Abstract
Results are presented of a systematic investigation of generation of the second optical harmonic in molecular crystals of organic compounds. The effect of frequency doubling of emission from ruby and neodymium-glass lasers in the powders of 300 organic substances of various classes is studied. Linear and nonlinear optical properties of single crystals of m-dinitrobenzene and m-toluenediamine are investigated. Generation of the second optical harmonic is correlated with the molecular and crystal structures of organic compounds.
Based on material of a dissertation for the degree of Doctor of Physicomathematical Sciences. The advisors were Academician A. M. Prokhorov and Candidate of Physicomathematical Sciences G. P. Shipulo. The dissertation was defended February 16, 1976 at the P. N. Lebedev Physics Institute of the Academy of Sciences of the USSR.
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Literature Cited
S. A. Akhmanov and R. V. Khokhlov, Problems in Nonlinear Optics [in Russian], VINITI, Moscow (1964).
P. A. Franken, A. E. Hill, C. W. Peters, and G. Weinreich, Phys. Rev. Lett., 7:118 (1961).
V. S. Suvorov and A. S. Sonin, Kristallografiya, 11:832 (1966).
A. I. Kitaigorodskii, Molecular Crystals [in Russian], Nauka, Moscow (1971).
G. V. Bokii, Crystal Chemistry [in Russian], Izd. Mosk. Gos. Univ. (1960).
A Short Chemical Encyclopedia [in Russian], Soy. Éntsikl., Moscow (1964).
Y. Okaya and R. Pepinsky, Acta. Crystallogr., 10:324 (1957).
W. Nowacki and H. Jaggi, Z. Kristallogr., 109:272 (1957).
T. Penkalya, Outlines of Crystal Chemistry [in Russian], Khimiya, Leningrad (1974).
J. Donohue and A. Caron, Acta Crystallogr., 17:663 (1964).
K. Hirayama, Handbook of UV and Visible Absorption Spectra of Organic Compounds, Plenum Press, New York (1971).
A. N. Winchell, The Optical Properties of Organic Compounds, Academic Press, New York (1954).
I. S. Rez, Kristallografiya, 5:63 (1960).
W. Nowacki, Am. Cryst. Assoc. Monograph, Vol. 6 (1967).
R. Yu. Orlov, Candidate’s thesis, Mosk. Gos. Univ. (1964).
K. E. Rieckhoff and W. L. Peticolas, Science, 147:610 (1965).
P. M. Rentzepis and Y. H. Pao, Appl. Phys. Lett., 5:156 (1964).
G. H. Heilmeier, N. Ockman, R. Braunstein, and D. A. Kramer, Appl. Phys. Lett., 5:229 (1964).
Éksp.A. A. Filimonov, V. S. Suvorov, and I. S. Rez, Zh. Éksp. Teor. Fiz, 56:1519 (1969).
S. K. Kurtz and T. T. Perry, J. Appl. Phys., 39:3798 (1968).
A. Graja, Phys. Status Solidi, 27:K93 (1968);
A. Graja, Acta. Phys. Pol., A37:539 (1970).
S. A. Akhmanov and A. S. Chrikin, Statistical Phenomena in Nonlinear Optics [in Russian], Izd. Mosk. Gos. Univ. (1971).
J. R. Gott, M. J. P. Musgrave, and J. N. Murrett, Mol. Phys., 12:295 (1967).
R. Yu. Orlov, Kristallografiya, 11:463 (1966).
A. A. Filimonov, V. S. Suvorov, R. I. Rez, et al., Proc. Fourth All-Union Symp. on Non-linear Optics [in Russian], Kiev (1968).
M. Bass, D. Bua, R. Mozzi, and R. Monchamp, Appl. Phys. Lett., 15:393 (1969).
L. D. Derkacheva, A. I. Krymova, and N. P. Sonina, Pis’ma Zh. Éksp. Teor. Fiz., 11:469 (1970).
B. L. Davydov, L. D. Derkacheva, V. V. Dunina, et al., Pis’ma Zh. Éksp. Teor. Fiz., 12:24 (1970).
J. P. Hazan and J. Haisma, Opt. Commun., 2:343 (1970).
B. L. Davydov, L. D. Derkacheva, V. V. Dunina, et al., Opt. Spektrosk., 30:503 (1971).
J. Jerphagnon, IEEE J. Quant. Electron, QE-7:42 (1971).
E. A. Tikhonov and M. T. Shpak, Ukr. Fiz. Zh., 17:190 (1972).
B. L. Davydov, V. F. Zolin, L. G. Koreneva, et al., Zh. Prikl. Spektrosk., 17:413 (1972).
G. P. Bolognesi, S. Mezzetti, and F. Pandarese, Opt. Commun., 8:267 (1973).
B. L. Davydov, V. F. Xolin, L. G. Koreneva, et al., Zh. Prikl. Spektrosk., 20:516 (1974).
L. G. Koreneva, B. L. Davydov, M. E. Zhabotinskii, and V. F. Zolin, IRÉ Preprint No. 105, Moscow (1972).
B. L. Davydov, V. V. Dunina, V. F. Zolin, and L. G. Koreneva, Opt. Spektrosk., 34:267 (1973).
B. L. Davydov, V. V. Dunina, V. F. Zolin, et al., Opt. Spektrosk., 32:225 (1972).
B. L. Davydov, L. G. Koreneva, and M. A. Samokhina, IRE Preprint No. 104, Moscow (1972).
B. L. Davydov, V. F. Zolin, L. G. Koreneva, and M. A. Samokhina, Zh. Priki. Spektrosk., 18:156 (1973).
K. Ito, Y. Kusuhara, K. Hamano, and S. Sawada, Jpn. J. Appl. Phys., 13:1299 (1974).
P. D. Southgate and D. S. Hall, J. App. Phys., 42:4480 (1971).
P. D. Southgate and D. S. Hall, J. Appl. Phys., 43:2765 (1972).
J. G. Bergman, G. R. Crane, B. F. Levine, and C. G. Bethea, Appl. Phys. Lett., 20:21 (1972).
S. Singh, W. A. Bonner, T. Kyle, et al., Opt. Commun., 5:131 (1972).
W. A. Norland, Ferroelectrics, 2:57 (1971).
B. F. Levine and C. G. Bethea, Appl. Phys. Lett., 20:272 (1972).
J. Jerphagnon, Appl. Phys. Lett., 16:298 (1970).
J. R. Gott, J. Phys., B4:116 (1971).
B. L. Davydov, L. G. Koreneva, and E. A. Lavrovskii, Radiotekh. Élektron., No. 6:1313 (1974).
P. D. Southgate and D. S. Hall, Appl. Phys. Lett., 18:456 (1971).
N. A. Vlasenko, B. L. Davydov, and L. G. Koreneva, Izv. Vyssh. Uchebn. Zaved., Radio-fiz., 16:363 (1973).
M. V. Hobden, J. Appl. Phys., 38:4365 (1967).
R. Yu. Orlov, Izv. Vyssh. Uchebn. Zaved., Radiofiz. 12:1351 (1969).
B. L. Davydov, M. E. Zhabotinskii, and V. F. Zolin, Pis’ ma Zh. Éksp. Teor. Fiz., 13:336 (1971).
N. L. Boling, M. J. Crisp, and G. Dube, Appl. Opt., 12:650 (1973).
F. N. H. Robinson, Bell System Tech. J., 46:913 (1967).
F. Lebon, Phys. Status Solidi, 41:297 (1970).
L. G. Koreneva, V. F. Zolin, and B. L. Davydov, Molecular Crystals in Nonlinear Optics, [in Russian], Nauka, Moscow (1975).
S. J. Syvin, J. E. Rauch, and J. C. Decius, J. Chem. Phys., 43:4083 (1965).
V. D. Shigorin and G. P. Shipulo, Kratk. Soobshch. Fiz., No. 5, p. 59 (1970).
V. D. Shigorin and G. P. Shipulo, Kratk. Soobshch. Fiz., No. 11, p. 31 (1970).
V. D. Shigorin and G. P. Shipulo, Kratk. Soobshch. Fiz., No. 10, p. 34 (1971).
V. K. Bel’skii and P. M. Zorkii, Kristallografiya, 15:704 (1970).
A. V. Voskanyan, D. N. Klyshko, and V. S. Tumanov, Zh. Éksp. Teor. Fiz., 45:1399 (1963).
Éksp.G. L. Gurevich and Yu. G. Khronopulo, Zh. Éksp. Teor. Fiz., 51:1497 (1966).
V. D. Shigorin and G. P. Shipulo, Kvantovaya Élektron., No. 4, p. 116 (1972).
Landolt-Bornstein, New Series, Group III, Vol. 5, Parts a, b, Springer-Verlag, Berlin-Heidelberg-New York (1971).
A. Hettichand and H. Steinmetz, Z. Phys., 76:688 (1932).
V. A. Koptsik, K. A. Minaeva, A. A. Voronkov, et al., Vestn. Mosk. Gos. Univ., 6:91 (1958).
I. S. Rez, A. S. Sonin, E. E. Tsepelevich, and A. A. Filimonov, Kri stallogr afiya, 4:65 (1959).
Shok Le Nguen and G. A. Gol’der, Zh. Strukt. Khim., 11:939 (1970).
L. A. Chetkina, O. A. Mukhno, and Z. I. Ezhkova, Zh. Strukt. Khim., 12:187 (1971).
H. Ranin, Radiat. Effects, 4:167 (1970).
T. P. Belikova and E. A. Sviridenkov, Pis’ma Zh. Éksp. Teor. Fiz., 5:29 (1967).
I. I. Konilenko, P. A. Korotkov, and V. I. Malyi, in: Quantum Electronics, No. 3 [in Russian], Naukova Dumka, Kiev (1969), p. 120.
V. D. Shigorin and G. P. Shipulo, Kristallografiya, 18:557 (1973).
V. D. Shigorin and G. P. Shipulo, Kristallografiya, 19:1006 (1974).
A. Coda, M. Fumagalli, F. Pandarese, and L. Ungaretti, Acta. Crystallogr., A31:S208 (1975).
V. E. Zavodnik, Z. P. Povet’eva, and Z. V. Zvonkova, Kristallografiya, 20:839 (1975).
D. Kalymnios, J. Phys., D5:667 (1972).
S. Ayers, M. M. Faktor, D. Marr, and J. L. Stevenson, J. Mater. Sci., 7:31 (1972).
J. L. Syeveson and A. C. Skapski, J. Phys., C5:L233 (1972).
J. L. Steveson, S. Ayers, and M. M. Faktor, J. Phys. Chem. Solids, 34:235 (1973).
J. L. Steveson, J. Phys., D6:L13 (1973).
G. S. Belikova, M. P. Golovei, V. D. Dhigorin, and G. P. Shipulo, in: Proc. Sixth All Union Conf. on Nonlinear Optics [in Russian], Minsk (1972), p. 55.
G. S. Belikova, M. P. Golovei, V. D. Shigorin, and G. P. Shipulo, Krat. Soobshch. Fiz., No. 6, p. 24 (1973).
G. S. Belikova, M. P. Golovei, V. D. Shigorin, and G. P. Shipulo, Opt. Spektrosk., 38: 779 (1975).
S. S. Grazhulene, L. A. Musikhin, V. Sh. Shekhtman, et al., in: Proc. Seventh All-Union Conf. on Coherent and Nonlinear Optics [in Russian], Moscow (1974), p. 30.
V. D. Shigorin, G. I. Shipulo, S. S. Grazhulene, et al., Kvantovaya Élektron., 2:2539 (1975).
E. M. Archer, Proc. Roy. Soc., A188:51 (1946).
K. Nakamoto, J. Am. Chem. Soc., 74:392 (1952).
J. Trotter, Acta Crystallogr., 14:244 (1961).
G. S. Belikova, L. E. Kraeva, and V. D. Shigorin, Inventor’s Certificate No. 459956, Byull. Izobr., No. 5 (1975).
S. S. Grazhulene, L. A. Musikhin, G. F. Telegin, and V. D. Shigorin, Inventor’s Certificate No. 496043, Byull. Izobr., No. 47 (1975).
J. Trotter and C. S. Williston, Acta Crystallogr., 21:285 (1966).
O. S. Filipenko, V. I. Ponomarev, V. D. Shigorin, et al., Kristallografiya, 20:937 (1975).
S. V. Grum-Grzhimailo, Instruments and Methods for Optical Investigation of Crystals [in Russian], Nauka, Moscow (1972).
I. S. Rez, Usp. Fiz. Nauk, 93:633 (1967).
A. V. Shubnikov, Fundamentals of Optical Crystallography [in Russian], Izd. Akad. Nauk. SSSR, Moscow (1958).
N. M. Melankholin, Methods for Investigating Optical Properties of Crystals [in Russian], Nauka, Moscow (1970).
L. S. Khrenov, Seven-Place Tables of the Trigonometric Functions [in Russian], Gos. Izd. Tekh. Teor. Lit., Moscow (1956).
W. L. Bond, J. Appl. Phys., 36:1674 (1965).
M. N. Datta, Indian J. Phys., 21:303 (1947).
M. A. Lasheen and A. M. Abdeen, Acta. Crystallogr., A28:245 (1972).
P. D. Maker, R. W. Terhune, M. Nisenoff, and C. M. Savage, Phys. Rev. Lett., 8:21 (1962).
J. Jerphagnon and S. K. Kurtz, J. Appl. Phys., 41:1667 (1970).
Y. Uematsu, Jpn. J. Appl. Phys., 12:1257 (1973).
G. E. Francois, Phys. Rev., 143:597 (1966).
A. Savage, J. Appl. Phys., 36:1496 (1965);
G. D. Boyd, H. Kasper, and J. H. McFee, IEEE J. Quant. Electron., 7:563 (1971).
D. A. Kleinman, Phys. Rev., 126:1977 (1965).
R. C. Miller, Appl. Phys. Lett., 5:17 (1964).
V. D. Shigorin and G. P. Shipulo, Kvantovaya Elektron., 3:2048 (1976).
H. E. Bates, J. Opt. Soc. Am., 63:146 (1973).
B. V. Bokut’, Zh. Prikl. Spektrosk., 7:621 (1967).
B. L. Davydov, V. F. Zolin, L. G. Koeneva, and E. A. Lavrovskii, Opt. Spektrosk., 39:713 (1975).
H. Ito, H. Naito, and H. Inaba, IEEE J. Quant. Electron., 10:247 (1974).
A. I. Kovrigin, N. K. Podsotskaya, and A. P. Sukhorukov, in: Nonlinear Optics [in Russian], Nauka, Novosibirsk (1968), p. 393.
G. D. Boyd and D. A. Kleinman, J. Appl. Phys., 39:3597 (1968).
G. S. Belikova, L. A. Kulevsky, Yu. N. Polivanov, et al., J. Raman Spectrosc., 2:493 (1974).
G. S. Belikova, S. S. Grazhulene, L. M. Doroshkin, et al., in: Proc. Eighth All-Union Conf. on Coherent and Nonlinear Optics, Vol. 1 [in Russian], Izd.“Metsniereba,” Tbilisi (1976), p. 229.
J. Ducuing and C. Flytzanis, in: Optical Properties of Solids, F. Abeles, ed., Amsterdam (1972), p. 863.
V. D. Shigorin and G. P. Shipulo, in: Proc. Sixth All-Union Conf. on Nonlinear Optics [in Russian], Minsk (1972), p. 19.
V. D. Shigorin and G. P. Shipulo, Opt. Spektrosk., 34:151 (1973).
N. Bloembergen, Nonlinear Optics, Benjamin, New York (1965).
C. G. B. Garrett, IEEE J. Quant. Electron., 4:70 (1968).
K. Higasi, H. Baba, and A. Rembaum, Quantum Organic Chemistry, Interscience, New York (1965).
A. D. McLachlan, Mol. Phys., 2:271 (1959).
V. D. Shigorin and G. P. Shipulo, Zh. Prikl. Spektrosk., 20:720 (1974).
R. S. Mulliken, J. Chem. Phys., 7:20 (1939).
H. Ratajczak, J. Phys. Chem., 76:3000, 3991 (1972).
S. Nagakura, M. Kojima, and Y. Marugama, J. Mol. Spectrosc., 13:174 (1974).
H. Suzuki, Electronic Absorption Spectra and Geometry of Organic Molecules, Academic Press, New York-London (1967).
M. Godfrey and J. N. Murrell, Proc. Roy. Soc., A278:71 (1964).
G. V. Saidov and N. G. Bakhshiev, Dokl. Akad. Nauk SSSR, 175:1090 (1967).
V. I. Danilova, Author’s Abstract of Doctoral Dissertation, Tomsk (1969).
S. Kobinata and S. Nagakura, J. Am. Chem. Soc., 88:3905 (1966).
J. L. Oudar and D. S. Chemla, Opt. Commun., 13:164 (1975).
J. Jerphagnon, Phys. Rev., B2:1091 (1970).
C. N. R. Rao, Ultraviolet and Visible Spectroscopy: Chemical Applications, Plenum Press, New York (1967).
K. B. Everard and L. E. Sutton, J. Chem. Soc., 2821 (1951).
L. Doub and J. M. Vandenbelt, J. Am. Chem. Soc., 69:2714 (1947).
B. F. Levine and C. G. Bethea, Appl. Phys. Lett., 24:445 (1974).
C. Flytzanis and J. Ducuing, Phys. Rev., 178:1218 (1969).
L. B. Meisner, Fiz. Tverd. Tela, 14:2220 (1972).
D. A. Dunmur, Mol. Phys., 23:109 (1972).
D. D. Karov, S. N. Koikov, and M. N. Rogova, Fiz. Tverd. Tela, 15:594 (1973).
G. E. Bacon and N. A. Curry, Proc. Roy. Soc., A235:552 (1956).
A. T. McPhail and G. A. Sim, J. Chem. Soc., 227 (1965).
V. I. Ponomarev, O. S. Filipenko, L. O. Atovmyan, et al., Kristallografiya, 22:394 (1977).
O. S. Filipenko, V. D. Shigorin, V. I. Ponomarev. et al., Kristallografiya, 22:534 (1977).
A. Schweig, Chem. Phys. Lett., 1:195 (1967).
P. Skrabal, J. Steiger, and H. Zollinger, Helv. Chim. Acta, 58:800 (1975).
Handbook of Dipole Moments [in Russian], “Vysshaya shkola,” Moscow (1971).
P. P. Shorygin, Usp. Khim., 40:694 (1971).
P. P. Shorygin, V. P. Roshchupkin, V. A. Petukhov, and Z. S. Egorova, Zh. Fiz. Khim., 35:258 (1961).
Ya. S. Bobovich and M. V. Vol’kenshtein, Dokl. Akad. Nauk SSSR, 71:1045 (1950).
Ya. S. Bobovich and M. Ya. Tsenter, Opt. Spektrosk., 8:45 (1960).
V. I. Minkin, O. A. Osipov, and Yu. A. Zhdanov, Dipole Moments in Organic Chemistry, Plenum Press, New York (1970).
A. Domenicano, A. Vaciago, and C. A. Coulson, Acta Crystallogr., B31:221 (1975).
R. W. Wyckoff, in: Crystal Structures, Vol. 6, Parts 1, 2, Interscience, New York-London (1971).
V. A. Koptsik, Izv. Akad. Nauk SSSR, Ser. Fiz., 20:219 (1956).
I. S. Zheludev, Kristallografiya, 2:90 (1957).
G. V. Boikii and M. A. Porai-Koshits, A. Practical Course in X-ray Analysis [in Russian], Izd. Mosk. Gos. Univ., Moscow (1951).
I. S. Rez, P’ezotekhnika, No. 1, p. 3 (1959).
B. V. Tul’skii, Zh. Strukt. Khim., 6:304 (1965).
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Shigorin, V.D. (1982). Investigation of Generation of the Second Optical Harmonic in Molecular Crystals. In: Basov, N.G. (eds) Materials and Apparatus in Quantum Radiophysics. The Lebedev Physics Institute Series / Materialy i Ustroistva Kvantovoi Radiofiziki / Matepиaлы и Уctpoйctba Кbaнtoboй Paдиoфизики. Springer, Boston, MA. https://doi.org/10.1007/978-1-4757-5788-0_3
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