Abstract
Semiconductor quantum dots are often referred to as artificial atoms because the electronic energy spectrum is determined by the effects of quantum mechanical confinement and interactions [1]. Zero-dimensional (0D) energy levels are well defined in a sufficiently small dot that the size of the confining potential is comparable to the Fermi wavelength of electrons. On the other hand, the interaction effect is characterized by a Coulombic energy (single electron charging energy) cost for trapping an additional electron in a dot. The charging energy is simply given by e 2 /C (C, total capacitance) when the dot is large enough for containing many electrons. This gives rise to so-called “Coulomb blockade” and is explained using an orthodox theory [2]. However, when the dot is small and contains just a few electrons, the interaction effect as well as the quantum mechanical effect depends strongly on the electronic configuration, and cannot be characterized using a capacitance model [2,3]. Adding an electron to such a small quantum dot costs a certain energy and simultaneously changes the electronic configuration to minimize the total energy, i.e. sum of the quantum mechanical energy and interaction energy. The cost for the quantum mechanical energy is associated with the orbital energy. Each orbital state is spin degenerate, so antiparallel spin filling of the same orbital state is generally favored. However, this is not the case when we consider the cost of interaction energy. Exchange energy is gained when electrons are added with parallel spins as compared to antiparallel spins.
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Tarucha, S., Ono, K., Fujisawa, T., van DerWiel, W.G., Kouwenhoven, L.P. (2003). Interactions, Spins and the Kondo Effect in Quantum-Dot Systems. In: Bird, J.P. (eds) Electron Transport in Quantum Dots. Springer, Boston, MA. https://doi.org/10.1007/978-1-4615-0437-5_1
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DOI: https://doi.org/10.1007/978-1-4615-0437-5_1
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