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Optical Diagnostics with Ultrafast and Strong Field Raman Techniques

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Book cover Ultrafast Phenomena in Molecular Sciences

Part of the book series: Springer Series in Chemical Physics ((CHEMICAL,volume 107))

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Abstract

In this chapter, we will discuss some coherent techniques, namely Raman Induced Polarization Spectroscopy (RIPS) and femtosecond Coherent Raman Anti-Stokes Spectroscopy (fs-CARS). We will demonstrate their ability to be used as non-invasive optical diagnostic tools for temperature, density, or concentration measurements, as well as a means of testing collision induced energy transfer models (in a low field regime), and studying the so-called inhomogeneous lineshape effects that are particularly enhanced in the case of hydrogen. We will also show how molecular alignment achieved in a strong field regime can provide additional information about collisional relaxation processes. In all cases, a precise knowledge of the collisional effects is required, and so a general modeling of collisional relaxations will be detailed.

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Acknowledgements

The authors would like to thank Ha Tran, P. Joubert, L. Bonamy, D. Robert, R. Saint-Loup, D. Sugny, Th. Vieillard, and V. Renard for their contributions to the results presented here.

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Authors and Affiliations

  1. Laboratoire Interdisciplinaire CARNOT de Bourgogne (ICB), UMR 6303 CNRS–Université de Bourgogne, BP 47870, 21078, Dijon Cedex, France

    Frederic Chaussard, Bruno Lavorel, Edouard Hertz & Olivier Faucher

Authors
  1. Frederic Chaussard
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  2. Bruno Lavorel
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  3. Edouard Hertz
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  4. Olivier Faucher
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Corresponding author

Correspondence to Olivier Faucher .

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Editors and Affiliations

  1. Institute of Physical Chemistry Rocasolano, Spanish National Research Council, Madrid, Spain

    Rebeca de Nalda

  2. Department of Physical Chemistry Faculty of Chemistry, Complutense University of Madrid, Madrid, Spain

    Luis Bañares

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Chaussard, F., Lavorel, B., Hertz, E., Faucher, O. (2014). Optical Diagnostics with Ultrafast and Strong Field Raman Techniques. In: de Nalda, R., Bañares, L. (eds) Ultrafast Phenomena in Molecular Sciences. Springer Series in Chemical Physics, vol 107. Springer, Cham. https://doi.org/10.1007/978-3-319-02051-8_11

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