Neutron Scattering of Magnetic Materials

  • Olivier Isnard


Neutron scattering is a comprehensive tool for condensed matter research. After a brief description of the interaction of neutrons with matter, the usefulness of neutrons to probe the physical properties of magnetic materials is illustrated using examples taken from different research areas. Then a description of the crystal structure investigation, including in situ and time-resolved studies is given. The use of polarized or unpolarized neutrons to study magnetic structures or magnetic phase transition is also illustrated. The potential of techniques such as small-angle neutron scattering or neutron scattering on magnetic surfaces is presented showing that neutron scattering now offers a wide range of useful techniques to probe the structural and magnetic properties of magnetic materials whatever their state: polycrystalline, single crystal, amorphous, bulk, or thin films. Examples are taken from a wide range of research fields: hard magnetic materials, nanocomposite soft magnets, multilayers, superlattices, geometrically frustrated magnetic materials, etc. The experimental aspects are not covered in detail but relevant references are given throughout the chapter.


Neutron Diffraction Neutron Scattering Magnetic Phase Transition Inelastic Neutron Neutron Diffraction Pattern 
These keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.


  1. 1.
    Chadwick J.: Possible existence of a neutron. Nature (London) 129  312 (1932).Google Scholar
  2. 2.
    Chadwick J.: Existence of a neutron. Proc. Roy. Soc. London Ser. A 136  692–708 (1932).CrossRefGoogle Scholar
  3. 3.
    Bacon G. E.: Neutron Diffraction. Clarendon Press, Oxford (1975).Google Scholar
  4. 4.
    Bacon G. E.: Fifty Years of Neutron Diffraction: the Advent of Neutron Scattering. Adam Hilger, Bristol (1986).Google Scholar
  5. 5.
    Lovesey S. W., Springer T.: Dynamic of Solids and Liquids by Neutron Scattering, Topics in Current Physics, Vol. 3. Springer-Verlag, Berlin (1977).CrossRefGoogle Scholar
  6. 6.
    Squires G. L.: Introduction to the Theory of Thermal Neutron Scattering. Cambridge University Press, Cambridge (1978).Google Scholar
  7. 7.
    Williams, W. G.: Polarized Neutrons. Clarendon Press: Oxford (1988).Google Scholar
  8. 8.
    Willis B. T.: Chemical Application of Thermal Neutron Scattering. Oxford University Press, Oxford (1973).Google Scholar
  9. 9.
    Chatterji T.: Neutron Scattering from Magnetic Materials. Elsevier B.V., Amsterdam (2006).Google Scholar
  10. 10.
    Izyumov Yu. A., Naish V. E., Ozerov R. P.: Neutron Diffraction of Magnetic Materials. Consultant Bureau, Plenum Pub. New York (1991).CrossRefGoogle Scholar
  11. 11.
    Bloch F.: On the Magnetic Scattering of Neutrons. Phys. Rev. B 50  259 (1936).Google Scholar
  12. 12.
    Schull C. G., Smart J. S.: Detection of Antiferromagnetism by Neutron Diffraction. Phys. Rev. 76 1256–1 (1949).CrossRefGoogle Scholar
  13. 13.
    Néel L.:  Influence des fluctuations du champ moléculaire sur les propriétés magnétique des corps. Ann. Phys. (Paris) 17 5–105 (1932).Google Scholar
  14. 14.
    Néel L.: Propriétés magnétiques des ferrites ferrimagnétisme et Antiferromagéntisme. Ann. Phys. (Paris) 3  137–198 (1948).Google Scholar
  15. 15.
    Baruchel J., Hodeau J. L., Lehmann M. S., Regnard J. R., Schlenker C.: Neutron and Synchrotron Radiation for Condensed Matter Studies, Vol. I: Theory, Instruments and Methods. Springer-Verlag, Berlin (1993).Google Scholar
  16. 16.
    Baruchel J., Hodeau J. L., Lehmann M. S., Regnard J. R., Schlenker C.: Theory, Instruments and Methods, Vol. II: Applications to Solid State Physics and Chemistry. Springer-Verlag, Berlin (1994).Google Scholar
  17. 17.
    Scherm R., Fak B.: Neutrons in Baruchel. J. Hodeau, J. L. Lehmann, M. S. Regnard, J. R. Schlenker (eds.) Neutron and Synchrotron Radiation for Condensed Matter Studies, Vol. I: Theory, Instruments and Methods, Springer-Verlag, Berlin (1993).Google Scholar
  18. 18.
    Brückel T., Heger G., Richter D., Zorn R. (Eds.): 5th Laboratory Course Neutron Scattering, Schriften des Forschungszentrums Jülich, Vol. 9 (2001).Google Scholar
  19. 19.
    Withers P.J.: Mapping residual and internal stress in materials by neutron diffraction. C.R. Physique 8 806–820 (2007).CrossRefGoogle Scholar
  20. 20.
    Von Der Hardt P., Röttger H.: Neutron Radiography Handbook. D. Reidel, Dordrecht (1981).CrossRefGoogle Scholar
  21. 21.
    Young R. A.: The Rietveld Method. Oxford University Press, Oxford (1993)Google Scholar
  22. 22.
    Mc Intyre G.: Single Crystal diffractometry in Baruchel. J. Hodeau, J. L. Lehmann, M. S. Regnard, J. R. Schlenker, (eds.) Neutron and Synchrotron Radiation for Condensed Matter Studies, Vol. I: Theory, Instruments and Methods, Springer-Verlag, Berlin (1993).Google Scholar
  23. 23.
    Chacon C., Isnard O.: Neutron diffraction determination of the preferential substitution scheme of gallium and study of the magnetic features of the Nd2Fe14-xGaxB phases. J. Appl. Phys. 88 3570–3577 (2000).CrossRefGoogle Scholar
  24. 24.
    Chacon C., Isnard O.: Crystal and magnetic structures of the YCoxFe4-xB compounds investigated by powder neutron diffraction and magnetisation measurements. J. Appl. Phys 89 71–75 (2001).CrossRefGoogle Scholar
  25. 25.
    Marasinghe G. K., Pringle O. A., Long G. J., James W. J., Yelon W. B., Grandjean F.: A neutron diffraction and Mössbauer effect study of the magnetic structure of Y2(Fe1-xMnx)14 B. J. Appl. Phys. 70 6149–6151 (1991).Google Scholar
  26. 26.
    Isnard O., Miraglia S., Soubeyroux J. L., Fruchart D., Stergiou A.: Neutron diffraction study of the structural and magnetic properties of the R2Fe17Hx ternary compounds (R = Ce, Nd, Ho).  J. Less-Common Met. 162 273–284(1990).CrossRefGoogle Scholar
  27. 27.
    Isnard O., Miraglia S., Soubeyroux J. L., Pannetier J., Fruchart D.: Neutron powder diffraction study of Pr2Fe17 and Pr2Fe17N3. Phys. Rev. B 45 2920–2926 (1992).CrossRefGoogle Scholar
  28. 28.
    Sun H., Coey J. M. D., Otani Y., Hurley D. P. F.: Magnetic properties of a new series of rare-earth iron nitrides: R2Fe17Ny (y ∼ 2.6). J. Phys. Condens. Matter. 2 6465–6470 (1990).CrossRefGoogle Scholar
  29. 29.
    Isnard O., Soubeyroux J. L., Miraglia S., Fruchart D., Garcia L. M., Bartolomé J.: Neutron powder diffraction study of the desorption of deuterium in Nd2Fe17Dx = 5. Physica B 180–181 629–631 (1992).CrossRefGoogle Scholar
  30. 30.
    Isnard O., Soubeyroux J. L., Fruchart D., Jacobs T. H., Buschow K. H. J.: Structural and magnetic behaviour of the series Th2Fe17Cx (x = 0 to 1.25). J. Alloys Comp. 186 135–145 (1992).CrossRefGoogle Scholar
  31. 31.
    Mamontov E., Udovic T. J., Isnard O., Rush J. J.: Neutron scattering study of hydrogen dynamics in Pr2Fe17H5. Phys. Rev. B 70 214305 (2004).CrossRefGoogle Scholar
  32. 32.
    Udovic T., Zhou W., Wu H., Brown C. M., Rush J. J., Yildirim T. Mamontov E., Isnard O.: Neutron vibrational spectroscopy of the Pr2Fe17-based hydrides. J. Alloys Comp. 446–447 504–507 (2007).CrossRefGoogle Scholar
  33. 33.
    Mamontov E., Udovic T. J., Rush J. J., Isnard O.: Dynamics of hydrogen in Pr2Fe17H4 and Pr2Fe17H5. J. Alloys Comp. 422 149–152 (2006).CrossRefGoogle Scholar
  34. 34.
    Mc Intyre G. J., Lemée-Cailleau M. H., Wilkinson C.: High-speed neutron Laue diffraction comes of age. Physica B 385–386 1055–1058 (2006).CrossRefGoogle Scholar
  35. 35.
    Ouladdiaf B., Archer J., McIntyre G. J., Hewat A. W., Brau D., York S.: OrientExpress: A new system for Laue neutron diffraction. Physica B 385–386 1052–1054 (2006).CrossRefGoogle Scholar
  36. 36.
    Chung E. M. L., Lees M. R., McIntyre G. J., Balakrishnan G., Hague J. P., Visser D., Paul D. Mc K., Wilkinson C.: Magnetic properties of tapiolite (FeTa2O6); a quasi two-dimensional (2D) antiferromagnet. J. Phys.: Cond. Matter 16 7837–7852 (2004).CrossRefGoogle Scholar
  37. 37.
    Soubeyroux J. L., Claret N.: Magnetic properties and crystallization behaviour of Fe28.75Co28.75Ni17.5X8B17 (X = Si, Ge) metallic glasses. Physica B 350 e59–e62 (2004).CrossRefGoogle Scholar
  38. 38.
    Soubeyroux J. L., Claret N.: J. Magnetic properties and crystallization behavior of Fe28.75Co28.75Ni17.5X8B17 (X = Si, Ge) metallic glasses. Magn. Magn. Mater. 1379, 272–276 (2004)Google Scholar
  39. 39.
    Soubeyroux J. L., Claret N.: Applied Phys. A 74, S1025–S1027 (2002).CrossRefGoogle Scholar
  40. 40.
    Soubeyroux J. L., Pelletier J. M., Perrier de la Bâthie R.: In situ crystallization of Zirconium-based bulk metallic glasses. Physica B 276–278 905–906 (2000).CrossRefGoogle Scholar
  41. 41.
    Isnard O.: A review of in situ and/or time resolved neutron scattering C.R. Physique 8 789–805 (2007)CrossRefGoogle Scholar
  42. 42.
    Isnard O.: In situ and or time resolved neutron scattering for materials sciences. J. Optoelec. Adv. Mat. 8, 411–417 (2006)CrossRefGoogle Scholar
  43. 43.
    Lyubina J., Isnard O., Gutfleisch O., Müller K. H., Schultz L.: Ordering of nanocrystalline Fe-Pt alloys studied by in situ powder neutron diffraction. J. Appl. Phys. 100 094308 (2006)CrossRefGoogle Scholar
  44. 44.
    Lyubina J., Opahle I., Richter M., Gutfleisch O., Müller K. H., Schultz L., Isnard O.: Influence of composition and order on the magnetism of Fe-Pt alloys: Neutron powder diffraction and theory. Appl. Phys. Letter 89 032506 (2006)CrossRefGoogle Scholar
  45. 45.
    Prokhnenko O., Ritter C., Arnold Z., Isnard O., Kamarad J., Teplykh A., Kuchin A.: Neutron diffraction studies of the magnetic phase transitions in Ce2Fe17 compound under pressure. J. Appl. Phys. 91 385–391(2002).CrossRefGoogle Scholar
  46. 46.
    Prokhnenko O., Arnold Z., Kamarad J., Ritter C., Isnard O., Kuchin A.: Helimagnetic order in the re-entrant ferromagnet Ce2Fe15.3Mn1.7. J. Appl. Phys. 97 113909-1 to 8 (2005)CrossRefGoogle Scholar
  47. 47.
    Kinast E. J., Antonetti V., Schmitt D., Isnard O., da Cunha J. B. M., Gusmao M. A., dos Santos C. A.: Bicriticality in FexCo1-xTa2O6. Phys. Rev. Letters 91 197208 (2003)CrossRefGoogle Scholar
  48. 48.
    Zlotea C., Isnard O.: Neutron powder diffraction and magnetic study of RCo4Ga intermetallic compounds (R = Y and Pr). J. Alloys Comp. 346 29–37 (2002).CrossRefGoogle Scholar
  49. 49.
    Isnard O.: Diffusion, diffraction en temps réel et études réalisées in situ. J. Phys. IV France 103 133–171(2003).CrossRefGoogle Scholar
  50. 50.
    Gutfleisch O., Harris I. R.: Fundamental and practical aspects of the hydrogenation disproportionation, desorption and recombination process. J. phys., D, Appl. phys. 29 2255–2265 (1996).CrossRefGoogle Scholar
  51. 51.
    McGuiness P. J., Zhang X. J., Yin X. J., Harris I. R.: Hydrogenation, disproportionation and desorption (HDD): An effective processing route for Nd---Fe---B-type magnets. J. Less-Common Met. 158 359–365 (1990).CrossRefGoogle Scholar
  52. 52.
    Takeshita T. Nakayama, R.: 10th Int. Workshop on Rare-Earth and Their Applications. Kyoto, Japan 551–557 (1989).Google Scholar
  53. 53.
    Takeshita T.: Present status of the hydrogenation-decomposition-desorption-recombination process as applied to the production of magnets. J. Alloys Comp. 193 231–234 (1993).CrossRefGoogle Scholar
  54. 54.
    Gutfleisch O., Martinez N., Verdier M., Harris I. R.: Phase transformations during the disproportionation stage in the solid HDDR process in a Nd16Fe76B8 alloy. J. Alloys Comp. 215  227–233 (1994).CrossRefGoogle Scholar
  55. 55.
    Liesert S., Fruchart D., de Rango P., Soubeyroux J. L.: The hydrogenation–disproportionation–desorption–recombination process of Nd2Fe14B studied by in-situ neutron diffraction and thermomagnetic measurements. J. Alloys Comp. 253–254 140–143 (1997).CrossRefGoogle Scholar
  56. 56.
    Soubeyroux J. L. Fruchart D., Liesert S., de Rango P., Rivoirard S.:  In situ neutron diffraction study of the HDDR process of Nd---Fe---B magnets. Physica B 241–243 341–343 (1998).Google Scholar
  57. 57.
    Isnard O., Yelon W. B, Miraglia S., Fruchart D.: Neutron diffraction study of the insertion scheme of hydrogen in Nd2Fe14 B. J. Appl. Phys. 78 1892–1898 (1995).Google Scholar
  58. 58.
    Goujon A., Gillon B., Debede A., Cousson A., Gukasov A., Jeftic J., Mc Intyre G. J., Varret F.: Neutron Laue diffraction on the spin crossover crystal [Fe(1-n-propyltetrazole)6](BF 4)2 showing continuous photoinduced transformation. Phys. Rev. B 73 104413 (2006).Google Scholar
  59. 59.
    Goujon A., Gillon B., Gukasov A., Jeftic J., Nau Q., Codjovi E., Varret F.: Photoinduced molecular switching studied by polarized neutron diffraction. Phys. Rev. B 67 220401(R) (2003).Google Scholar
  60. 60.
    de Gennes P. G.: Theory of neutron scattering by magnetic materials Chap. 3 in Magnetism Vol. III. G.T. Rado, H. Suhl (eds.) Academic Press New-York (1963).Google Scholar
  61. 61.
    Cox D. E.: Neutron-Diffraction determination of magnetic structures. IEEE trans. Magn. 8  161–182 (1972).CrossRefGoogle Scholar
  62. 62.
    Rossat-Mignot J.: Magnetic structures Chap. 19 in Neutron Scattering, part C. K. Sköld, L. D. Price (eds.) Academic Press New-York (1987).Google Scholar
  63. 63.
    Hicks T. J.: Experiments with neutron polarization analysis. Adv. Phys. 45 243–298 (1996).CrossRefGoogle Scholar
  64. 64.
    Tasset F.: Magnetic Structures and neutron polarimetry. J. Magn. Magn. Mater. 129 47–52 (1994).CrossRefGoogle Scholar
  65. 65.
    Tasset F.: Zero field neutron polarimetry, Physica B 156–157 627–630 (1992).Google Scholar
  66. 66.
    Mirebeau I., Apetrei A., Rodriguez-Carvajal J., Bonville P., Forget A., Colson,D., Glaskov V., Sanchez J. P., Isnard O., Suard E.: Magnetic order induced by dipolar interactions in the spin liquid Tb2Sn2O7. Phys. Rev. Letters. 94 246402 (2005).CrossRefGoogle Scholar
  67. 67.
    Givord D., Lemaire R.:  Magnetic transition and amorphous thermal expansion in R2Fe17 compounds. IEEE Trans. Magn. Mag-10, 109–113 (1974).CrossRefGoogle Scholar
  68. 68.
    Isnard O., Miraglia S., Fruchart D., Georgetti C., Pizzini S., Dartyge E., Kappler J. P., Krill G.: Magnetic circular X-ray dichroism study of the Ce2Fe17Hx compounds. Phys. Rev. B 49 15692–15701 (1994).CrossRefGoogle Scholar
  69. 69.
    Hautot D., Long G. J., Grandjean F., Isnard O. A. Mössbauer spectral study of the magnetic properties of Ce2Fe17 and its hydrides. Phys. Rev. B 62 11731–11741 (2000).CrossRefGoogle Scholar
  70. 70.
    Prokhnenko O., Ritter C., Arnold Z., Isnard O., Teplikh A., Kamarad J., Pirogov A., Kuchin A.: Effect of pressure and Mn substitution on the magnetic ordering of Ce2Fe17-xMnx Appl. Phys. A. 74 S610–S612 (2002).CrossRefGoogle Scholar
  71. 71.
    Teplykh A., Pirogov A., Kuchin A., Prokhnenko O., Ritter C., Arnold Z., Isnard O.: Magnetic field induced phase transition in Ce2Fe17-xMnx compounds. Appl. Phys. A. 74 S577–S579 (2002)CrossRefGoogle Scholar
  72. 72.
    Moon R., Riste T., Koehler W.: Polarization Analysis of Thermal-Neutron Scattering. Phys. Rev. 181  920–931 (1969).CrossRefGoogle Scholar
  73. 73.
    Ziebeck K. R. A., Brown P. J. J.: Measurement of the paramagnetic response function in the weak itinerant magnetic compound MnSi using polarised neutron scattering. Phys. F 10 2015–2024 (1980).CrossRefGoogle Scholar
  74. 74.
    Nield V. M., Keen D. A.: Diffuse neutron scattering from crystalline materials. Clarendon Press, Oxford (2001).Google Scholar
  75. 75.
    Stewart J. R.: Disordered materials studied using neutron polarization analysis, collection SFN7 (2007) 173–197 EDP Sciences Publ. Paris doi: 10.1051/sfn:2007022Google Scholar
  76. 76.
    Tasset F.: Recent progress in polarised neutron diffraction at ILL and the emergence of a 3He neutron polarisation filter. Physica B 174 506–513 (1991).CrossRefGoogle Scholar
  77. 77.
    Izyumov Yu. A., Naish V. E., Ozerov R. P.: Neutron Diffraction of Magnetic Materials, Consultant Bureau. Plenum Pub. New York (1991).CrossRefGoogle Scholar
  78. 78.
    Cracknell A. P.: Magnetism in crystalline materials. Pergamon Press, New York (1975).Google Scholar
  79. 79.
    Ressouche E.: Investigating molecular magnetism with polarized neutrons. Physica B 267–268 27–36 (1999).CrossRefGoogle Scholar
  80. 80.
    Schweitzer J., Tasset F.: Polarised neutron study of the RCo5 intermetallic compounds. I. The cobalt magnetisation in YCo5. J. Phys. F. 10 2799–2817 (1980).CrossRefGoogle Scholar
  81. 81.
    Steinbeck L., Richter M., Eschrig H.: Itinerant-electron magnetocrystalline anisotropy energy of YCo5 and related compounds. Phys. Rev. B 63, 184431 (2001).CrossRefGoogle Scholar
  82. 82.
    Givord D., Laforest J., Schweizer J.: Temperature dependence of the samarium magnetic form factor in SmCo5. J. Appl. Phys. 50 2008–2010 (1979).CrossRefGoogle Scholar
  83. 83.
    Givord D., Laforest J., Lemaire R.: Polarized neutron study of the itinerant electron metamagnetism in ThCo5. J. Appl. Phys. 50, 7489–7491 (1979).CrossRefGoogle Scholar
  84. 84.
    Givord D., Laforest J., Lemaire R.: Magnetic transition in ThCo5 due to change of Co-moment. Physica B+C 86–88, 204–206 (1977).CrossRefGoogle Scholar
  85. 85.
    Zheludev A., Bonnet M., Ressouche E., Schweizer J., Wan M., Wang H.: Experimental spin density in the first purely organic ferromagnet: the β para-nitrophenyl nitronyl nitroxide. J. Magn. Magn. Mater. 135 147–160 (1994).CrossRefGoogle Scholar
  86. 86.
    Givord D., Li H. S., Tasset F.: Polarized neutron on Y2Fe14B and Nd2Fe14 B. J. Appl. Phys. 57 4100–4102 (1985)Google Scholar
  87. 87.
    Schweizer J., Golhen S., Lelièvre-Berna E., Ouahab L., Pontillon Y., Ressouche E.: Magnetic interactions and spin densities in molecular compounds. Physica B 297 213–220 (2001).CrossRefGoogle Scholar
  88. 88.
    Fermon C., Ott F. Menelle A.: Neutron reflectometry, in X-Ray and Neutron Reflectivity: Principles and Applications. J. Daillant, A. Gibaud (eds.) Springer, Berlin (1999).Google Scholar
  89. 89.
    Ott F.: Neutron scattering on magnetic surfaces. C.R. Phys. 8 763–776 (2007).CrossRefGoogle Scholar
  90. 90.
    Wills A. S., Lelièvre-Berna E., Tasset F., Schweizer J., Ballou R.: Magnetisation distribution measurements from powders using a 3He spin filter. Physica B 356 254–258 (2005).CrossRefGoogle Scholar
  91. 91.
    Brown P. J.: Spherical neutron polarimetry Chap. 5 in Neutron Scattering from magnetic materials. T. Chatterji (eds.) Elsevier, Amsterdam (2006).Google Scholar
  92. 92.
    Guinier A., Fournet G.: Small-Angle Scattering of x-rays. John Wiley, New York (1955).Google Scholar
  93. 93.
    Kostorz G.: in Neutron scattering. G. Korstorz (ed.) Academic, New York 227 (1979).Google Scholar
  94. 94.
    Wiedenmann A.: Small Angle Neutrons Scattering investigations of Magnetic Nanostructures Chap. 10 in Neutron Scattering from magnetic Materials. T. Chatterji (ed.) Elsevier, Amsterdam 473 (2006).Google Scholar
  95. 95.
    Kostorz G.: Small-angle scattering studies of phase separation and defects in inorganic materials. J. Appl. Cryst. 24 444–456 (1991).CrossRefGoogle Scholar
  96. 96.
    Gerold V., Kostorz G.: Small-angle scattering applications to materials science. J. Appl. Cryst. 11  376–404 (1978).CrossRefGoogle Scholar
  97. 97.
    Fujii H., Saga M., Takeda T., Komura S., Okamoto T., Hiroshima S., Sagawa M.: Small angle neutron scattering from Nd15Fe77B8 and Nd15Fe77AlB8 permanents magnets. IEEE trans. Magn. 23 3119–3121 (1987).CrossRefGoogle Scholar
  98. 98.
    Vecchini C., Moze O., Suzuki K., Cadogan J. M., Pranzas K., Michels A., Weissmuller J.: Small angle neutron scattering investigations of spin disorder in nanocomposite soft magnets. J. Alloys Compds. 423 31–36 (2006).CrossRefGoogle Scholar
  99. 99.
    Ito N., Michels A., Kohlbrecher J., Garitaonandia J. S., Suzuki K., Cashion J. D.: Effect of magnetic field annealing on the soft magnetic properties of nanocrystalline materials. J. Magn. Magn. Mater. 316 458–461 (2007).CrossRefGoogle Scholar
  100. 100.
    Kohlbrecher J., Wiedenmann A., Wollenberger H.: SANS investigation of the nano-sized crystalline and magnetic microstructure of Fe-Si-B based alloys. Physica B 213–214 579–581 (1995).CrossRefGoogle Scholar
  101. 101.
    Hermann H., Wiedenmann A., Mattern N., Heinemann A.: SANS study of nanocrystalline Fe3Si particles in amorphous FeSiBCuNb matrix. Physica B 276–277 704–705 (2000).CrossRefGoogle Scholar
  102. 102.
    Ohnuma M., Suzuki J, Funahashi S, Ishigaki T., Kuwano H., Hamaguchi Y.: Small-angle neutron scattering study on Fe-Cu-Nb-Si-B nanocrystalline alloys. Physica B 213–214, 582–584 (1995).CrossRefGoogle Scholar
  103. 103.
    Weissmuller J., Michels A., Barker J. C., Wiedenmann A., Erb U., Shull R. D.: Analysis of the small-angle neutron scattering of nanocrystalline ferromagnets using a micromagnetics model. Phys. Rev. B 63 214414 (2001).CrossRefGoogle Scholar
  104. 104.
    Wiedenmann A.: Magnetically controllable fluids and their applications, Lecture Notes in Physics Vol. 594. S. Odenbach (ed.) 33, Spinger-Verlag, Berlin (2002).Google Scholar
  105. 105.
    Adveev M. V., Aksenov V. L., Balasoiu M., Garamus V. M., Schreyer A., Torok Gy., Rosta L., Bica D., Vekas L.: Comparative analysis of the structure of sterically stabilized ferrofluids on polar carriers by small-angle neutron scattering. J. Coll. Interface Sci. 295 100–107 (2006).CrossRefGoogle Scholar
  106. 106.
    Adveev M. V.: Contrast variation in small-angle scattering experiments on polydisperse and superparamagnetic systems: basic functions approach. J. Appl. Cryst. 40, 56–70 (2007)CrossRefGoogle Scholar
  107. 107.
    Farrell D. F., Ijiri Y., Kelly C. V., Borschers J. A., Rhyne J. J., Ding Y., Majetich S. A.: Small angle neutron scattering study of disordered and crystalline iron nanoparticle assemblies. J. Magn. Magn. Mater. 303 318–322 (2006).CrossRefGoogle Scholar
  108. 108.
    Forgan E. M., Paul D. M., Mook H. A., Timmins P. A., Keller H., Sutton S., Abell J. S.: Observation by neutron diffraction of the magnetic flux lattice in single crystal YBa2Cu3O7-δ. Nature 343  735–737 (1990).CrossRefGoogle Scholar
  109. 109.
    Pannetier M., Ott F., Fermon C., Sanson Y.: Surface diffraction on magnetic nanostructures in thin films using grazing incidence SANS. Physica B 335 54–58(2003).CrossRefGoogle Scholar
  110. 110.
    Rhyne J. J., Salamon M. B., Flynn C. P., Erwin R. W., Borchers J. A.: Magnetic structures of superlattices. J. Magn. Magn. Mater 129 39–46 (1994).CrossRefGoogle Scholar
  111. 111.
    Werner S. A., Rhyne J. J.: in Recent Progress in Random Magnets. E. D. Ryan (ed.) World Scientific, Singapore 237 (1992).Google Scholar
  112. 112.
    Rhyne J. J., Erwin R. W., Borchers J. A., Salamon M. B., Tsui F., Du R., Flynn C. P.: in Science and Technology of nanostructured Magnetic Materials. G. C. Hadjipanayis, G. A. Prinz (eds.) Plenum Press, New York 117 (1991).Google Scholar
  113. 113.
    Beach R. S., Borchers J. A., Matheny A., Erwin R. W., Salamon M. B., Everitt B., Pettit K., Rhyne J. J., Flynn C. P.: Enhanced Curie temperatures and magnetoelastic domains in Dy/Lu superlattices and film. Phys. Rev. Lett. 70 3502–3505 (1993).CrossRefGoogle Scholar
  114. 114.
    Baibich M. N., Broto J. M., Fert A., Nguyen Van Dau F., Petroff F., Eitenne P., Creuzet G., Friederich A., Chazelas J.: Giant magnetoresistance of (001)Fe/(001)Cr magnetic superlattices. Phys. Rev. Lett. 61 2472–2475 (1988).CrossRefGoogle Scholar
  115. 115.
    Majkrzak C. F., Cable J. W., Kwo J., Hong M., McWhan D. B., Yafet Y., Waszczak J. V., Vettier C.: Observation of a magnetic antiphase domain structure with long-range order in a synthetic Gd-Y superlattice. Phys. Rev. Lett. 56, 2700–2702 (1986)CrossRefGoogle Scholar
  116. 116.
    Ott F.: Neutron scattering on magnetic surfaces. C.R. Physique 8  763–776 (2007).CrossRefGoogle Scholar
  117. 117.
    Majkrzak C. F., O’Donovan K. V., Berk N. F.: Polarized neutron reflectometry Chap. 9 in Neutron Scattering from magnetic materials. T. Chatterji (ed). Elsevier, Amsterdam (2006).Google Scholar
  118. 118.
    Kentzinger E., Rücker U., Caliebe W., Goerigk G., Werges F., Nerger S., Voigt J., Schmidt W., Alefeld B., Fermon C., Brückel Th.: Structural and magnetic characterization of Fe/δ-Mn thin films. Physica B 276–278 586–587 (2000).CrossRefGoogle Scholar
  119. 119.
    Nerger S., Kentzinger E., Rücker U., Voigt J., Ott F., Seeck O. H., Brückel Th.: Proximity effects in Fe1−xCox/Mn/Fe1−xCox trilayers. Physica B 297 185–188 (2001).CrossRefGoogle Scholar
  120. 120.
    Lauter H., Lauter-Pasyuk V., Toperverg B., Romashev L., Milyaev M., Krinitsina T., Kravtsov E., Ustinov V., Petrenko A., Aksenov V.: Domains and interface roughness in Fe/Cr multilayers: Influence on the GMR effect. J. Magn. Magn. Mater. 258–259, 338–341 (2003).CrossRefGoogle Scholar
  121. 121.
    Lauter-Pasyuk V., Lauter H. J., Toperverg B., Nikonov O., Kravtsov E., Romashev L., Ustinov V.: Magnetic neutron off-specular scattering for the direct determination of the coupling angle in exchange-coupled multilayers. J. Magn. Magn. Mater. 226–227, 1694–1696 (2001).CrossRefGoogle Scholar
  122. 122.
    Paul A., Kentzinger E., Rücker U., Burgler D. E., Grünberg P.: Measurement and simulation of polarized neutron reflectivity and off-specular scattering from evolving magnetic domain structure in Co/Cu multilayers. Physica B 356 31–35 (2005).CrossRefGoogle Scholar
  123. 123.
    Fermon C., Ott F., Gilles B., Marty, A. Menelle, A., Samson Y., Legoff G., Francinet G.: Towards a 3D magnetometry by neutron reflectometry. Physica B 267 162–167 (1999).CrossRefGoogle Scholar
  124. 124.
    Lauter-Pasyuk V.: Techniques de diffusion des neutrons en incidence rasante Collection SFN7 (2007) 221–240 EDP Sciences Publ. Paris DOI: 10.105/sfn:2007024Google Scholar
  125. 125.
    Chang-Peng Li, Roshchin I. V., Battle X., Viret M., Ott F., Schuller I. K.: Fabrication and structural characterization of highly ordered sub-100-nm planar magnetic nanodot arrays over 1 cm2 coverage area. J. Appl. Phys. 100 074318–25 (2006)CrossRefGoogle Scholar
  126. 126.
    Szuszkiewicz W., Fronc K., Hennion B., Ott F., Aleszkiewicz M.: Magnetic stripe domains in Fe/Fe–N multilayers. J. Alloys Comp. 423  172–175 (2006).CrossRefGoogle Scholar
  127. 127.
    Williams W. G., Boland B. C., Bowden Z. A., Taylor A. D., Culverhouse S., Rainford B. D.: Observation of intermultiplet transitions in rare-earth metal ions by inelastic neutron scattering. J. Phy. F: Met. Phys. 17 L151–L155 (1987).CrossRefGoogle Scholar
  128. 128.
    Balcar E., Lovesey S.W.: Theory of magnetic neutron and photon scattering. Clarendon Press, Oxford (1989).Google Scholar
  129. 129.
    Balcar E., Lovesey S. W.: Neutron-electron spectroscopy of rare-earth ions. J. Phys. C: Solid State Phys. 19 4605–4611 (1986).CrossRefGoogle Scholar
  130. 130.
    Hippert F., Geissler E., Hodeau J. L., Lelièvre-Berna E., Regnard J. R.: Neutron and X-ray spectroscopy. Springer, Dordrecht (2006).CrossRefGoogle Scholar
  131. 131.
    Fulde P., Loewenhaupt M.: Magnetic excitations in crystal-field split 4f systems. Adv. phys. 34  (1986) 589–661.CrossRefGoogle Scholar
  132. 132.
    Loewenhaupt M., Fischer K. H.: Neutron Scattering n heavy fermion and valence fluctuation 4f-systems Chap. 6 in handbook of magnetic materials Vol. 7 503 (1993).Google Scholar
  133. 133.
    Loewenhaupt M., Fischer K. H.: Valence fluctuation and heavy-fermion 4f systems Chap. 105 in Handbook on the physics and chemistry of rare-earths Vol. 16. K. A. Gschneidner and L. Eyring (eds.) North Holland Publisher 1 (1993).Google Scholar
  134. 134.
    Moze, O.: Crystal field effects in intermetallic compounds studied by inelastic neutron scattering, chapter 4 in Handbook of Magnetic Materials, Vol. 11. K. H. J. Buschow (ed.) Elsevier Science Amsterdam 493 (1998).Google Scholar
  135. 135.
    Stirling W. G., Mc Ewen K. A.: Magnetic excitations Chapter 20 in Methods of experimental physics, Vol. 23, Pat. C 189 Academic Press Inc. (1987).Google Scholar
  136. 136.
    Fulde P., Loewenhaupt M.: Spin waves and magnetic excitations, 1. A. S. Borovik-Romanov, S. K. Sinha (eds.) North-Holland, Amsterdam Ch. 6, 367. (1988)Google Scholar
  137. 137.
    Dönni A., Fürrer A., Kitazawa H., Zolliker M.: Neutron Crystalline-Electric-Field Spectroscopy of RPd2A13 (R = Ce, Pr, Nd). J. Phys. Condens. Matter. 9 5921–5933 (1997).CrossRefGoogle Scholar
  138. 138.
    Gasser U., Allenspach P., Fauth F., Henggeler W., Mesot J., Furrer A., Rosenkrants S., Vorederwisch P., Buchgesiter M.: Neutron crystal-field spectroscopy of RNi2B2C (Ho, Er, Tm). Z. Phys. B 101 345–352 (1996).CrossRefGoogle Scholar
  139. 139.
    Loewenhaupt M., Sosnovska I., Frick B.: Ground state multiplet of rare earth 3+ ions in R2Fe14B investigated by inelastic neutron scattering. Phys. Rev. 42 3866–3876 (1990).CrossRefGoogle Scholar
  140. 140.
    Isnard O., Sippel A., Loewenhaupt M., Bewley R.: A high energy inelastic neutron scattering investigation of the Gd-Fe exchange coupling in Gd2Fe17Dx (x = 0, 3 and 5). J. Phys. Cond. Matter 13 1–11 (2001)CrossRefGoogle Scholar
  141. 141.
    Isnard O., Loewenhaupt M., Bewley R.: A high energy inelastic neutron scattering investigation of the Gd-Fe exchange coupling in GdFe11TiDx (x = 0 ,1). Physica B 350 suppl. 1 e31–e33 (2004).CrossRefGoogle Scholar
  142. 142.
    Loewenhaupt M., Sosnovska I.: Exchange and Crystal fields in R2Fe14B studied by inelastic neutron scattering. J. Appl. Phys. 70 5967–5971 (1991).CrossRefGoogle Scholar
  143. 143.
    Loewenhaupt M., Tils P., Buschow K. H. J., Eccleston R. S.: Exchange interactions in Gd-Fe compounds studied by inelastic neutron scattering. J. Magn. Magn. Mater. 152 10–16 (1996).CrossRefGoogle Scholar
  144. 144.
    Loewenhaupt M., Tils P., Buschow K. H. J., Eccleston R. S.: Intersublattice exchange coupling in Gd-Co compounds studied by INS. J. Magn. Magn. Mater. 138, 52–56 (1994).CrossRefGoogle Scholar
  145. 145.
    Tils P., Loewenhaupt M., Buschow K. H. J., Eccleston R. S.: Intersublattice exchange coupling in Gd–Mn compounds studied by INS. J. Alloys Comp. 279 123–126 (1998).CrossRefGoogle Scholar
  146. 146.
    Mirebeau I.:  Magnetic neutron diffraction under high pressure. C.R. Physique 8  737–744 (2007).CrossRefGoogle Scholar
  147. 147.
    Lemée-Cailleau M-H. Kernavanois N., Fak B., Bellisent-Funel M-C.: Proceedings of the Medium pressure advances for neutron scattering. J. Phys. Condens. Matter. 17 (2003)Google Scholar
  148. 148.
    Mignot J. M.: Neutron scattering under extreme conditions. Collection SFN9 (2008) 159–179 EDP Sciences Publ. Paris doi: 10.1051/sfn: 2008012 (2008)Google Scholar
  149. 149.
    Somenkov V. A.: High-pressure neutron scattering over the ages. J. Phys. Condens. Matter. 17 S2991–S3003 (2003).CrossRefGoogle Scholar
  150. 150.
    Goncharenko I. N.: Neutron diffraction experiments in diamond and sapphire anvil cells. High Pressure Res. 24  193–204 (2003).CrossRefGoogle Scholar
  151. 151.
    Goncharenko I. N.: New techniques for high-pressure neutron and x-ray studies. High Press. Res. 27 (1) 183–188 (2007).MathSciNetCrossRefGoogle Scholar
  152. 152.
  153. 153.
    Mirebeau I., Goncharenko I. N., Golosovsky I. V.: Neutron diffraction in Ho(Mn0.9Al0.1)2 under pressure up to 7.8 GPa: Long-range magnetic order induced by pressure in a frustrated system. Phys. Rev. B 64 140401R (2001).CrossRefGoogle Scholar
  154. 154.
    Klotz S., Braden M., Besson M.: Inelastic neutron scattering to very high pressures. J. Hyp. Int. 128 245–254 (2000).CrossRefGoogle Scholar
  155. 155.
    Klotz S., Braden M.: Phys. Spin-phonon coupling in CuGeO3. Rev. Lett. 80 3634–3637 (1998).CrossRefGoogle Scholar
  156. 156.
    Klotz S., Braden M.: Phonon dispersion of bcc Iron to 10 GPa. Phys. Rev. Lett. 85 3209–3212 (2000).CrossRefGoogle Scholar
  157. 157.
    Jyrkkiö T. A., Huiku M. T., Siemensmeyer K., Clausen K. N.: Neutron diffraction studies of nuclear magnetic ordering in copper. J. Low Temp. Phys. 74 435–474 (1989).CrossRefGoogle Scholar
  158. 158.
    Tuoriniemi J. T., Nummila K. K., Vuorinen R. T., Lounasmaa O. V., Metz A., Siemensmeyer K., Steiner M., Lefmann K., Clausen K. N., Rasmussen F. B.: Neutron experiments on antiferromagnetic nuclear order in silver at picokelvin temperatures. Phys. Rev. Lett. 75 3744–3747 (1995).CrossRefGoogle Scholar
  159. 159.
    Goncharenko I. N.: Evidence for a magnetic collapse in the epsilon phase of solid oxygen. Phys. Rev. Lett. 94 205503 (2005)CrossRefGoogle Scholar
  160. 160.
    Goncharenko I. N., Makarova O. A., Ulivi L.: Direct determination of the magnetic structure of the delta phase of oxygen. Phys. Rev. Lett. 93 55502 (2004).CrossRefGoogle Scholar
  161. 161.
    Grenier B., Ziman T.: Modern quantum magnetism by means of neutron scattering. C.R. Physique 8 717–736 (2007).CrossRefGoogle Scholar
  162. 162.
    Mezei F.: New perspectives from new generations of neutron sources. C.R. Physique 8 909–920 (2007)CrossRefGoogle Scholar

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© Springer Science+Business Media, LLC 2009

Authors and Affiliations

  1. 1.Institut Néel, CNRS, Boîte FGrenobleFrance

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