Abstract
In a vibrating lattice, the effective force between two ions consists of (i) the direct ion-ion interaction and (ii) the interaction via mediating electrons. The electronic contribution to the lattice dynamics is very important in many classes of crystals spanning from metals to insulators. The electronic contribution in simple metals has been fairly satisfactorily treated by the method of pseudopotentials, essentially treating the electrons as nearly free. However, there remains an enormous class of transition metals, their compounds, covalent and ionic crystals, in which there are important electrons which are not nearly free nor yet so tightly bound so as to be moving rigidly with the ion. In section 2 we shall describe a method which takes into account the effects of these electrons on the lattice dynamics.
Research supported by the National Science Foundation, Grant No. GP-28997.
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Sham, L.J. (1974). Electronic Influence on Lattice Dynamics. In: Devreese, J.T., Kunz, A.B., Collins, T.C. (eds) Elementary Excitations in Solids, Molecules, and Atom. NATO Advanced Study Institutes Series, vol 2. Springer, Boston, MA. https://doi.org/10.1007/978-1-4684-2823-0_1
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