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Surface-Enhanced Nonlinear Optical Effects and Detection of Absorbed Molecular Monolayers

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Laser Spectroscopy V

Part of the book series: Springer Series in Optical Sciences ((SSOS,volume 30))

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Abstract

In recent years, we have been interested in the study of nonlinear optical effects at interfaces. Our motivation is twofold. First, while nonlinear optics in a bulk medium is now well developed, that at an interface has not received much attention since the early investigations of BLOEMBERGEN and co-workers on second-harmonic reflection from a surface [1]. Second, with the understanding of surface nonlinear optics, we hope to use it for the study of surface properties, in particular, for the study of molecular adsorption and overlayers on surfaces. There already exist various techniques for studies of this nature, such as photoemission, LEED, Auger, infrared, and Raman spectroscopy [2], but laser optical techniques are intrinsically better in spectral resolution.

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References

  1. N. Bloembergen and P. S. Pershan, Phys. Rev. 128, 606 (1962)

    Article  MathSciNet  ADS  MATH  Google Scholar 

  2. N. Bloembergen, R. K. Chang, S. S. Jha, and C. H. Lee, Phys. Rev. 174, 813 (1968)

    Article  ADS  Google Scholar 

  3. See, for example, G, A. Somorjai, M. A. Van Hove, Adsorbed Monolayers on Solid Surfaces, Structure and Bonding, Vol. 38 ( Springer, Berlin, Heidelberg, New York 1979 )

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  4. C. K. Chen, A. R. B. de Castro, Y. R. Shen, and F. DeMartini, Phys. Rev. 43, 946 (1979)

    ADS  Google Scholar 

  5. J. P. Heritage and D. L. Allara, Chem. Phys. Lett. 74, 507 (1980)

    Article  ADS  Google Scholar 

  6. B. F. Levine, C. G. Bethea, A. R. Tretola, and M. Korngor, Appl. Phys. Lett. 37, 595 (1980)

    Article  ADS  Google Scholar 

  7. M. Fleischmann, P. J. Hendra, and A. J. McQuillan, Chem. Phys. Lett. 26, 163 (1974)

    Article  ADS  Google Scholar 

  8. D. L. teanmaire and R. P. Van Duyne, J. Electroanal. Chem. 34, 1 (1977)

    Article  Google Scholar 

  9. C. K. Chen, A. R. B. de Castro, and Y. R. Shen, Phys.. Rev. Lett. 46, 145 (1981)

    Article  ADS  Google Scholar 

  10. C. K. Chen, T. F. Heinz, D. Ricard, and Y. R. Shen, Phys. Rev. Lett. 46, 1010 (1981)

    Article  ADS  Google Scholar 

  11. See J. Gersten and A. Nitzan, J. Chem. Phys. 73, 3023 (1980) and references therein

    Google Scholar 

  12. See, for example, N. Bloembergen, Nonlinear Optics (Benjamin, New York, 1964 )

    Google Scholar 

  13. G. T. Boyd and Z. H. Yu (unpublished)

    Google Scholar 

  14. R. K. Chang (to be published)

    Google Scholar 

  15. For weak static fields, see B. F. Levine and C. G. Bethea, J. Chem. Phys. 63, 2666 (1975)

    Article  ADS  Google Scholar 

  16. See, for example, M. J. Rosen, Surfactants and Interfacial Phenomena (J. Wiley and Sons, New York, 1978), Chap.2

    Google Scholar 

  17. R. Dornhaus, B. M. Long, R. E. Benner, and R. K. Chang, Surf. Sci. 93, 240 (1980)

    Article  ADS  Google Scholar 

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Author information

Authors and Affiliations

  1. Department of Physics, University of California, Berkeley, CA, 94720, USA

    Y. R. Shen, C. K. Chen, T. F. Heinz & D. Ricard

  2. Materials and Molecular Research Division, Lawrence Berkeley Laboratory, Berkeley, CA, 94720, USA

    Y. R. Shen, C. K. Chen, T. F. Heinz & D. Ricard

Authors
  1. Y. R. Shen
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  2. C. K. Chen
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  3. T. F. Heinz
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  4. D. Ricard
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Editor information

Editors and Affiliations

  1. Herzberg Institute of Astrophysics, National Research Council of Canada, K1A OR6, Ottawa, Ontario, Canada

    A. Robert W. McKellar

  2. Department of Chemistry, of Astronomy, and Astrophysics, University of Chicago, 60637, Chicago, IL, USA

    Takeshi Oka

  3. Department of Physics, McLennan Physics Laboratory, University of Toronto, M5S 1A7, Toronto, Ontario, Canada

    Boris P. Stoicheff

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© 1981 Springer-Verlag Berlin Heidelberg

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Shen, Y.R., Chen, C.K., Heinz, T.F., Ricard, D. (1981). Surface-Enhanced Nonlinear Optical Effects and Detection of Absorbed Molecular Monolayers. In: McKellar, A.R.W., Oka, T., Stoicheff, B.P. (eds) Laser Spectroscopy V. Springer Series in Optical Sciences, vol 30. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-540-38804-3_71

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  • DOI: https://doi.org/10.1007/978-3-540-38804-3_71

  • Publisher Name: Springer, Berlin, Heidelberg

  • Print ISBN: 978-3-662-15380-2

  • Online ISBN: 978-3-540-38804-3

  • eBook Packages: Springer Book Archive

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