Abstract
The theory of excitonic quasimolecules (formed of spatially separated electrons and holes) in nanosystems that consist of semiconductor quantum dots synthesized in a borosilicate glass matrix is presented. It is shown that exciton quasimolecule formation is of the threshold character and possible in nanosystem, if the spacing between the quantum dot surfaces is larger than a certain critical spacing. It was found that the binding energy of singlet ground state of exciton quasimolecule, consisting of two semiconductor quantum dots, is a significant large value, larger than the binding energy of the biexciton in a semiconductor single crystal by almost two orders of magnitude.
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Ashoori RC (1996) Electrons in artificial atoms. Nature 379:413–415
Pokutnyi SI (2013) On an exciton with a spatially separated electron and hole in quasi-zero-dimensional semiconductor nanosystems. Semiconductors 47(6):791–798
Pokutnyi SI (2014) Theory of excitons and excitonic quasimolecules formed from spatially separated electrons and holes in quasi-zero-dimensional nanosytems. Optics 3(1):10–21
Yakimov AI, Dvurechensky AV et al (2001) Effects of electron-electron interaction in the optical properties of dense arrays of quantum dots Ge/Si. JETP 119:574–589
Grabovskis V, Dzenis Y, Ekimov A (1989) Photoionization of semiconductor microcrystals in glass. Sov Phys Solid State 31(1):272–275
Bondar N (2010) Photoluminescence quantum and surface states of excitons in ZnSe and CdS nanoclusters. J Luminescence 130(1):1–7
Ovchinnikov OV, Smirnov MS, Shatskikh TS (2014) Spectroscopic investigation of colloidal CdS quantum dots – methylene blue hybrid associates. J Nanopart Res 16:2286–2292
Dzyuba VP, Kulchin YN, Milichko VA (2013) Quantum size states of a particle inside the nanospheres. Adv Mater Res A 677:42–48
Pokutnyi SI (2013) Binding energy of the exciton with a spatially separated electron and hole in quasi-zero-dimensional semiconductor nanosystems. Tech Phys Lett 39(3):233–235
Pokutnyi SI, Kulchin YN, Dzyuba VP (2015) Binding energy of excitons formed from spatially separated electrons and holes in insulating quantum dots. Semiconductors 49(10):1311–1315
Pokutnyi SI (2013) Biexcitons formed from spatially separated electrons and holes in quasi-zero-dimensional semiconductor nanosystems. Semiconductors 47(12):1626–1635
Pokutnyi SI (2016) Biexciton in Nanosystem of quantum dots of cadmium Sulfide in a dielectric matrix. Tech Phys 61(11):1737–1739
Pokutnyi SI, Kulchin YN, Dzyuba VP, Amosov AV (2016) Biexciton in nanoheterostructures of dielectric quantum dots. J Nanophotonics 10(3):036008-1–036008-8
Pokutnyi SI (2016) Quantum – chemical analysis of system consisting of two CdS quantum dots. Theor Exp Chem 52(1):27–32
Lalumiure K, Sanders B, Van Loo F et al (2013) Input - output theory for waveguide QED with an ensemble of inhomogeneous atoms. Phys Rev A 88:43806–43811
Van Loo F, Fedorov A, Lalumiure K et al (2013) Photon-mediated interactions between distant artificial atoms. Science 342:1494–1496
Lozovik YE (2014) Electronic and collective properties of topological insulators. Advanc. Phys. Scienc. 57:653–658
Valiev K (2005) Quantum computers and quantum computing. Advanc Phys Scienc 48:1–22
Pokutnyi SI (2007) Exciton states in semiconductor quantum dots in the framework of the modified effective mass method. Semiconductors 41(11):1323–1328
Schiff L (1955) Quantum mechanics. McGraw-Hill Book Company, Inc. New York- Toronto-London
Pokutnyi SI, Ovchinnikov OV, Kondratenko TS (2016) Absorption of light by colloidal semiconductor quantum dots. J Nanophotonics 10(3):033506-1–033506-9
Pokutnyi SI (1992) Size quantization of excitons in quasi-zero-dimensional semiconductor structures. Phys Lett A 168(5–6):433–436
Pokutnyi SI (2005) Optical nanolaser on the heavy hole transition in semiconductor nanocrystals: theory. Phys Lett A 342:347–350
Pokutnyi SI et al (2004) Stark effect in semiconductor quantum dots. J Appl Phys 96(2):1115–1119
Pokutnyi SI, Kulchin YN (2016) Special section guest editorial: optics, spectroscopy, and Nanophotonics of quantum dots. J. Nanophotonics 10(3):033501-1–033501-8
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Pokutnyi, S.I. (2017). Excitonic Quasimolecules in Nanoheterosystems Containing Semiconductor and Dielectric Quantum Dots. In: Fesenko, O., Yatsenko, L. (eds) Nanophysics, Nanomaterials, Interface Studies, and Applications . NANO 2016. Springer Proceedings in Physics, vol 195. Springer, Cham. https://doi.org/10.1007/978-3-319-56422-7_10
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DOI: https://doi.org/10.1007/978-3-319-56422-7_10
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