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The primary field this dissertation lies within is magnetic resonance theory and experiment, specifically concerning nuclear magnetic resonance (NMR) and electron paramagnetic (or spin) resonance (EPR or ESR). NMR studies presented in Chap. 2 involve solid xenon that is polarized by spin-exchange optical pumping (SEOP), thus there is some discussion of atomic physics related to this technique. Chapter 3 concerns EPR of electron-hole pairs in semiconductors, specifically electrically or optically detected magnetic resonance (EDMR and PDMR).