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Structural and Dielectric Studies of PbYb1/2Nb1/2O3 Ceramics with the Differing Degree of the Long-Range Compositional Ordering Fabricated by Mechanoactivation

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Part of the book series: Springer Proceedings in Physics ((SPPHY,volume 207))

Abstract

It was found out that compositional ordering degree S of Yb3+ and Nb5+ ions in PbYb1/2Nb1/2O3 ceramics and correspondingly both the temperature and diffusion of antiferroelectric phase transition can be varied within a wide range by means of high-energy mechanical activation. In particular, for the first time disordered PbYb1/2Nb1/2O3 ceramics exhibiting relaxor-like dielectric properties was fabricated without the use of any additives. For the most ordered PbYb1/2Nb1/2O3 samples (S ≈ 0.82), the coexistence of cubic paraelectric and orthorhombic antiferroelectric phases in a temperature range 190–300 °C was revealed.

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Acknowledgements

This work was supported in part by the Ministry of Education and Science of the Russian Federation (research project No. 3.1649.2017/4.6) and by the Russian Foundation for Basic Research (grant No. 17-03-01293_a).

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Authors and Affiliations

  1. Research Institute of Physics and Faculty of Physics, Southern Federal University, 344090, Rostov-on-Don, Russia

    I. P. Raevski, Yu. A. Kuprina, I. N. Zakharchenko, O. A. Bunina, V. V. Titov, S. I. Raevskaya, M. A. Malitskaya, A. V. Blazhevich, S. V. Orlov & E. I. Sitalo

  2. Institute of Solid State Chemistry and Mechanochemistry, SB RAS, 630128, Novosibirsk, Russia

    Yu. A. Kuprina, A. A. Gusev & V. P. Isupov

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Correspondence to I. P. Raevski .

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  1. I. I. Vorovich Mathematics, Mechanics and Computer Sciences Institute, Southern Federal University, Rostov-on-Don, Russia

    Ivan A. Parinov

  2. Department of Microelectronics Engineering, National Kaohsiung University of Science and Technology, Kaohsiung, Taiwan

    Shun-Hsyung Chang

  3. Indian Institute of Information Technology, Design and Manufacturing, Jabalpur, Jabalpur, Madhya Pradesh, India

    Vijay K. Gupta

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Raevski, I.P. et al. (2018). Structural and Dielectric Studies of PbYb1/2Nb1/2O3 Ceramics with the Differing Degree of the Long-Range Compositional Ordering Fabricated by Mechanoactivation. In: Parinov, I., Chang, SH., Gupta, V. (eds) Advanced Materials . PHENMA 2017. Springer Proceedings in Physics, vol 207. Springer, Cham. https://doi.org/10.1007/978-3-319-78919-4_17

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