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Laser-Induced Photoacoustic Spectroscopy for the Speciation of Actinides in Submicromol Concentrations

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Photoacoustic and Photothermal Phenomena

Part of the book series: Springer Series in Optical Sciences ((SSOS,volume 58))

Abstract

Laser-induced Photoacoustic Spectroscopy (LPAS) is developed for the direct speciation of actinides in aquatic solutions. The speciation sensitivity is attained in the submicromol range, e.g. Ami3+ (ε = 400 L mol−1cm−1 down to 10−8 mol L−1, or ppb. The method provides spectroscopic information of chemical states of actinides and hence facilitates the study of their hydrolysis-reaction, complexation, redox-reaction and colloid generation. The application of LPAS is demonstrated for the speciation of Am and Pu ions in different solutions.

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References

  1. J.I. Kim: In Handbook on the Physics and Chemistry of the Actinides, Vol. 4, Eds.: A.J. Freeman and C. Keller, Elsevier Science Publishers B.V., 1986, p. 413

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Author information

Authors and Affiliations

  1. Institut für Radiochemie, TU München, D-8046, Garching, Fed. Rep. of Germany

    R. Klenze, R. Stumpe & J. I. Kim

Authors
  1. R. Klenze
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  2. R. Stumpe
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  3. J. I. Kim
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Editor information

Editors and Affiliations

  1. Institute of Physical Chemistry, University of Heidelberg, Im Neuenheimer Feld 253, D-6900, Heidelberg, Fed. Rep. of Germany

    Peter Hess

  2. Institute of Experimental Physics, Ruhr University, Universitätsstr. 150, D-4630, Bochum, Fed. Rep. of Germany

    Josef Pelzl

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© 1988 Springer-Verlag Berlin Heidelberg

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Klenze, R., Stumpe, R., Kim, J.I. (1988). Laser-Induced Photoacoustic Spectroscopy for the Speciation of Actinides in Submicromol Concentrations. In: Hess, P., Pelzl, J. (eds) Photoacoustic and Photothermal Phenomena. Springer Series in Optical Sciences, vol 58. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-540-48181-2_35

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  • DOI: https://doi.org/10.1007/978-3-540-48181-2_35

  • Publisher Name: Springer, Berlin, Heidelberg

  • Print ISBN: 978-3-662-13705-5

  • Online ISBN: 978-3-540-48181-2

  • eBook Packages: Springer Book Archive

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