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In Situ PM IRRAS Studies of Redox-Inactive Molecular Films Adsorbed on Electrodes

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Application of Polarization Modulation Infrared Reflection Absorption Spectroscopy in Electrochemistry

Part of the book series: Monographs in Electrochemistry ((MOEC))

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Abstract

Adsorption of ions or neutral molecules on electrode surfaces leads to changes in the macroscopic properties of surfaces such as the surface energy, contact angle, surface charge density or surface potential. Potential-driven adsorption-desorption process of ions or neutral molecules on electrode surfaces belongs to an important research topic in electrochemistry. The process of adsorption of ions and molecules on the electrode surface may be understood at the molecular level when structure analyzing techniques, such as PM IRRAS, are applied to the electrochemical interface. Since the first application of PM IRRAS to the electrochemical interface the picture of potential-dependent changes in the structure, composition, and orientation of ions and amphiphilic molecules present on metallic electrode surfaces is available in the literature. Numerous studies are dedicated to investigate potential-dependent structural changes in biomimetic systems such as lipid bilayers, their interaction with proteins as well as self-assembled protein or DNA films.

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  1. Department of Chemistry, University of Oldenburg, Oldenburg, Germany

    Izabella Brand

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Brand, I. (2020). In Situ PM IRRAS Studies of Redox-Inactive Molecular Films Adsorbed on Electrodes. In: Application of Polarization Modulation Infrared Reflection Absorption Spectroscopy in Electrochemistry . Monographs in Electrochemistry. Springer, Cham. https://doi.org/10.1007/978-3-030-42164-9_3

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