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Modelling the Deposition of Reduced Nitrogen at Different Scales in the United Kingdom

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Air Pollution Modeling and Its Application XIX

Abstract

A national scale atmospheric transport model (FRAME) was applied to the UK to generate maps of ammonia concentration and the wet and dry deposition of reduced nitrogen. The model was found to give satisfactory agreement with measurements from the national monitoring networks of ammonia and ammonium aerosol concentrations and wet deposition of ammonium. Scatter in the model correlation with measurements of ammonia concentration was observed due to the strong sub-model grid (5 km) variation in ammonia concentration. Application of a local dispersion model to calculate ammonia concentrations emitted from a typical poultry unit showed that areas of high concentration were restricted to a 1 km2 area surrounding the point source. FRAME showed good overall agreement with the EMEP model for national average levels of ammonia concentration and reduced nitrogen deposition. However, a difference in spatial patterns of wet deposition occurred due to the different treatment of precipitation in the two models. It was concluded that finer resolution national scale modelling of reduced nitrogen is required in order to improve estimates of critical loads exceedance for acid deposition and nutrient nitrogen deposition.

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References

  • Dore AJ, Vieno M, Fournier N, Weston KJ, Sutton MA (2006a) Development of a new wind rose for the British Isles using radiosonde data and application to an atmospheric transport model. Quart. J. Roy. Met. Soc., 132, 2769-2784.

    Article  Google Scholar 

  • Dore AJ, Mousavi-Baygi M, Smith RI, Hall J, Fowler D, Choularton TW (2006b) A Model of Annual Orographic Precipitation and Acid Deposition and its application to Snowdonia. Atmos. Environ., 40, 3316-3326.

    Article  CAS  Google Scholar 

  • Dore AJ, Vieno M, Tang YS, Dragosits U, Dosio A, Weston KJ, Sutton MA (2007) Modelling the atmospheric transport and deposition of sulphur and nitrogen over the United Kingdom and assessment of the influence of SO2 emissions from international shipping. Atmos. Environ., 41, 2355-2367.

    Article  CAS  Google Scholar 

  • Dragosits U, Theobald MR, Place CJ, Lord E, Webb J, Hill J, ApSimon HM, Sutton MA (2002) Ammonia emission, deposition and impact assessment at the field scale: a case study of sub-grid spatial variability. Environ. Pollut., 117, 147-158.

    Article  CAS  Google Scholar 

  • Fournier N, Weston KJ, Dore AJ, Sutton MA (2005a) Modelling the wet deposition of reduced nitrogen over the British Isles using a Lagrangian multi-layer atmospheric transport model. Quart. J. Roy. Met. Soc., 131, 703-722.

    Article  Google Scholar 

  • Fournier N, Tang YS, Dragosits U, Kluizenaar Y, Sutton MA (2005b) Regional atmospheric budgets of reduced nitrogen over the British Isles assessed using an atmospheric transport model. Water, Air Soil Pollut., 162, 331-351.

    Article  CAS  Google Scholar 

  • Fowler D, Smith RI, Muller JBA, Hayman G, Vincent KJ (2005) Changes in the atmospheric deposition of acidifying compounds in the UK between 1986 and 2001. Environ. Pollut., 137, 15-25.

    Article  CAS  Google Scholar 

  • NEGTAP (2001) Transboundary Air Pollution: Acidification, Eutrophication and Ground Level ozone in the UK. Report of the National Expert Group on Transboundary Air Pollution, DEFRA, London.

    Google Scholar 

  • Singles RJ, Sutton MA, Weston KJ (1998) A multi-layer model to describe the atmospheric transport and deposition of ammonia in Great Britain. Atmos. Environ., 32, 393-399.

    Article  CAS  Google Scholar 

  • Sutton MA, Tang YS, Miners B, Fowler D (2001) A new diffusion denuder system for long-term, regional monitoring of atmospheric ammonia and ammonium. Water, Air Soil Pollut.: Focus, 1, 145-156.

    Article  CAS  Google Scholar 

  • Tang YS, Cape JN, Sutton MA (2001) Development and types of passive samplers for monitoring atmospheric NO2 and NH3 concentrations. TheScientificWorld, 1, 513-529.

    Article  CAS  Google Scholar 

  • Tarrasón L, Fagerli H, Eiof Jonson J, Klein H, van Loon M, Simpson D, Tsyro S, Vestreng V, Wind P, Posch M, Solberg S, Spranger T, Cuvelier K, Thunis P, White L (2003) Transboundary Acidification, Eutrophication and Ground Level Ozone in Europe. PART I Unified EMEP Model description. EMEP Status Report 2003.

    Google Scholar 

  • Vieno M (2005) The use of an Atmospheric Chemistry-Transport Model (FRAME) over the UK and the development of its numerical and physical schemes. Ph.D. thesis, University of Edinburgh, Edinburgh.

    Google Scholar 

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Dore, A.J., Theobald, M.R., Kryza, M., Vieno, M., Tang, S.Y., Sutton, M.A. (2008). Modelling the Deposition of Reduced Nitrogen at Different Scales in the United Kingdom. In: Borrego, C., Miranda, A.I. (eds) Air Pollution Modeling and Its Application XIX. NATO Science for Peace and Security Series Series C: Environmental Security. Springer, Dordrecht. https://doi.org/10.1007/978-1-4020-8453-9_14

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