Tannor, J. Chem. Phys. 98, 3168 (1993)

    Article  ADS  Google Scholar 

  67. A. Emmanouilidou, X.G. Zhao, P. Ao, Q. Niu, Phys. Rev. Lett. 85, 1626 (2000)

    Article  ADS  Google Scholar 

  68. P. Passarinho, M.L. da Silva, J. Mol. Spectros. 236, 148 (2006)

    Article  ADS  Google Scholar 

  69. J.H. Posthumus, Rep. Prog. Phys. 67, 623 (2004)

    Article  ADS  Google Scholar 

  70. A.D. Bandrauk (ed.), Molecules in Laser Fields (Dekker, New York, 1994)

    Google Scholar 

  71. U. Saalmann, R. Schmidt, Z. Phys. D 38, 153 (1996)

    Article  ADS  Google Scholar 

  72. T. Kunert, R. Schmidt, Eur. Phys. J. D 25, 15 (2003)

    Article  ADS  Google Scholar 

  73. M. Thoss, H. Wang, Annu. Rev. Phys. Chem. 55, 299 (2004)

    Article  ADS  Google Scholar 

  74. J. Manz, L. Wöste (eds.) Femtosecond Chemistry, vols. 1 and 2 (VCH, Weinheim, 1995)

    Google Scholar 

  75. M. Grifoni, P. Hänggi, Phys. Rep. 304, 229 (1998)

    Article  MathSciNet  ADS  Google Scholar 

  76. P. Brumer, M. Shapiro, Principles of the Quantum Control of Molecular Processes (Wiley-VCH, Berlin, 2003)

    Google Scholar 

Download references

Rights and permissions

Reprints and permissions

Copyright information

© 2008 Springer-Verlag Berlin Heidelberg

About this chapter

Cite this chapter

(2008). Molecules in Strong Laser Fields. In: Theoretical Femtosecond Physics. Springer Series on Atomic, Optical, and Plasma Physics, vol 48. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-540-77897-4_5

Download citation

Publish with us

Policies and ethics