Skip to main content
SpringerLink
Log in
Book cover

Ultrafast Phenomena XIX pp 48–51Cite as

Direct Comparison of Multi-photon and EUV Single-Photon Probing of Molecular Relaxation Processes

  • Conference paper
  • First Online:

  • 151 Accesses

Part of the book series: Springer Proceedings in Physics ((SPPHY,volume 162))

Abstract

We present a new setup for time-resolved photoelectron and photoion spectroscopy allowing for single-photon EUV or multi-photon NIR ionization. Comparison of the two different probe schemes reveals disagreements shedding light on the underlying advantages of different probes.

This is a preview of subscription content, log in via an institution.

Chapter
USD   29.95
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
eBook
USD   169.00
Price excludes VAT (USA)
  • Available as EPUB and PDF
  • Read on any device
  • Instant download
  • Own it forever
Softcover Book
USD   219.99
Price excludes VAT (USA)
  • Compact, lightweight edition
  • Dispatched in 3 to 5 business days
  • Free shipping worldwide - see info
Hardcover Book
USD   219.99
Price excludes VAT (USA)
  • Durable hardcover edition
  • Dispatched in 3 to 5 business days
  • Free shipping worldwide - see info

Tax calculation will be finalised at checkout

Purchases are for personal use only

Learn about institutional subscriptions

References

  1. Stolow, A, Underwood, J. G.: Time-Resolved Photoelectron Spectroscopy of Nonadiabatic Dynamics in Polyatomic Molecules., Advances in Chemical Physics 19, 497–587 (2008).

    Google Scholar 

  2. Hudock, H. R., Levine, B. G., Thompson, A. L., Satzger, H., Townsend, D., Gador, N., Ullrich, S., Stolow, A., Martínez, T. J.: Ab Initio Molecular Dynamics and Time-Resolved Photoelectron Spectroscopy of Electronically Excited Uracil and Thymine. J. Phys. Chem. A 111, 8500–8508 (2007).

    Google Scholar 

  3. Barbatti, M., Ullrich, S.: Ionization potentials of adenine along the internal conversion pathways. Phys. Chem. Chem. Phys. 13, 15492–15500 (2011).

    Google Scholar 

  4. Koch, M., Wolf, T. J. A., Grilj, J., Sistrunk, E., Gühr, M.: Femtosecond photoelectron and photoion spectrometer with vacuum ultraviolet probe pulses. arXiv:1404.3039 (2014).

  5. Grilj, J., Sistrunk, E., Koch, M., Gühr, M.: A Beamline for Time-Resolved Extreme Ultraviolet and Soft X-Ray Spectroscopy. J. Anal. Bioanal. Tech. S12:005. (2014).

    Google Scholar 

  6. Kiba, T., Sato, S., Akimoto, S., Kasajima, T., Yamazaki, I: Solvent-assisted intramolecular vibrational energy redistribution of S1 perylene in ketone solvents. J. Photochem. Photobiol., A 178, 201–207 (2006).

    Google Scholar 

Download references

Acknowledgments

This material is based on work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Science, Chemical Sciences, Geosciences, and Biosciences Division. M. G. acknowledges funding via the Office of Science Early Career Research Program through the Office of Basic Energy Sciences, U.S. Department of Energy. T. W. acknowledges support from the German Academy of Sciences Leopoldina. M. K. acknowledges support form the Austrian Science Fund FWF (Schroedinger Grant) J3299-N20). J. G. acknowledges support from the European Commission under the Marie Curie Fellowship Programme.

Author information

Authors and Affiliations

  1. Stanford PULSE Institute, SLAC National Accelerator Laboratory, Menlo Park, CA, 94025, USA

    T. J. A. Wolf, E. Sistrunk & M. Gühr

  2. Stanford PULSE Institute and Institute of Experimental Physics, Graz University of Technology, Petersgasse 16, 8010, Graz, Austria, EU

    M. Koch

  3. Stanford PULSE Institute and Laboratoire de Spectroscopie Ultrarapide, Ecole Polytechnique Federale de Lausanne EPFL, 1015, Lausanne, Switzerland

    J. Grilj

Authors
  1. T. J. A. Wolf
    View author publications

    You can also search for this author in PubMed Google Scholar

  2. M. Koch
    View author publications

    You can also search for this author in PubMed Google Scholar

  3. E. Sistrunk
    View author publications

    You can also search for this author in PubMed Google Scholar

  4. J. Grilj
    View author publications

    You can also search for this author in PubMed Google Scholar

  5. M. Gühr
    View author publications

    You can also search for this author in PubMed Google Scholar

Corresponding author

Correspondence to T. J. A. Wolf .

Editor information

Editors and Affiliations

  1. Department of Chemistry, The University of Tokyo, Tokyo, Japan

    Kaoru Yamanouchi

  2. JILA, University of Colorado, Boulder, Colorado, USA

    Steven Cundiff

  3. Department of Chemistry, Ludwig-Maximilians-University, München, Germany

    Regina de Vivie-Riedle

  4. Department of Physics, The University of Tokyo, Tokyo, Japan

    Makoto Kuwata-Gonokami

  5. Department of Physics, The Ohio State University, Columbus, Ohio, USA

    Louis DiMauro

Rights and permissions

Reprints and permissions

Copyright information

© 2015 Springer International Publishing Switzerland

About this paper

Cite this paper

Wolf, T.J.A., Koch, M., Sistrunk, E., Grilj, J., Gühr, M. (2015). Direct Comparison of Multi-photon and EUV Single-Photon Probing of Molecular Relaxation Processes. In: Yamanouchi, K., Cundiff, S., de Vivie-Riedle, R., Kuwata-Gonokami, M., DiMauro, L. (eds) Ultrafast Phenomena XIX. Springer Proceedings in Physics, vol 162. Springer, Cham. https://doi.org/10.1007/978-3-319-13242-6_12

Download citation

Publish with us

Policies and ethics

Search

Navigation