Abstract
Subpicosecond ultraviolet laser technology is enabling the exploration of nonlinear atomic interactions with electric field strengths considerably in excess of an atomic unit. As this regime is approached, experiments studying multiple ionization, photoelectron energy spectra, and harmonically produced radiation all exhibit strong nonlinear coupling. Peak total energy transfer rates on the order of ∼ 2 × 10−4 W/atom have been observed at an intensity of ∼ 1016 W/cm2, and it is expected that energy transfer rates approaching ∼0.1–1 W/atom will occur under more extreme conditions for which the ultraviolet electric field E is significantly greater than e/a2 0. In this high intensity regime, a wide range of new nonlinear phenomena will be open to study. These will include the possibility of ordered driven motions in atoms, molecules, and plasmas, mechanisms involving collisions, and relativistic processes such as electron-positron pair production. An understanding of these physical interactions may provide a basis for the generation of stimulated emission in the x-ray range.
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Rhodes, C.K. (1987). Ordered Many-Electron Motions in Atoms and X-Ray Lasers. In: Connerade, J.P., Esteva, J.M., Karnatak, R.C. (eds) Giant Resonances in Atoms, Molecules, and Solids. NATO ASI Series, vol 151. Springer, Boston, MA. https://doi.org/10.1007/978-1-4899-2004-1_34
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