Skip to main content

A Student’s Introduction to Resonant Inelastic Soft X-ray Scattering

  • Conference paper
  • First Online:
Magnetism and Synchrotron Radiation: Towards the Fourth Generation Light Sources

Part of the book series: Springer Proceedings in Physics ((SPPHY,volume 151))

  • 1611 Accesses

Abstract

Recent instrumental advances have opened an important window for studying magnetic excitations with resonant inelastic x-ray scattering (RIXS). This contribution outlines the main theoretical and experimental aspects underlying this spectroscopic technique. The aspects discussed cover self-absorption corrections, scattering geometry, resonant scattering cross sections and methods for identifying and exploiting spectral information. State of the art diffraction grating spectrometers are assessed in view of RIXS opportunities that lie ahead.

This is a preview of subscription content, log in via an institution to check access.

Access this chapter

Chapter
USD 29.95
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
eBook
USD 169.00
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
Softcover Book
USD 219.99
Price excludes VAT (USA)
  • Compact, lightweight edition
  • Dispatched in 3 to 5 business days
  • Free shipping worldwide - see info
Hardcover Book
USD 219.99
Price excludes VAT (USA)
  • Durable hardcover edition
  • Dispatched in 3 to 5 business days
  • Free shipping worldwide - see info

Tax calculation will be finalised at checkout

Purchases are for personal use only

Institutional subscriptions

Preview

Unable to display preview. Download preview PDF.

Unable to display preview. Download preview PDF.

References

  1. A. Kotani, S. Shin, Rev. Mod. Phys. 73, 203 (2001)

    Google Scholar 

  2. A. Kotani, Eur. Phys. J. B 47, 3 (2005)

    Google Scholar 

  3. L.J.P. Ament, M. van Veenendaal, T.P. Devereaux, J.P. Hill, J. van den Brink, Rev. Mod. Phys. 83, 705 (2011)

    Google Scholar 

  4. J.P. Rueff, A. Shukla, Rev. Mod. Phys. 82, 847 (2010)

    Google Scholar 

  5. W. Schülke, Electron Dynamics by Inelastic X-Ray Scattering, Oxford Series on Synchrotron Radiation, vol. 7 (Oxford University Press, Oxford, 2007)

    Google Scholar 

  6. F.M.F. de Groot, A. Kotani, Core Level Spectroscopy of Solids (CRC Press, Boca Raton, 2008)

    Google Scholar 

  7. F. Gel’mukhanov, H. Ågren, Phys. Rep. 312, 87 (1999)

    Google Scholar 

  8. J. Stöhr, H.C. Siegmann, Magnetism: From Fundamentals to Nanoscale Dynamics. Springer Series in Solid-State Sciences (Springer, Berlin, 2006)

    Google Scholar 

  9. A. Zangwill, Physics at Surfaces (Cambridge University Press, Cambridge, 1988)

    Google Scholar 

  10. R. Kurian, K. Kunnus, P. Wernet, S.M. Butorin, P. Glatzel, F.M.F. de Groot, J. Phys.: Condens. Matter 24, 452201 (2012)

    Google Scholar 

  11. S. Eisebitt, T. Böske, J.E. Rubensson, W. Eberhardt, Phys. Rev. B 47, 14103 (1993)

    Google Scholar 

  12. M.T. Hutchings, E.J. Samuelsen, Phys. Rev. B 6, 3447 (1972)

    Google Scholar 

  13. J.J. Sakurai, Advanced Quantum Mechanics (Addison-Wesley, Lebanon, 1967)

    Google Scholar 

  14. M. Blume, J. Appl. Phys. 57, 3615 (1985)

    Google Scholar 

  15. F. de Groot, J. Vogel, Neutron and X-ray Spectroscopy (Springer, Berlin, 2006), chap. Fundamentals of x-ray absorption and dichroism: the multiplet approach, pp. 3–66

    Google Scholar 

  16. S.F.A. Kettle, Symmetry and Structure: Readable Group Theory for Chemists (John Wiley & Sons, New York, 2007)

    Google Scholar 

  17. B. Fromme, dd Excitations in Transition-Metal Oxides: A Spin-Polarized Electron Energy (SPEELS) Study, Springer Tracts in Modern Physics, vol. 170 (Springer, Berlin, 2001)

    Google Scholar 

  18. F.M.F. de Groot, P. Kuiper, G.A. Sawatzky, Phys. Rev. B 57, 14584 (1998)

    Google Scholar 

  19. O. Keski-Rahkonen, M.O. Krause, Atomic Data and Nuclear Data Tables 14, 139 (1974)

    Google Scholar 

  20. J.E. Rubensson, J. Elec. Spec. Rel. Phenom. 110 - 111, 135 (2000)

    Google Scholar 

  21. P. Glatzel, M. Sikora, M. Fernández-García, Eur. Phys. J. Special Topics 169, 207 (2009)

    Google Scholar 

  22. S. Hüfner, Adv. Phys. 43, 183 (1994)

    Google Scholar 

  23. J. Zaanen, G.A. Sawatzky, J.W. Allen, Phys. Rev. Lett. 55, 418 (1985)

    Google Scholar 

  24. A.E. Bocquet, T. Mizokawa, K. Morikawa, A. Fujimori, S.R. Barman, K. Maiti, D.D. Sarma, Y. Tokura, M. Onoda, Phys. Rev. B 53, 1161 (1996)

    Google Scholar 

  25. A.K. Masahiko Matsubara, Takayuki Uozumi, J.C. Parlebas, J. Phys. Soc. Jpn 74, 2052 (2005)

    Google Scholar 

  26. S.G. Chiuzbăian, G. Ghiringhelli, C. Dallera, M. Grioni, P. Amann, X. Wang, L. Braicovich, L. Patthey, Phys. Rev. Lett. 95, 197402 (2005)

    Google Scholar 

  27. S.G. Chiuzbăian, T. Schmitt, M. Matsubara, A. Kotani, G. Ghiringhelli, C. Dallera, A. Tagliaferri, L. Braicovich, V. Scagnoli, N.B. Brookes, U. Staub, L. Patthey, Phys. Rev. B 78, 245102 (2008)

    Google Scholar 

  28. M. Magnuson, S.M. Butorin, A. Agui, J. Nordgren, J. Phys.: Condens. Matter 14, 3669 (2002)

    Google Scholar 

  29. A. Shukla, J.P. Rueff, J. Badro, G. Vanko, A. Mattila, F.M.F. de Groot, F. Sette, Phys. Rev. B 67, 081101 (2003)

    Google Scholar 

  30. L.C. Duda, T. Schmitt, M. Magnuson, J. Forsberg, A. Olsson, J. Nordgren, K. Okada, A. Kotani, Phys. Rev. Lett. 96, 067402 (2006)

    Google Scholar 

  31. G. van der Laan, in Magnetism: A Synchrotron Radiation Approach, ed. by E. Beaurepaire, H. Bulou, F. Scheurer, J.-P. Kappler, (Springer, Berlin, 2006), p.143

    Google Scholar 

  32. E. Saitoh, S. Okamoto, K. Takahashi, K. Tobe, K. Yamamoto, T. Kimura, S. Ishihara, S. Maekawa, Y. Tokura, Nature 410, 180 (2001)

    Google Scholar 

  33. J. Schlappa, K. Wohlfeld, K. Zhou, M. Mourigal, M. Haverkort, V. Strocov, L. Hozoi, C. Monney, S. Nishimoto, S. Singh, A. Revcolevschi, J.S. Caux, L. Patthey, H. Rønnow, J. van den Brink, T. Schmitt, Nature 485, 82 (2012)

    Google Scholar 

  34. G. Ghiringhelli, A. Piazzalunga, C. Dallera, T. Schmitt, V.N. Strocov, J. Schlappa, L. Patthey, X. Wang, H. Berger, M. Grioni, Phys. Rev. Lett. 102, 027401 (2009)

    Google Scholar 

  35. L. Braicovich, J. van den Brink, V. Bisogni, M.M. Sala, L.J.P. Ament, N.B. Brookes, G.M. De Luca, M. Salluzzo, T. Schmitt, V.N. Strocov, G. Ghiringhelli, Phys. Rev. Lett. 104, 077002 (2010)

    Google Scholar 

  36. L. Braicovich, L.J.P. Ament, V. Bisogni, F. Forte, C. Aruta, G. Balestrino, N.B. Brookes, G.M. De Luca, P.G. Medaglia, F.M. Granozio, M. Radovic, M. Salluzzo, J. van den Brink, G. Ghiringhelli, Phys. Rev. Lett. 102, 167401 (2009)

    Google Scholar 

  37. W.B. Peatman, Gratings, Mirrors and Slits (Taylor & Francis, London, 1997)

    Google Scholar 

  38. S.C. Locklin, E.J. Moler, J. Spring, Z. Hussain, M.R. Howells, Progress in soft-x-ray Fourier transform spectrometry. Tech. rep., Advanced Light Source, LBNL, Berkeley, CA (1998)

    Google Scholar 

  39. M. Agåker, J. Andersson, C.J. Englund, A. Olsson, M. Strom, J. Nordgren, Nucl. Instrum. Meth. A 601, 213 (12009)

    Google Scholar 

  40. J.H. Underwood, in X-ray Data Booklet (Lawrence Berkeley National Laboratory, Berkeley, 2009), pp. 4.6–4.12

    Google Scholar 

  41. J. Nordgren, R. Nyholm, Nucl. Instrum. Meth. A 246, 242 (1986)

    Google Scholar 

  42. T.A. Callcott, K.L. Tsang, C.H. Zhang, D.L. Ederer, E.T. Arakawa, Rev. Sci. Instrum. 57, 2680 (1986)

    Google Scholar 

  43. M.R. Howells, in X-ray Data Booklet (Lawrence Berkeley National Laboratory, Berkeley, 2009), pp. 4.16–4.26

    Google Scholar 

  44. C. Dallera, E. Puppin, G. Trezzi, N. Incorvaia, A. Fasana, L. Braicovich, N. Brookes, J. Goedkoop, J. Synch. Rad. 3, 231 (1998)

    Google Scholar 

  45. G. Ghiringhelli, A. Piazzalunga, C. Dallera, G. Trezzi, L. Braicovich, T. Schmitt, V.N. Strocov, R. Betemps, L. Patthey, X. Wang, M. Grioni, Rev. Sci. Instrum. 77, 113108 (2006)

    Google Scholar 

  46. Y. Harada, M. Kobayashi, H. Niwa, Y. Senba, H. Ohashi, T. Tokushima, Y. Horikawa, S. Shin, M. Oshima, Rev. Sci. Instrum. 83, 013116 (2012)

    Google Scholar 

  47. S.G. Chiuzbăian, C.F. Hague, J. Lüning, Appl. Optics 51, 4684 (2012)

    Google Scholar 

  48. M.C. Hettrick, J.H. Underwood. US patent no 4,776,696: Optical system for high resolution spectrometer/monochromator (1988)

    Google Scholar 

  49. J.H. Underwood, J.A. Koch, Appl. Optics 36, 4913 (1997)

    Google Scholar 

  50. C.F. Hague, J.H. Underwood, A. Avila, R. Delaunay, H. Ringuenet, M. Marsi, M. Sacchi, Rev. Sci. Instrum. 76, 023110 (2005)

    Google Scholar 

  51. Y.D. Chuang, J. Pepper, W. McKinney, Z. Hussain, E. Gullikson, P. Batson, D. Qian, M.Z. Hasan, J. Phys. Chem. Solids 66, 2173 (2005)

    Google Scholar 

  52. O. Fuchs, L.Weinhardt, M. Blum, M.Weigand, E. Umbach, M. Bar, C. Heske, J. Denlinger, Y.D. Chuang, W. McKinney, Z. Hussain, E. Gullikson, M. Jones, P. Batson, B. Nelles, R. Follath, Rev. Sci. Instrum. 80, 063103 (2009)

    Google Scholar 

  53. S.G. Chiuzbăian, et al. (to be published)

    Google Scholar 

  54. R. Könnecke, R. Follath, N. Pontius, J. Schlappa, F. Eggenstein, T. Zeschke, P. Bischoff, J.S. Schmidt, T. Noll, C. Trabant, S. Schreck, P.Wernet, S. Eisebitt, F. Senf, C. Schüßler-Langeheine, A. Erko, A. Föhlisch, J. Electron Spectrosc. (2012) In press

    Google Scholar 

  55. H.S. Fung, C.T. Chen, L.J. Huang, C.H. Chang, S.C. Chung, D.J. Wang, T.C. Tseng, K.L. Tsang, AIP Conf. Proc. 705, 655 (2004)

    Google Scholar 

Download references

Acknowledgments

The writing of this chapter has benefited from stimulating discussions with Coryn Frank Hague, Jan Lüning and Jean-Michel Mariot at Laboratoire de Chimie Physique-Matière et Rayonnement. The author is grateful to C.F.H. and J.-M.M. for critical reading of the manuscript.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Sorin G. Chiuzbăian .

Editor information

Editors and Affiliations

Rights and permissions

Reprints and permissions

Copyright information

© 2013 Springer International Publishing Switzerland

About this paper

Cite this paper

Chiuzbăian, S.G. (2013). A Student’s Introduction to Resonant Inelastic Soft X-ray Scattering. In: Beaurepaire, E., Bulou, H., Joly, L., Scheurer, F. (eds) Magnetism and Synchrotron Radiation: Towards the Fourth Generation Light Sources. Springer Proceedings in Physics, vol 151. Springer, Cham. https://doi.org/10.1007/978-3-319-03032-6_6

Download citation

Publish with us

Policies and ethics