Abstract
The complex structure-property relationships in the disordered systems under normal and exogenic conditions can be understood after characterizing the spatial arrangement of constituents. Here, an integral approach including the relevant experimental technique, phenomenological, and theoretical analyses as well as atomistic modeling is presented. Application of such a combined approach is demonstrated for the cases of glycerol and propylene glycol.
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References
Brandt, W. and Dupasquier, A. (eds.) (1983) Positron Solid State Physics, North- Holland, Amsterdam.
Jean, Y.C. (1995) Characterizing free volume and holes in polymers by positron annihilation spectroscopy in Dupasquer, A. (ed.) Positron Spectroscopy of Solids, IOS, Ohmsha, Amsterdam, p. 563.
Bartoš, J. (2000) Positron annihilation spectroscopy of polymers and rubbers in R.A. Meyers (eds.) Encyclopedia of Analytical Chemistry, Wiley & Sons, Chichester, p. 7968.
Jean, Y.C., Mallon, P.E., and Schrader, D.M. (eds.) (2003) Principles and Applica-tions of Positron & Positronium Chemistry, World Scientific Publ., Ne rsey. w Je
Bartoš, J., Šauša, O., and Krištiak, J. Annihilation response of the ortho-positronium probe from positron annihilation lifetime spectroscopy and its relationships to the free volume and dynamics of glass-forming systems in ARW NATO Series: Nonlinear Dielectric Phenomena in Complex Liquids, Kluwer, Acad. Publ., Dordrecht, The Netherlands, p. 289.
Bartoš, J., Šauša, O., Krištiak, J., Blochowicz, T., and Rössler, E. (2001) J. Phys.- Cond. Matter 13, 11473.
Šauša, O., Bartoš, J., and Krištiak, J. to be published.
Bartoš, J., Šauša, O., Bandžuch, P., Zrubcová, J., and Krištiak, J. (2002) J. Non-Cryst. Solids 307 -310,417.
Kovacs, A. (1963) Adv. Polym. Sci. 3, 394.
Parks, G.S. and Huffman, H.M. (1927) J. Phys. Chem. 11, 1842.
Angell, C.A. (1985) Strong and fragile liquids in Ngai, K., Wright, G.S. (eds.) Relaxations in Complex Systems, NTIS, Springfield, p. 1.
Leon, C., Ngai, K., and Roland, C.M. (1999) J. Chem. Phys. 110, 11585.
Pawlus, S., Bartoš, J., Šauša, O., Krištiak, J., and Paluch, M. (2005) J. Chem. Phys. 124, 104505.
Lunkenheimer, P. and Loidl, A. (2002) Chem. Phys. 284, 205.
Donth, E., The Glass Transition, Springer, Berlin, 2001.
Bartoš, J., Šauša, O., Raþko, D., Krištiak, J., and Fontanella, J.J. (2005) J. Non-Cryst. Solids 351, 2599.
Stickel, F.J. (1995) Ph.D. Thesis, Shaker-Verlag, Aachen.
Schönhals, A. (2001) Europhys. Letts. 56, 815.
Tao, J. (1972) J. Chem. Phys. 56, 5499; Eldrup, M., Lightbody, D., Sherwood, J.N. (1981) Chem. Phys. 63, 51; Nakanishi, H., Wang, S.J., and Jean, Y.C. (1988) in S.C. Sharma (eds.), Positron Annihilation Studies of Fluids, World Science, Singapore, p. 292.
Goworek, B. (1999)Acta Phys. Polonica A 95, 557; Olson, B.G., Prodpran, T., and Jamieson, A.M., Nazarenko, S. (2002) Polymer43, 6775.
Consolati, G. (2002) J. Chem. Phys. 117, 7279.
Cohen, M.H. and Grest, G.S. (1979) Phys. Rev. B20,1077; Grest, G.S., and Cohen, M.H. (1980) Phys. Rev. B21, 4113; Grest, G.S. and Cohen,M.H. (1981) Adv. Chem. Phys. 48, 455.
Procacci, P., Darden, T.A., Paci, E., and Marchi, M. (1996) J. Phys. Chem. 100, 10464.
Raþko, D., Chelli, R., Bartoš, J., Cardini, G. and Califano, S. (2005) Eur. Phys. J. E32, 289.
Angell, C.A., and Wang, L.M. (2003) Biophys. Chem. 105, 621.
Sastry, S., Truskett, T.M., Debenedetti, P.G., Torquato, S., and Stillin ger, F.H. (1998) Mol. Phys. 95, 289.
McCullagh, C.M., Yu, Z., Jamiesson, A.M., Blackwell, J. and McGervey, J.D. (1995) Macromole cules 28, 6100; Yu, Z. (1995) Ph.D. thesis, Case Western Reserve University, Cleveland, OH.
Götze, W., and Sjörgen, L., (1992) Rep. Progr. Phys. 55, 241.
Paluch, M., Casalini, R., and Roland, C.M. (2003) Phys. Rev. E67, 021508.
Novikov, V.N., and Sokolov, A.P. (2003) Phys. Rev. E67, 031507.
Adichtchev, S., Blochowicz, T., Tschirwitz, Ch., Novikov, V.N., and Rössler, E.A. (2003) Phys. Rev. E68, 011504.
Götze, W. (1999) J. Phys.-Cond. Matt. 11, A1.
Ngai, L.K. (1979) Comment Solid State Phys. 9, 127; Ngai, K.L., Rendell, R.W. (1997) in Fourkas, J.T., Kivelson, D., Mohanty, U., and Nelson, K. (eds.)Super- cooled Liquids. Advances and Novel Applications, ACS Symposium Series, Vol. 676 Amer. Chem. Soc. Washington, DC p. 45.
Casalini, R., Ngai, K.L., and Roland, C.M. (2003) Phys. Rev. B68, 014201.
Ngai, K.L., and Paluch, M. (2004) J. Chem. Phys. 120, 857.
Ngai, K.L. (2005) J. Non-Cryst. Solids 351, 2635.
Ngai, K.L., Lunkenheimer, P., Leon, C., Scheneider, U., Brand, R., and Loidl, A. (2001) J. Chem. Phys. 115, 1405.
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Bartoš, J., Račko, D., Šauša, O., Krištiak, J. (2007). Positron annihilation lifetime spectroscopy and atomistic modeling – effective tools for the disordered condensed systems characterization. In: Rzoska, S.J., Mazur, V.A. (eds) Soft Matter under Exogenic Impacts. NATO Science Series II: Mathematics, Physics and Chemistry, vol 242. Springer, Dordrecht. https://doi.org/10.1007/978-1-4020-5872-1_7
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DOI: https://doi.org/10.1007/978-1-4020-5872-1_7
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